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城市湖泊影响城市低空大气污染物时空分布的机制
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作者 黄奥 刘振鑫 +2 位作者 陈诗雨 胡建林 陈梓轩 《大气科学学报》 CSCD 北大核心 2024年第6期928-948,共21页
湖泊在调节局地气候和空气质量方面发挥着重要的作用,城市湖泊对城市局地大气边界层环流和大气污染物输送机制的影响是目前城市空气质量研究的重要问题。本文分析了夏季南京城区濒湖站近地面大气污染物质量浓度的日变化特征,并与相对远... 湖泊在调节局地气候和空气质量方面发挥着重要的作用,城市湖泊对城市局地大气边界层环流和大气污染物输送机制的影响是目前城市空气质量研究的重要问题。本文分析了夏季南京城区濒湖站近地面大气污染物质量浓度的日变化特征,并与相对远离湖泊的非濒湖站的观测结果进行比较。结果表明:对于以近地面排放为主的NO_(2),日间濒湖站平均质量浓度比非濒湖站高(1.64±0.29)μg·m^(-3),夜间则低(0.51±1.39)μg·m^(-3);以边界层中高层生成与传输为主的O_(3),呈现出与NO_(2)相反的趋势,日间濒湖站平均质量浓度比非濒湖站低(9.57±2.19)μg·m^(-3),夜间则高(1.24±4.68)μg·m^(-3);PM_(2.5)质量浓度的差值没出现类似特征。利用二维陆面过程模式,并结合不同排放情景,对湖泊-城市陆地分布进行敏感性数值试验。试验结果表明,城市区域内湖面与陆面的热力性质差异影响了低空大气环流和垂直热力稳定度,并进一步影响城市近地面大气污染浓度的扩散传输过程。受湖泊存在的影响,白天位于湖泊及濒湖区域上方的垂直大气热力稳定度高于非濒湖区域上空,低层大气垂直扩散较弱,导致濒湖区域以近地面排放为主的污染物比质量浓度偏高,而以边界层中高层排放与生成为主的污染物比质量浓度则偏低;夜间情况则与之相反。该试验结果与观测数据的变化趋势吻合,且与WRF-Chem模拟结果类似。 展开更多
关键词 土地利用类型 陆面过程 垂直大气稳定度 城市空气质量
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Contrast patterns and trends of lapse rates calculated from near-surface air and land surface temperatures in China from 1961 to 2014 被引量:7
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作者 Yanyi He Kaicun Wang 《Science Bulletin》 SCIE EI CAS CSCD 2020年第14期1217-1224,M0004,共9页
The near-surface lapse rate reflects the atmospheric stability above the surface.Lapse rates calculated from land surface temperature(γTs)and near-surface air temperature( γTa )have been widely used.However,γTs and... The near-surface lapse rate reflects the atmospheric stability above the surface.Lapse rates calculated from land surface temperature(γTs)and near-surface air temperature( γTa )have been widely used.However,γTs and γTa have different sensitivity to local surface energy balance and large-scale energy transport and therefore they may have diverse spatial and temporal variability,which has not been clearly illustrated in existing studies.In this study,we calculated and compared γTa and γTs at^2200 stations over China from 1961 to 2014.This study finds that γTa and γTs have a similar multiyear national average(0.53°C/100 m)and seasonal cycle.Nevertheless,γTs shows steeper multiyear average than γTa at high latitudes,and γTs in summer is steeper than γTa ,especially in Northwest China.The North China shows the shallowest γTa and γTs,then inhibiting the vertical diffusion of air pollutants and further reducing the lapse rates due to accumulation of pollutants.Moreover,the long-term trend signs for γTa and γTs are opposite in northern China.However,the trends in γTa and γTs are both negative in Southwest China and positive in Southeast China.Surface incident solar radiation,surface downward longwave radiation and precipitant frequency jointly can account for 80%and 75%of the long-term trends in γTa and γTs in China,respectively,which provides an explanation of trends of γTa and γTs from perspective of surface energy balance. 展开更多
关键词 Lapse rate Near-surface air temperature Land surface temperature Long-term trend Climatic factor
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