We have adapted and characterized electrolysis reactors to complement the conversion of regional- and community-scale quantities of waste into fuel or chemicals, The overall process must he able to contend with a wide...We have adapted and characterized electrolysis reactors to complement the conversion of regional- and community-scale quantities of waste into fuel or chemicals, The overall process must he able to contend with a wide range of feedstocks, must he inherently safe, and should not rely on external facilities for co-reactants or heat rejection and supply, Our current approach is based on the upgrading of hio-oil produced by the hydrothermal liquefaction (HTL) of carbon-containing waste feedstocks, HTL can convert a variety of feedstocks into a bio-oil that requires much less upgrading than the products of other ways of deconstructing hiomass, We are now investigating the use of electrochemical processes for the further conversions needed to transform the hio-oil from HTL into fuel or higher value chemicals, We, and others, have shown that electrochemical reduction can offer adequate reaction rates and at least some of the nec- essary generality, In addition, an electrochemical reactor necessarily both oxidizes (removes electrons) on one side of the reactor and reduces (adds electrons) on the other side, Therefore, the two types of reac- tions could, in principle, he coupled to upgrade the hio-oil and simultaneously polish the water that is employed as a reactant and a carrier in the upstream HTL, Here, we overview a notional process, the possible conversion chemistry, and the economics of an HTL-electrochemical process,展开更多
From a multi-dimensional perspective of economic development,carbon dioxide and industrial pollutant emission and resource consumption in the case study of Shenyang,this paper analyzes the resource consumption and env...From a multi-dimensional perspective of economic development,carbon dioxide and industrial pollutant emission and resource consumption in the case study of Shenyang,this paper analyzes the resource consumption and environmental impact in the process of urban economic development and low-carbon transition and evaluates the emission reduction potential and scenario of various technologies. The results show that city plays a key role in global low-carbon economic construction,and it is pointed out that emission reduction technology in urban scale can reduce total amount of carbon emission to substantial extent. From the aspect of future development,the input of technology and economic growth pattern should be strengthened so as to realize economic development as well as the total amount reduction of pollutant emission.展开更多
Although the relationship between the size of urban industrial land use and pollutant emissions has been widely discussed from different perspectives(e.g.,the scale and crowding effects),the results of various studies...Although the relationship between the size of urban industrial land use and pollutant emissions has been widely discussed from different perspectives(e.g.,the scale and crowding effects),the results of various studies have revealed positive,negative,and combined impact relationships.However,how the expansion of urban industrial land use affects SO_(2) emissions remains unknown.We need to clarify this relationship in order to facilitate the realization of China’s pollution reduction and emission reduction goals.This study used the panel data from 294 cities spanning from 2011 to 2019 to construct a spatial econometric model.The objective was to explore the correlation between the scale of urban industrial land and sulfur dioxide emissions in China.The results show that a large scale of urban industrial land use corresponds to lower sulfur dioxide emissions per unit of industrial added value.By gaining a deeper understanding of the relationship between the scale of urban industrial land use and sulfur dioxide emissions,policymakers can further reduce pollutant emissions by rationalizing the planning of urban industrial land use and industrial layout.In addition to promoting industrial agglomeration and economies of scale in cities with extensive industrial land use,this strategy can support the development of efficient and environmentally friendly industries in areas with limited industrial land use.Optimizing the technology and encouraging the development of green industries can help reduce environmental pollution and promote sustainable urban development.展开更多
基金supported by the Laboratory Directed Research & Development program at Pacific Northwest National Laboratory (PNNL)
文摘We have adapted and characterized electrolysis reactors to complement the conversion of regional- and community-scale quantities of waste into fuel or chemicals, The overall process must he able to contend with a wide range of feedstocks, must he inherently safe, and should not rely on external facilities for co-reactants or heat rejection and supply, Our current approach is based on the upgrading of hio-oil produced by the hydrothermal liquefaction (HTL) of carbon-containing waste feedstocks, HTL can convert a variety of feedstocks into a bio-oil that requires much less upgrading than the products of other ways of deconstructing hiomass, We are now investigating the use of electrochemical processes for the further conversions needed to transform the hio-oil from HTL into fuel or higher value chemicals, We, and others, have shown that electrochemical reduction can offer adequate reaction rates and at least some of the nec- essary generality, In addition, an electrochemical reactor necessarily both oxidizes (removes electrons) on one side of the reactor and reduces (adds electrons) on the other side, Therefore, the two types of reac- tions could, in principle, he coupled to upgrade the hio-oil and simultaneously polish the water that is employed as a reactant and a carrier in the upstream HTL, Here, we overview a notional process, the possible conversion chemistry, and the economics of an HTL-electrochemical process,
基金Key Program of National Natural Science Foundation of China(No.71033004)Post-doctor Foundation of Chinese Academy of Sciences,Institute of Applied Ecology(No.Y0SBS161S3)
文摘From a multi-dimensional perspective of economic development,carbon dioxide and industrial pollutant emission and resource consumption in the case study of Shenyang,this paper analyzes the resource consumption and environmental impact in the process of urban economic development and low-carbon transition and evaluates the emission reduction potential and scenario of various technologies. The results show that city plays a key role in global low-carbon economic construction,and it is pointed out that emission reduction technology in urban scale can reduce total amount of carbon emission to substantial extent. From the aspect of future development,the input of technology and economic growth pattern should be strengthened so as to realize economic development as well as the total amount reduction of pollutant emission.
基金The Yunnan Fundamental Research Projects(202301AT070062,202401AT070108,202401AS070037)The Key Program of the NationalNatural Science Foundation of China(42130712)+2 种基金The Scientific Research Fund Project of Yunnan Provincial Department of Education(2024Y155)The Yunnan Province Innovation Team Project(202305AS350003)The Yunnan Revitalization Talent Support Program in YunnanProvince(XDYC-QNRC-2022-0740,XDYC-WHMJ-2022-0016).
文摘Although the relationship between the size of urban industrial land use and pollutant emissions has been widely discussed from different perspectives(e.g.,the scale and crowding effects),the results of various studies have revealed positive,negative,and combined impact relationships.However,how the expansion of urban industrial land use affects SO_(2) emissions remains unknown.We need to clarify this relationship in order to facilitate the realization of China’s pollution reduction and emission reduction goals.This study used the panel data from 294 cities spanning from 2011 to 2019 to construct a spatial econometric model.The objective was to explore the correlation between the scale of urban industrial land and sulfur dioxide emissions in China.The results show that a large scale of urban industrial land use corresponds to lower sulfur dioxide emissions per unit of industrial added value.By gaining a deeper understanding of the relationship between the scale of urban industrial land use and sulfur dioxide emissions,policymakers can further reduce pollutant emissions by rationalizing the planning of urban industrial land use and industrial layout.In addition to promoting industrial agglomeration and economies of scale in cities with extensive industrial land use,this strategy can support the development of efficient and environmentally friendly industries in areas with limited industrial land use.Optimizing the technology and encouraging the development of green industries can help reduce environmental pollution and promote sustainable urban development.