Here we used Empirical Mode Decomposition (EMD) method to study seasonal variability and nonlinear trend of corrected AERONET Aerosol Optical Depth (AOD/Hi) and corrected PM10 mass concentrations (PMmxf(RH)) i...Here we used Empirical Mode Decomposition (EMD) method to study seasonal variability and nonlinear trend of corrected AERONET Aerosol Optical Depth (AOD/Hi) and corrected PM10 mass concentrations (PMmxf(RH)) in Hong Kong during 2005-2011. AODPrli is highly correlated with PMI0xf(RH) in semi-annual and annual time scales (with correlation coefficient 0.67 for semi-annual and 0.79 for annual components, 95% confidence interval). On the semi-annual scale, both AOD/Hi and PM10xf(RH) can capture the two maxima in March and October, respectively, with much stronger amplitude in March proba- bly due to the long-range transport of dust storm. On the annual cycle, the AOD/Hi and PMI0xf(RH), which are negatively correlated with the precipitation and solar radiation, vary coherently with the maxima in February. This annual peak occurs about one month earlier than the first peak of the semi-annual variability in March, but with only half amplitude. During 2005-2011, both AOD/Hi and PM10xf(RH) exhibit the pronounced decreasing trend with the mean rate of 14 gg m-3 per year for PM10xf(RH), which reflects the significant effects of the air pollution control policy in Hong Kong during the past decade. The nonlinear trend analysis indicates that the decreasing of PM10xf(RH) is slower than that of AOD/Hi when the AOD/Hi is less than 0.44 but becomes faster when the AOD/Hi exceeds 0.44. These results illustrate that the AERONET AOD can be used quantitatively to estimate local air-quality variability on the semi-annual, annual, and long-term trend time scales.展开更多
基金sponsored by the National Natural Science Foundation of China(Grant No.41206027)the China Postdoctoral Science Foundation(Grant No.2012M511460)+1 种基金the Key Laboratory of Global Change and Marine-Atmospheric Chemistry(Grant No.GCMAC1205)the Public Science and Technology Research Funds Projects of Ocean(Grant No.201105019)
文摘Here we used Empirical Mode Decomposition (EMD) method to study seasonal variability and nonlinear trend of corrected AERONET Aerosol Optical Depth (AOD/Hi) and corrected PM10 mass concentrations (PMmxf(RH)) in Hong Kong during 2005-2011. AODPrli is highly correlated with PMI0xf(RH) in semi-annual and annual time scales (with correlation coefficient 0.67 for semi-annual and 0.79 for annual components, 95% confidence interval). On the semi-annual scale, both AOD/Hi and PM10xf(RH) can capture the two maxima in March and October, respectively, with much stronger amplitude in March proba- bly due to the long-range transport of dust storm. On the annual cycle, the AOD/Hi and PMI0xf(RH), which are negatively correlated with the precipitation and solar radiation, vary coherently with the maxima in February. This annual peak occurs about one month earlier than the first peak of the semi-annual variability in March, but with only half amplitude. During 2005-2011, both AOD/Hi and PM10xf(RH) exhibit the pronounced decreasing trend with the mean rate of 14 gg m-3 per year for PM10xf(RH), which reflects the significant effects of the air pollution control policy in Hong Kong during the past decade. The nonlinear trend analysis indicates that the decreasing of PM10xf(RH) is slower than that of AOD/Hi when the AOD/Hi is less than 0.44 but becomes faster when the AOD/Hi exceeds 0.44. These results illustrate that the AERONET AOD can be used quantitatively to estimate local air-quality variability on the semi-annual, annual, and long-term trend time scales.