In this paper, we calculate the low-lying spectra of a single-electron magnetic quantum ring with an offcenter Coulomb impurity, where the magnetic field is zero within the ring and constant elsewhere. The impurity, e...In this paper, we calculate the low-lying spectra of a single-electron magnetic quantum ring with an offcenter Coulomb impurity, where the magnetic field is zero within the ring and constant elsewhere. The impurity, either an acceptor or a donor, is located at a distance d as measured from the plane of the ring along the vertical z direction. The magnetic moments are found in order to get visible discontinuities at the points of the ground-state orbital angular momentum L transitions induced by magnetic fields.展开更多
With brief statements of the linear electro-optical modulation and magnetooptical modulation, using the method of resultant of optical amplitude vectors and the methed of Jones matrix, formulas for intensity of transm...With brief statements of the linear electro-optical modulation and magnetooptical modulation, using the method of resultant of optical amplitude vectors and the methed of Jones matrix, formulas for intensity of transmitted light through the optical analyzer of various composition of electro-optical effect with magneto-optical effect are derived. The results show that the output beam from the analyzer carries information on current (or magnetic field), voltage (or electric field), active power and apparent power. When the light beam transmitted through the analyzer are transformed into electric signals, three kinds of information are included: the DC term corresponding to an active power, the term with frequency ω(50 Hz) corresponding to current or voltage, and the term with frequency 2ω(100 Hz) corresponding to an apparnt power.So, we can use the electric filter circuit to pick out the DC component for measuring active power; to pick out the component with frequency ω(50 Hz) for measuring current or voltage; and to pick out the component with frequency 2ω(100 Hz) for measuring apparent power. The paper discusses what quantities are measured when the analyzer is set on certain definite values, and ponts out the optimum selection for various measurements.展开更多
When circularly polarized light travels through a ferrofluid film in the presence of an applied magnetic field, the transmitted light will behave as elliptically polarized light, because of magnetic birefringence and ...When circularly polarized light travels through a ferrofluid film in the presence of an applied magnetic field, the transmitted light will behave as elliptically polarized light, because of magnetic birefringence and dichroism. The angular distribution of the relative intensity of the transmitted light can be obtained using a polarizer, so that the ratio of both the long and short ax- es-as well as the orientation angle of the ellipse, corresponding to the direction of the applied magnetic field--can be deter- mined, and whether the ferrofluids samples are stable during the measurement can be directly judged from the shape of the distribution curves. Thus, the ratio of the amplitudes Ax/Ay and the added phase difference A r can be resolved in the elliptically polarized light, and information on both the magnetic birefringence An and the dichroism Ak can be deduced for the ferrofluid sample. From the orientation angles of both right-handed and left-handed elliptically polarized transmitted light, the direction of the applied magnetic field can be accurately determined. Using circularly polarized light, the magnetic birefringence and dichroism of pure γ-Fe2O3 ferrofluids and γ--Fe2O3/ZnFe2O4 binary ferrofluids were studied. For the binary ferrofluids, a mod- ulating effect on the magnetic birefringence and dichroism was revealed.展开更多
Two types of lanthanide coordination polymers, namely, [Ln(PA)(NO3)(DMA)3]n (Ln=Gd (1), Dy (2), Eu (3), Tb (4)) (type I), and {[Ln2(PA)3(DMF)4]'2DMF} (Ln=Eu (5), Tb (6)) (type II) (PA=P...Two types of lanthanide coordination polymers, namely, [Ln(PA)(NO3)(DMA)3]n (Ln=Gd (1), Dy (2), Eu (3), Tb (4)) (type I), and {[Ln2(PA)3(DMF)4]'2DMF} (Ln=Eu (5), Tb (6)) (type II) (PA=Pamoic acid, DMA=dimethylacetamide, DMF=N,N-dimethylformamide), have been synthesized by the reaction of Ln(NO3)a-6H20 with pamoic acid through layer diffusion method. These complexes were characterized by single crystal X-ray diffraction, infrared spectroscopy (IR), thermogravimetric analysis (TGA), fluorescence and magnetic measurements. Solvents and lanthanide atoms in the reaction play an important role in controlling different structures. Type I demonstrated 1-D linear chain structure connected by Ln atoms and PA ligands. Type II exhibited non-interpenetrating 3-D 6-connected 43612 nets based on binuclear [Ln2(CO2)6(DMF)4] cores. Magnetic properties of complexes 1-4 were investigated in details. Complex 1 shows significant magnetocaloric effect with -△Sm=20.37 J kg^-1 K^-1 at 3.0 K and 7 T. Complex 2 exhibits slow relaxation of the magnetization. Complexes 3-6 exhibit both ligand- and metal-centered fluorescent properties. Complex 6 demonstrates fluorescent sensing of DMF and Cu^2+ ion.展开更多
Mixed-valence manganites have attracted considerable research focus in recent years not only because of the potential application of colossal magnetoresistance(CMR) in magnetic devices,but also because of many intrigu...Mixed-valence manganites have attracted considerable research focus in recent years not only because of the potential application of colossal magnetoresistance(CMR) in magnetic devices,but also because of many intriguing physical properties observed in these materials.Doping elements at A-site can alter the filling of 3d Mn band and the tolerance factor.Therefore the hole-and electron-doped CMR manganites exhibit a rich phase diagram.In addition,more theoretical and experimental results suggest that phase separation is a critical factor for the understanding of CMR phenomena.Recently,there is an increasing interest in the fabrication and investigation on manganite-based heterojunction,which demonstrated excellent rectifying property,large MR,and photovoltaic effect.展开更多
Exchange bias between ferromagnetic and antiferromagnetic layers has been widely utilized in spintronic devices.Controlling the exchange bias in magnetic multilayers by an electric field(E-field)has been proposed as a...Exchange bias between ferromagnetic and antiferromagnetic layers has been widely utilized in spintronic devices.Controlling the exchange bias in magnetic multilayers by an electric field(E-field)has been proposed as a low-power solution for manipulating the macroscopic properties such as exchange bias fields and magnetization values,while how the magnetic domains respond to the E-fields has rarely been reported in an exchange-biased system.Here,we realize the vector imaging of reversible electrical modulation of magnetization reversal in exchange-biased CoFeB/IrMn/PMN-PT(011)multiferroic heterostructures,utilizing in-situ quantitative magneto-optical Kerr effect(MOKE)microscopy.Under the electrical control,magnetic domains at-80 Oe rotate reversibly between around 160°and 80°-120°,whose transverse components reverse from 225°to 45°correspondingly.Moreover,pixel-by-pixel comparisons are conducted to further imply the reversible magnetization reversal by E-fields.Efield-induced reversible magnetization reversal is also demonstrated without applying external magnetic fields.Vector imaging of electrical manipulation of exchange bias is of great significance in understanding the magnetoelectric effect and the development of next-generation spintronic devices.展开更多
To solve the problems encountered in practical processes of magneto-optical sensing, the infinitesimal distributed-parameter model and finite-element accumulation of different dielectric properties of micromaterials w...To solve the problems encountered in practical processes of magneto-optical sensing, the infinitesimal distributed-parameter model and finite-element accumulation of different dielectric properties of micromaterials were used to describe the evolution of light polarization states, instead of the previously commonly used method of lumped-parameter simulation, thus essentially explaining the mechanism of sensing, magneto-optical effects, and related factors, and achieving multiphysics coupling using the COMSOL finite-element analysis method. Considering the cases of the Faraday effect without and with line birefringence, the magneto-optical effect and output characteristics of an infinitesimal magneto-optical sensor were simulated and studied. The results verified the effectiveness of the infinitesimal sensor model. Because the magnetic field, stress, and temperature changes alter the dielectric properties of magneto-optical materials, the finite-element accumulation method lays a good foundation for research on theoretical analysis and performance of magneto-optical sensors affected by factors such as the magnetic field, temperature, and stress.展开更多
Because of the toxicity of Gd(Ⅲ)complexes and the poor T1 magnetic resonance imaging(MRI)contrast of superparamagnetic iron oxide,the development of new stable,non-toxic,and efficient contrast agents is desirable.Her...Because of the toxicity of Gd(Ⅲ)complexes and the poor T1 magnetic resonance imaging(MRI)contrast of superparamagnetic iron oxide,the development of new stable,non-toxic,and efficient contrast agents is desirable.Herein,tannic acid(TA),a large natural polyphenol,and bovine serum albumin(BSA)were used to construct non-toxic Fe(Ⅲ)complexes with increased relaxivity based on a strategy slowing the molecular spin.Compared with the commercial T1 contrast agent Magnevist■,TA-Fe@BSA not only exhibits comparable T1 MRI contrast enhancement under 0.5,1 and 7 T magnetic fields both in vitro and in vivo,but also has better stability and biocompatibility.Moreover,TA-Fe@BSA with near-infrared(NIR)absorption demonstrates efficient tumor ablation via photothermal effects.These results demonstrate their strong potential as an alternative T1 MRI contrast agent and tumor theranostics agent in clinical settings.展开更多
基金The project supported by National Natural Science Foundation of China under Grant Nos. 50371058 and 90103028
文摘In this paper, we calculate the low-lying spectra of a single-electron magnetic quantum ring with an offcenter Coulomb impurity, where the magnetic field is zero within the ring and constant elsewhere. The impurity, either an acceptor or a donor, is located at a distance d as measured from the plane of the ring along the vertical z direction. The magnetic moments are found in order to get visible discontinuities at the points of the ground-state orbital angular momentum L transitions induced by magnetic fields.
文摘With brief statements of the linear electro-optical modulation and magnetooptical modulation, using the method of resultant of optical amplitude vectors and the methed of Jones matrix, formulas for intensity of transmitted light through the optical analyzer of various composition of electro-optical effect with magneto-optical effect are derived. The results show that the output beam from the analyzer carries information on current (or magnetic field), voltage (or electric field), active power and apparent power. When the light beam transmitted through the analyzer are transformed into electric signals, three kinds of information are included: the DC term corresponding to an active power, the term with frequency ω(50 Hz) corresponding to current or voltage, and the term with frequency 2ω(100 Hz) corresponding to an apparnt power.So, we can use the electric filter circuit to pick out the DC component for measuring active power; to pick out the component with frequency ω(50 Hz) for measuring current or voltage; and to pick out the component with frequency 2ω(100 Hz) for measuring apparent power. The paper discusses what quantities are measured when the analyzer is set on certain definite values, and ponts out the optimum selection for various measurements.
基金supported by the National Natural Science Foundation of China (Grant No. 11074205)
文摘When circularly polarized light travels through a ferrofluid film in the presence of an applied magnetic field, the transmitted light will behave as elliptically polarized light, because of magnetic birefringence and dichroism. The angular distribution of the relative intensity of the transmitted light can be obtained using a polarizer, so that the ratio of both the long and short ax- es-as well as the orientation angle of the ellipse, corresponding to the direction of the applied magnetic field--can be deter- mined, and whether the ferrofluids samples are stable during the measurement can be directly judged from the shape of the distribution curves. Thus, the ratio of the amplitudes Ax/Ay and the added phase difference A r can be resolved in the elliptically polarized light, and information on both the magnetic birefringence An and the dichroism Ak can be deduced for the ferrofluid sample. From the orientation angles of both right-handed and left-handed elliptically polarized transmitted light, the direction of the applied magnetic field can be accurately determined. Using circularly polarized light, the magnetic birefringence and dichroism of pure γ-Fe2O3 ferrofluids and γ--Fe2O3/ZnFe2O4 binary ferrofluids were studied. For the binary ferrofluids, a mod- ulating effect on the magnetic birefringence and dichroism was revealed.
基金supported by the National Natural Science Foundation of China(21571092,21403102)the Natural Science Foundation of Shandong Province(ZR2012BQ023)the University Scientific Research Development Plan of the Education Department of Shandong Province(J14LC10)
文摘Two types of lanthanide coordination polymers, namely, [Ln(PA)(NO3)(DMA)3]n (Ln=Gd (1), Dy (2), Eu (3), Tb (4)) (type I), and {[Ln2(PA)3(DMF)4]'2DMF} (Ln=Eu (5), Tb (6)) (type II) (PA=Pamoic acid, DMA=dimethylacetamide, DMF=N,N-dimethylformamide), have been synthesized by the reaction of Ln(NO3)a-6H20 with pamoic acid through layer diffusion method. These complexes were characterized by single crystal X-ray diffraction, infrared spectroscopy (IR), thermogravimetric analysis (TGA), fluorescence and magnetic measurements. Solvents and lanthanide atoms in the reaction play an important role in controlling different structures. Type I demonstrated 1-D linear chain structure connected by Ln atoms and PA ligands. Type II exhibited non-interpenetrating 3-D 6-connected 43612 nets based on binuclear [Ln2(CO2)6(DMF)4] cores. Magnetic properties of complexes 1-4 were investigated in details. Complex 1 shows significant magnetocaloric effect with -△Sm=20.37 J kg^-1 K^-1 at 3.0 K and 7 T. Complex 2 exhibits slow relaxation of the magnetization. Complexes 3-6 exhibit both ligand- and metal-centered fluorescent properties. Complex 6 demonstrates fluorescent sensing of DMF and Cu^2+ ion.
基金supported by the National Natural Science Foundation of China(Grant Nos.10774146,10974205,10904150 and 11274313)Anhui Provincial Natural Science Foundation(Grant No.1208085MA06)+1 种基金Joint Funds of the National Natural Science Foundation of China and the Chinese Academy of Sciences' Large-scale Scientific Facility(Grant No. U1232138)support by the National Key Basic Research(Grant No. 2011CBA00111)
文摘Mixed-valence manganites have attracted considerable research focus in recent years not only because of the potential application of colossal magnetoresistance(CMR) in magnetic devices,but also because of many intriguing physical properties observed in these materials.Doping elements at A-site can alter the filling of 3d Mn band and the tolerance factor.Therefore the hole-and electron-doped CMR manganites exhibit a rich phase diagram.In addition,more theoretical and experimental results suggest that phase separation is a critical factor for the understanding of CMR phenomena.Recently,there is an increasing interest in the fabrication and investigation on manganite-based heterojunction,which demonstrated excellent rectifying property,large MR,and photovoltaic effect.
基金supported by the National Key R&D Program of China(2018YFB0407601)the National Natural Science Foundation of China(91964109,62071374 and 51802248)the National 111 Project of China(B14040).
文摘Exchange bias between ferromagnetic and antiferromagnetic layers has been widely utilized in spintronic devices.Controlling the exchange bias in magnetic multilayers by an electric field(E-field)has been proposed as a low-power solution for manipulating the macroscopic properties such as exchange bias fields and magnetization values,while how the magnetic domains respond to the E-fields has rarely been reported in an exchange-biased system.Here,we realize the vector imaging of reversible electrical modulation of magnetization reversal in exchange-biased CoFeB/IrMn/PMN-PT(011)multiferroic heterostructures,utilizing in-situ quantitative magneto-optical Kerr effect(MOKE)microscopy.Under the electrical control,magnetic domains at-80 Oe rotate reversibly between around 160°and 80°-120°,whose transverse components reverse from 225°to 45°correspondingly.Moreover,pixel-by-pixel comparisons are conducted to further imply the reversible magnetization reversal by E-fields.Efield-induced reversible magnetization reversal is also demonstrated without applying external magnetic fields.Vector imaging of electrical manipulation of exchange bias is of great significance in understanding the magnetoelectric effect and the development of next-generation spintronic devices.
基金supported by the National Natural Science Foundation of China(Grant No.51277066)
文摘To solve the problems encountered in practical processes of magneto-optical sensing, the infinitesimal distributed-parameter model and finite-element accumulation of different dielectric properties of micromaterials were used to describe the evolution of light polarization states, instead of the previously commonly used method of lumped-parameter simulation, thus essentially explaining the mechanism of sensing, magneto-optical effects, and related factors, and achieving multiphysics coupling using the COMSOL finite-element analysis method. Considering the cases of the Faraday effect without and with line birefringence, the magneto-optical effect and output characteristics of an infinitesimal magneto-optical sensor were simulated and studied. The results verified the effectiveness of the infinitesimal sensor model. Because the magnetic field, stress, and temperature changes alter the dielectric properties of magneto-optical materials, the finite-element accumulation method lays a good foundation for research on theoretical analysis and performance of magneto-optical sensors affected by factors such as the magnetic field, temperature, and stress.
基金the National Natural Science Foundation of China(91959105 and 21671135)Shanghai Sailing Program(19YF1436200)+2 种基金Shanghai Rising-Star Program(17QA1402600)Shanghai Talent Development Fund(2018082)Shanghai Engineering Research Center of Green Energy Chemical Engineering(18DZ2254200)。
文摘Because of the toxicity of Gd(Ⅲ)complexes and the poor T1 magnetic resonance imaging(MRI)contrast of superparamagnetic iron oxide,the development of new stable,non-toxic,and efficient contrast agents is desirable.Herein,tannic acid(TA),a large natural polyphenol,and bovine serum albumin(BSA)were used to construct non-toxic Fe(Ⅲ)complexes with increased relaxivity based on a strategy slowing the molecular spin.Compared with the commercial T1 contrast agent Magnevist■,TA-Fe@BSA not only exhibits comparable T1 MRI contrast enhancement under 0.5,1 and 7 T magnetic fields both in vitro and in vivo,but also has better stability and biocompatibility.Moreover,TA-Fe@BSA with near-infrared(NIR)absorption demonstrates efficient tumor ablation via photothermal effects.These results demonstrate their strong potential as an alternative T1 MRI contrast agent and tumor theranostics agent in clinical settings.