Metastable 40Ar＊ atoms are produced in the two metastable states 3p54s [3/2]2 and 3p5 4s′ [1/2]0 in a pulsed DC discharge in a beam, and are subsequently excited to the even-parity autoionizing resonance series 3pSn...Metastable 40Ar＊ atoms are produced in the two metastable states 3p54s [3/2]2 and 3p5 4s′ [1/2]0 in a pulsed DC discharge in a beam, and are subsequently excited to the even-parity autoionizing resonance series 3pSnp′[3/2]1,2, 3p5 np′ [1/2]1, and 3p5nf′[5/2]3 using single photon excitation with a pulsed dye laser. The excitation spectra of the even-parity autoion- izing resonance series from the metastable 40Ar＊ are obtained by recording the autoionized Ar＋ ions with time-of-flight ion detection in the photon energy range of 32500-35600 cm-1 with an experimental bandwidth of 〈0.1 cm-1. A wealth of autoionizing resonances are newly observed, from which more precise and systematic spectroscopic data of the level energies and quantum defects are derived.展开更多
Sliced velocity mapping ion imaging technique was employed to investigate the dynamics of the hydroxyl elimination channel in the photodissociaiton of nitric acid in the ultraviolet region. The OH product was detected...Sliced velocity mapping ion imaging technique was employed to investigate the dynamics of the hydroxyl elimination channel in the photodissociaiton of nitric acid in the ultraviolet region. The OH product was detected by （2＋1） resonance enhanced multiphoton ionization via the D^2∑^- electronic state. The total kinetic energy spectra of the OH＋NO2 channel from the photolysis of HONO2 show that both ：NO2（X2A1） and NO2（A2B2） channels are present, suggesting that both 1^1A″ and 2^1A″ excited electronic states of HONO2 are involved in the excitation. The parallel angular distributions suggest that the dissociation of the nitric acid is a fast process in comparison with the rotational period of the HNO3 molecule. The anisotropy parameter β for the hydroxyl elimination channel is found to be dependent on the OH product rotational state as well as the photolysis energy.展开更多
The even-parity autoionizing resonance series 4p^5np＇ [3/2] 1,2, [ 1/2] 1, and 4p^2nf＇ [5/213 of krytpon have been investigated by laser excitation from the two metastable states 4p55s [3/2]2 and 4p^55s＇ [1/2]0 in ...The even-parity autoionizing resonance series 4p^5np＇ [3/2] 1,2, [ 1/2] 1, and 4p^2nf＇ [5/213 of krytpon have been investigated by laser excitation from the two metastable states 4p55s [3/2]2 and 4p^55s＇ [1/2]0 in the photon energy region of 2900（P40000 cm^-1 at experimental bandwidth of -0.1 cm-1. The excitation spectra of the even-parity autoionizing resonance series, most of which are experimentally studied for the first time in this work, show typical asymmetric line shapes. Complementary information on level energies, quantum defects, line profile indices and resonance widths, resonance lifetimes and reduced widths of the auto- ionizing resonances are derived by Fano-type line-shape analyses of the experimental results. Results from this work indicate that the line profile index （q） and the resonance width （F） are approximately proportional to the effective principal quantum number （n＊）; the line separation of the 4p^5np＇ autoionizing resonances is also in good agreement with theoretical model展开更多
Cooling is very important for the safe operation of an electron cyclotron resonance ion source(ECRIS),especially when the window current density is very high(up to 11 A/mm2).We proposed an innovative cooling method us...Cooling is very important for the safe operation of an electron cyclotron resonance ion source(ECRIS),especially when the window current density is very high(up to 11 A/mm2).We proposed an innovative cooling method using evaporative cooling technology.A demonstration prototype was designed,built and tested.The on-site test results showed that the temperature of the solenoids and permanent magnets maintains well in the normal operational range of 14–18 GHz.A simple computational model was developed to predict the characteristics of the two-phase flow.The predicted temperatures agreed well with the on-site test data within 2 K.We also proposed useful design criteria.The successful operation of the system indicates the potential for broad application of evaporative cooling technology in situations in which the power intensity is very high.展开更多
文摘Metastable 40Ar＊ atoms are produced in the two metastable states 3p54s [3/2]2 and 3p5 4s′ [1/2]0 in a pulsed DC discharge in a beam, and are subsequently excited to the even-parity autoionizing resonance series 3pSnp′[3/2]1,2, 3p5 np′ [1/2]1, and 3p5nf′[5/2]3 using single photon excitation with a pulsed dye laser. The excitation spectra of the even-parity autoion- izing resonance series from the metastable 40Ar＊ are obtained by recording the autoionized Ar＋ ions with time-of-flight ion detection in the photon energy range of 32500-35600 cm-1 with an experimental bandwidth of 〈0.1 cm-1. A wealth of autoionizing resonances are newly observed, from which more precise and systematic spectroscopic data of the level energies and quantum defects are derived.
基金Ⅴ. ACKNOWLEDGMENTS This work was supported by the National Natural Science Foundation of China, the Ministry of Sciences and Technology, and the Chinese Academy of Sciences.
文摘Sliced velocity mapping ion imaging technique was employed to investigate the dynamics of the hydroxyl elimination channel in the photodissociaiton of nitric acid in the ultraviolet region. The OH product was detected by （2＋1） resonance enhanced multiphoton ionization via the D^2∑^- electronic state. The total kinetic energy spectra of the OH＋NO2 channel from the photolysis of HONO2 show that both ：NO2（X2A1） and NO2（A2B2） channels are present, suggesting that both 1^1A″ and 2^1A″ excited electronic states of HONO2 are involved in the excitation. The parallel angular distributions suggest that the dissociation of the nitric acid is a fast process in comparison with the rotational period of the HNO3 molecule. The anisotropy parameter β for the hydroxyl elimination channel is found to be dependent on the OH product rotational state as well as the photolysis energy.
基金financially supported by the National Natural Science Foundation of China(51007092)
文摘The even-parity autoionizing resonance series 4p^5np＇ [3/2] 1,2, [ 1/2] 1, and 4p^2nf＇ [5/213 of krytpon have been investigated by laser excitation from the two metastable states 4p55s [3/2]2 and 4p^55s＇ [1/2]0 in the photon energy region of 2900（P40000 cm^-1 at experimental bandwidth of -0.1 cm-1. The excitation spectra of the even-parity autoionizing resonance series, most of which are experimentally studied for the first time in this work, show typical asymmetric line shapes. Complementary information on level energies, quantum defects, line profile indices and resonance widths, resonance lifetimes and reduced widths of the auto- ionizing resonances are derived by Fano-type line-shape analyses of the experimental results. Results from this work indicate that the line profile index （q） and the resonance width （F） are approximately proportional to the effective principal quantum number （n＊）; the line separation of the 4p^5np＇ autoionizing resonances is also in good agreement with theoretical model
基金supported by the Open Research Project of the Major Science and Technology Infrastructure in the Chinese Academy of Sciences-Application of Evaporative Cooling Technology in the Field of Accelerator
文摘Cooling is very important for the safe operation of an electron cyclotron resonance ion source(ECRIS),especially when the window current density is very high(up to 11 A/mm2).We proposed an innovative cooling method using evaporative cooling technology.A demonstration prototype was designed,built and tested.The on-site test results showed that the temperature of the solenoids and permanent magnets maintains well in the normal operational range of 14–18 GHz.A simple computational model was developed to predict the characteristics of the two-phase flow.The predicted temperatures agreed well with the on-site test data within 2 K.We also proposed useful design criteria.The successful operation of the system indicates the potential for broad application of evaporative cooling technology in situations in which the power intensity is very high.
