Direct N2O decomposition has been investigated over bare NiO and a series of its alkali-promoted catalysts. These catalysts were characterized by X-ray diffractometry, X-ray photoelectron spectroscopy （XPS） and fiel...Direct N2O decomposition has been investigated over bare NiO and a series of its alkali-promoted catalysts. These catalysts were characterized by X-ray diffractometry, X-ray photoelectron spectroscopy （XPS） and field emission scanning electron microscopy. XPS analysis revealed that surface nickel is present in three forms： metal particles, NiO and Ni（OH）2. It is suggested that nickel（0） valent atoms are essential for the interaction with N2O molecules at the catalyst surfaces. Bare NiO exhibited a very low N2O decomposition reactivity. However, the alkali-containing catalysts exhibited a marked activity enhancement.展开更多
Network modeling is an important approach in many fields in analyzing complex systems. Recently new series of methods have emerged, by using Kronecker product and similar tools to model real systems. One of such appro...Network modeling is an important approach in many fields in analyzing complex systems. Recently new series of methods have emerged, by using Kronecker product and similar tools to model real systems. One of such approaches is the multiplicative attribute graph(MAG) model, which generates networks based on category attributes of nodes. In this paper we try to extend this model into a continuous one, give an overview of its properties, and discuss some special cases related to real-world networks, as well as the influence of attribute distribution and affinity function respectively.展开更多
文摘Direct N2O decomposition has been investigated over bare NiO and a series of its alkali-promoted catalysts. These catalysts were characterized by X-ray diffractometry, X-ray photoelectron spectroscopy （XPS） and field emission scanning electron microscopy. XPS analysis revealed that surface nickel is present in three forms： metal particles, NiO and Ni（OH）2. It is suggested that nickel（0） valent atoms are essential for the interaction with N2O molecules at the catalyst surfaces. Bare NiO exhibited a very low N2O decomposition reactivity. However, the alkali-containing catalysts exhibited a marked activity enhancement.
基金the National Natural Science Foundation of China(No.61379074)the Zhejiang Provincial Natural Science Foundation of China(No.LZ12F02003)
文摘Network modeling is an important approach in many fields in analyzing complex systems. Recently new series of methods have emerged, by using Kronecker product and similar tools to model real systems. One of such approaches is the multiplicative attribute graph(MAG) model, which generates networks based on category attributes of nodes. In this paper we try to extend this model into a continuous one, give an overview of its properties, and discuss some special cases related to real-world networks, as well as the influence of attribute distribution and affinity function respectively.
