As one of the regions with intensive agriculture and rapid economic development in China,North China also has a high nitrogen(N)deposition.This study characterized the spatial pattern of N deposition in North China,co...As one of the regions with intensive agriculture and rapid economic development in China,North China also has a high nitrogen(N)deposition.This study characterized the spatial pattern of N deposition in North China,combining the tropospheric columns from satellite measurements and the simulated profiles from an atmospheric chemistry transport model.The total N deposition fluxes ranged from 16.3 to 106.5 kg N ha−1 yr−1,with an average of 54.5±17.2 kg N ha−1 yr−1.The high values were concentrated in urban and farmland areas,while low values were found in forests and grasslands with less human activities.Of the total N deposition,36%was deposited via precipitation,12%was deposited through dry particulate deposition,and the remaining 52%was comprised of dry gaseous deposition.For the seasonal variation of dry deposition,gaseous HNO3 and particulate NO3−were higher in winter and autumn,but lower in spring and summer.In contrast,gaseous NH3 and particulate NH4+were higher in spring and summer,but lower in winter and autumn.This is possibly caused by the seasonal differences in emission intensity between NOx and NH3 emission sources.The gaseous NO2 deposition did not show strong seasonal variation.The wet deposition was mainly affected by precipitation,with high values in summer and low values in winter.This research provides an objective spatial perspective and insight into the total N deposition in North China.展开更多
In this study, a special method is proposed for detecting aerosols over land by analyzing satellitemeasured far IR radiation at three channels, 8.7, 11.5, and 12.5 lain. Sensitivity tests revealed that the behavioral ...In this study, a special method is proposed for detecting aerosols over land by analyzing satellitemeasured far IR radiation at three channels, 8.7, 11.5, and 12.5 lain. Sensitivity tests revealed that the behavioral features of radiative brightness temperatures （BTs） at these three channels with increasing optical depth are different among different types of aerosols. Analyzing how BTs and their differences, xBT （BT11.5-BT12.5） and YBT （BT8.7-BT11.5）, behave with varying optical depth can help to qualitatively distinguish among aerosols and semi-quantitatively estimate their optical thicknesses. In addition, the authors found that the vertical density profile of aerosols has little impact on this method.展开更多
基金This study was supported by the National Natural Science Foundation of China[grant numbers 41471343 and 41601457].
文摘As one of the regions with intensive agriculture and rapid economic development in China,North China also has a high nitrogen(N)deposition.This study characterized the spatial pattern of N deposition in North China,combining the tropospheric columns from satellite measurements and the simulated profiles from an atmospheric chemistry transport model.The total N deposition fluxes ranged from 16.3 to 106.5 kg N ha−1 yr−1,with an average of 54.5±17.2 kg N ha−1 yr−1.The high values were concentrated in urban and farmland areas,while low values were found in forests and grasslands with less human activities.Of the total N deposition,36%was deposited via precipitation,12%was deposited through dry particulate deposition,and the remaining 52%was comprised of dry gaseous deposition.For the seasonal variation of dry deposition,gaseous HNO3 and particulate NO3−were higher in winter and autumn,but lower in spring and summer.In contrast,gaseous NH3 and particulate NH4+were higher in spring and summer,but lower in winter and autumn.This is possibly caused by the seasonal differences in emission intensity between NOx and NH3 emission sources.The gaseous NO2 deposition did not show strong seasonal variation.The wet deposition was mainly affected by precipitation,with high values in summer and low values in winter.This research provides an objective spatial perspective and insight into the total N deposition in North China.
基金supported by the National Basic Research Program of China (Grant No. 2006CB403705)
文摘In this study, a special method is proposed for detecting aerosols over land by analyzing satellitemeasured far IR radiation at three channels, 8.7, 11.5, and 12.5 lain. Sensitivity tests revealed that the behavioral features of radiative brightness temperatures （BTs） at these three channels with increasing optical depth are different among different types of aerosols. Analyzing how BTs and their differences, xBT （BT11.5-BT12.5） and YBT （BT8.7-BT11.5）, behave with varying optical depth can help to qualitatively distinguish among aerosols and semi-quantitatively estimate their optical thicknesses. In addition, the authors found that the vertical density profile of aerosols has little impact on this method.
