The structure and working principle of a self-deigned high pressure electronic pneumatic pressure reducing valve (EPPRV) with slide pilot are introduced.The resistance value formulas and the relationship between the r...The structure and working principle of a self-deigned high pressure electronic pneumatic pressure reducing valve (EPPRV) with slide pilot are introduced.The resistance value formulas and the relationship between the resistance and pressure of three typical pneumatic resistances are obtained.Then,the method of static characteristics analysis only considering pneumatic resistances is proposed,the resistance network from gas supply to load is built up,and the mathematical model is derived from the flow rate formulas and flow conservation equations,with the compressibility of high pressure gas and temperature drop during the expansion considered in the model.Finally,the pilot spool displacement of 1.5 mm at an output pressure of 15MPa and the enlarging operating stroke of the pilot spool are taken as optimization targets,and the optimization is carried out based on genetic algorithm and the model mentioned above.The results show that the static characteristics of the EPPRV are significantly improved.The idea of static characteristics analysis and optimization based on pneumatic resistance network is valuable for the design of pneumatic components or system.展开更多
We propose a probabilistic scheme for realizing teleportation of bipartite photonic states using linear optical elements where only requires a two-photon Bell state used as quantum channel. It reduces the requirement ...We propose a probabilistic scheme for realizing teleportation of bipartite photonic states using linear optical elements where only requires a two-photon Bell state used as quantum channel. It reduces the requirement of the entanglement of quantum channel, but requires an additional photon and an auxiliary maximally entangled photon pair locally.展开更多
In 3-mode Fock space we find a new tripartite entangled state |α,γ 】 λ,which make up a new quantum mechanical representation. The state |α,γ 】 λ, can be generated byusing the setup composing of a beam splitter...In 3-mode Fock space we find a new tripartite entangled state |α,γ 】 λ,which make up a new quantum mechanical representation. The state |α,γ 】 λ, can be generated byusing the setup composing of a beam splitter and a parametric down-conversion amplifier. Applicationof the state is briefly discussed.展开更多
Photocatalytic oxidative organic reactions are important synthetic transformations,and research on reaction selectivity by reactive oxygen species(ROS)is significant.To date,however,there has rarely been any focus on ...Photocatalytic oxidative organic reactions are important synthetic transformations,and research on reaction selectivity by reactive oxygen species(ROS)is significant.To date,however,there has rarely been any focus on the directed generation of ROSs.Herein,we report the first identification of tunable molecular oxygen activation induced by polymeric conjugation in nonmetallic conjugated microporous polymers(CMP).The conjugation between these can be achieved by the introduction of alkynyl groups.CMP-A with an alkynyl bridge facilitates the intramolecular charge mobility while CMP-D,lacking an alkynyl group enhances the photoexcited carrier build-up on the surface from diffusion.These different processes dominate the directed ROS generation of the superoxide radical(·O_(2)^(-))and singlet oxygen(^(1)O_(2)),respectively.This theory is substantiated by the different performances of these CMPs in the aerobic oxidation of sulfides and the dehydrogenative coupling of amines,and could provide insight into the rational design of CMPs for various heterogeneous organic photosynthesis.展开更多
Solid-state nanopores are generally considered as an indispensable element in the research field of fundamental ion transport and molecular sensing. The im- provement in fabrication and chemical modification of the so...Solid-state nanopores are generally considered as an indispensable element in the research field of fundamental ion transport and molecular sensing. The im- provement in fabrication and chemical modification of the solid-state nanopores remains increasingly updated. During the last decades, numerous works have been reported on the nanopore-based sensing applications. More and more new analytical methods using nanopore-based devices are emerging. In this review, we highlight the recent progress on the analytical methods for the interdisciplinary and fast- growing area of nanopore research. According to the dif- ferent types of the electrical readout, whether it is steady- state ionic current or transient current fluctuation, the nanopore-based sensing and analysis can be generally di- vided into two categories. For the first type, the electrical readout shows a stable blockade or reopening of the nanopore conductance in the presence of target analytes, termed steady-state analysis, including the conductance change, electrochemical analysis, and two-dimensional scanning and imaging. The other type is based on the transient fluctuation in the transmembrane ionic current, termed transient-state analysis, including the noise analysis, transient ion transport, and transverse tunneling current. The investigation of solid-state nanopores for chemical sensing is just in its infancy. For further research work, not only new nanopore materials and chemical modifications are needed, but also other non-electric-based sensing techniques should be developed. We will focus our future research in the framework of bio-inspired, smart, multiscale interfacial materials and extend the spirit of binary cooperative complementary nanomaterials.展开更多
We introduce a non-uniform gravity-like force field to control the granular flow state in a quasi-one- dimensional system, and study the system by the molecular dynamics simulation. We find that the granular flow unde...We introduce a non-uniform gravity-like force field to control the granular flow state in a quasi-one- dimensional system, and study the system by the molecular dynamics simulation. We find that the granular flow under non-uniform force field can be well described by a density wave with fixed time period if a fixed partiele number condition is used. The base frequency of the density wave does not depend on the position of the flow, while both the average density and oseillation amplitude of the flow vary continuously with the position. The formation of the density wave results from the aggregation of the granules in the decelerated region and the feed-back mechanism in the fixed particle number condition.展开更多
基金Project(50575202) supported by the National Natural Science Foundation of China
文摘The structure and working principle of a self-deigned high pressure electronic pneumatic pressure reducing valve (EPPRV) with slide pilot are introduced.The resistance value formulas and the relationship between the resistance and pressure of three typical pneumatic resistances are obtained.Then,the method of static characteristics analysis only considering pneumatic resistances is proposed,the resistance network from gas supply to load is built up,and the mathematical model is derived from the flow rate formulas and flow conservation equations,with the compressibility of high pressure gas and temperature drop during the expansion considered in the model.Finally,the pilot spool displacement of 1.5 mm at an output pressure of 15MPa and the enlarging operating stroke of the pilot spool are taken as optimization targets,and the optimization is carried out based on genetic algorithm and the model mentioned above.The results show that the static characteristics of the EPPRV are significantly improved.The idea of static characteristics analysis and optimization based on pneumatic resistance network is valuable for the design of pneumatic components or system.
基金The project supported by the Natural Science Foundation of the Education Department of Anhui Province of China under Grant Nos. 2006KJ070A, 2006KJ057B, and the Talent Foundation of Anhui University.
文摘We propose a probabilistic scheme for realizing teleportation of bipartite photonic states using linear optical elements where only requires a two-photon Bell state used as quantum channel. It reduces the requirement of the entanglement of quantum channel, but requires an additional photon and an auxiliary maximally entangled photon pair locally.
文摘In 3-mode Fock space we find a new tripartite entangled state |α,γ 】 λ,which make up a new quantum mechanical representation. The state |α,γ 】 λ, can be generated byusing the setup composing of a beam splitter and a parametric down-conversion amplifier. Applicationof the state is briefly discussed.
基金supported by the National Natural Science Foundation of China(51902121,52073110,22071072,51872107,21975090,and 21801086)the Fundamental Research Funds for the Central Universities of China(2662018QD011,2662018PY052,and 2662019PY023)the Natural Science Foundation of Hubei Province(2019CFB322)。
文摘Photocatalytic oxidative organic reactions are important synthetic transformations,and research on reaction selectivity by reactive oxygen species(ROS)is significant.To date,however,there has rarely been any focus on the directed generation of ROSs.Herein,we report the first identification of tunable molecular oxygen activation induced by polymeric conjugation in nonmetallic conjugated microporous polymers(CMP).The conjugation between these can be achieved by the introduction of alkynyl groups.CMP-A with an alkynyl bridge facilitates the intramolecular charge mobility while CMP-D,lacking an alkynyl group enhances the photoexcited carrier build-up on the surface from diffusion.These different processes dominate the directed ROS generation of the superoxide radical(·O_(2)^(-))and singlet oxygen(^(1)O_(2)),respectively.This theory is substantiated by the different performances of these CMPs in the aerobic oxidation of sulfides and the dehydrogenative coupling of amines,and could provide insight into the rational design of CMPs for various heterogeneous organic photosynthesis.
基金supported by the National Basic Research Program of China (2011CB935700)the National Natural Science Foundation of China (21103201, 11290163, 91127025, 21121001)The Chinese Academy of Sciences is gratefully acknowledged under the Key Research Program of the Chinese Academy of Sciences (KJZD-EW-M01)
文摘Solid-state nanopores are generally considered as an indispensable element in the research field of fundamental ion transport and molecular sensing. The im- provement in fabrication and chemical modification of the solid-state nanopores remains increasingly updated. During the last decades, numerous works have been reported on the nanopore-based sensing applications. More and more new analytical methods using nanopore-based devices are emerging. In this review, we highlight the recent progress on the analytical methods for the interdisciplinary and fast- growing area of nanopore research. According to the dif- ferent types of the electrical readout, whether it is steady- state ionic current or transient current fluctuation, the nanopore-based sensing and analysis can be generally di- vided into two categories. For the first type, the electrical readout shows a stable blockade or reopening of the nanopore conductance in the presence of target analytes, termed steady-state analysis, including the conductance change, electrochemical analysis, and two-dimensional scanning and imaging. The other type is based on the transient fluctuation in the transmembrane ionic current, termed transient-state analysis, including the noise analysis, transient ion transport, and transverse tunneling current. The investigation of solid-state nanopores for chemical sensing is just in its infancy. For further research work, not only new nanopore materials and chemical modifications are needed, but also other non-electric-based sensing techniques should be developed. We will focus our future research in the framework of bio-inspired, smart, multiscale interfacial materials and extend the spirit of binary cooperative complementary nanomaterials.
基金Supported by the National Basic Research Program of China under Grant No.2009CB930800by the National Natural Science Foundation of China under Grant Nos.10875166 and 11274355
文摘We introduce a non-uniform gravity-like force field to control the granular flow state in a quasi-one- dimensional system, and study the system by the molecular dynamics simulation. We find that the granular flow under non-uniform force field can be well described by a density wave with fixed time period if a fixed partiele number condition is used. The base frequency of the density wave does not depend on the position of the flow, while both the average density and oseillation amplitude of the flow vary continuously with the position. The formation of the density wave results from the aggregation of the granules in the decelerated region and the feed-back mechanism in the fixed particle number condition.
