The contributions of persistent organic pollutants (POPs) from the subtropical regions of China to pollution of the global environment have been paid great attention; however, little is known about the state of POPs...The contributions of persistent organic pollutants (POPs) from the subtropical regions of China to pollution of the global environment have been paid great attention; however, little is known about the state of POPs in agricultural ecosystems within these regions of China. This study primarily revealed the state of the contamination and distribution of polycyclic aromatic hydrocarbons (PAH) in agricultural soils in the subtropical regions. 115 surface soils (0-20 cm) were sampled in the breadbaskets of these regions. The concentrations and types of PAH were determined using gas chromatography linked to mass spectrometry (GC-MS). The total PAH concentrations ranged from 22.1 to 1 256.9 ng g^-1 with a mean of 318.2 ± 148.2 ng g^-1. In general terms, the current PAH concentrations were lower than most PAH levels reported in a number of investigations from different countries and regions. PAH isomer ratios indicated that pyrolytic origins, such as fossil fuel combustion related to vehicle tail gas and industrial emissions, were the dominant sources of PAH in the southern subtropical areas of China. Although PAH concentrations decreased with decreasing pollution, population, and traffic density, to a great extent PAH compositions were similar throughout subtropical soils, with naphthalene, phenanthrene, fluoranthene, and benzo(b)fluoranthene being dominant.展开更多
Fossil reproductive structure from the Eocene of the Changchang Basin (Hainan Island,South China) is recognized as Chaneya hainanensis sp.nov.This new species is characterized by persistent corolla of five obovate pet...Fossil reproductive structure from the Eocene of the Changchang Basin (Hainan Island,South China) is recognized as Chaneya hainanensis sp.nov.This new species is characterized by persistent corolla of five obovate petals with three subparallel primary venation linked by arching secondary veins,circular central disk bearing two orbicular ovaries or fruit bodies.This discovery confirms the presence of the extinct fruit genus Chaneya in low-latitude tropical area,providing significant fossil evidence for investigating the origin,migration,and phytogeography of this genus and discussing the Tertiary floristic exchanges among North America,eastern Asia,and Europe.Considering the distribution of this genus and its extant relatives and the climate changes during the Cenozoic,we hypothesize that Chaneya was a widespread tropical or subtropical taxon,but,with climate cooling,became extinct in northern latitudes and evolved into Picrasma (Simaroubaceae) and Rutaceae mainly in modern tropics and subtropics.展开更多
基金Project supported by the State Environmental Protection Administration of China (No.2001-1-2)State Environmental Protection Administration of Guangdong (No.2001-08)Guangdong Key Laboratory of Agricultural Environment Pollution Integrated Control,and the National Natural Science Foundation of China(Nos.30170147 and 30270282)
文摘The contributions of persistent organic pollutants (POPs) from the subtropical regions of China to pollution of the global environment have been paid great attention; however, little is known about the state of POPs in agricultural ecosystems within these regions of China. This study primarily revealed the state of the contamination and distribution of polycyclic aromatic hydrocarbons (PAH) in agricultural soils in the subtropical regions. 115 surface soils (0-20 cm) were sampled in the breadbaskets of these regions. The concentrations and types of PAH were determined using gas chromatography linked to mass spectrometry (GC-MS). The total PAH concentrations ranged from 22.1 to 1 256.9 ng g^-1 with a mean of 318.2 ± 148.2 ng g^-1. In general terms, the current PAH concentrations were lower than most PAH levels reported in a number of investigations from different countries and regions. PAH isomer ratios indicated that pyrolytic origins, such as fossil fuel combustion related to vehicle tail gas and industrial emissions, were the dominant sources of PAH in the southern subtropical areas of China. Although PAH concentrations decreased with decreasing pollution, population, and traffic density, to a great extent PAH compositions were similar throughout subtropical soils, with naphthalene, phenanthrene, fluoranthene, and benzo(b)fluoranthene being dominant.
基金supported by National Natural Science Foundation of China (Grant Nos. 40972011,31070200)National Basic Research Program of China (973 Program) (Grant No. 2012CB822003)+2 种基金the joint Project of National Natural Science Foundation of China and Russian Foundation for Basic Research (Grant Nos. 41111120083,11-04-91175)Guangdong Natural Science Foundation (Grant No. 10151027501000020)Key Project of the Sun Yat-sen University for inviting foreign teachers and Scientific Research Fund, Hongda Zhang, Sun Yat-sen University
文摘Fossil reproductive structure from the Eocene of the Changchang Basin (Hainan Island,South China) is recognized as Chaneya hainanensis sp.nov.This new species is characterized by persistent corolla of five obovate petals with three subparallel primary venation linked by arching secondary veins,circular central disk bearing two orbicular ovaries or fruit bodies.This discovery confirms the presence of the extinct fruit genus Chaneya in low-latitude tropical area,providing significant fossil evidence for investigating the origin,migration,and phytogeography of this genus and discussing the Tertiary floristic exchanges among North America,eastern Asia,and Europe.Considering the distribution of this genus and its extant relatives and the climate changes during the Cenozoic,we hypothesize that Chaneya was a widespread tropical or subtropical taxon,but,with climate cooling,became extinct in northern latitudes and evolved into Picrasma (Simaroubaceae) and Rutaceae mainly in modern tropics and subtropics.