Formamidinium lead bromide(FAPbBr_(3))nanocrystals(NCs)have been considered to be a good optoelectronic material due to their pure green emission,excellent stability and superior carrier transport characteristics.Howe...Formamidinium lead bromide(FAPbBr_(3))nanocrystals(NCs)have been considered to be a good optoelectronic material due to their pure green emission,excellent stability and superior carrier transport characteristics.However,two-photon pumped amplified spontaneous emission(ASE)and the corresponding nonlinear optical properties of FAPbBr_(3) NCs are scarcely revealed.Herein,we synthesized colloidal FAPbBr_(3) NCs with different sizes by changing the molar ratio of FABr/PbBr_(2) in the precursor solution,using ligand assisted precipitation(LARP)technology at room temperature.Photoluminescence(PL)and time resolved photoluminescence(TRPL)spectroscopy were measured to characterize their ASE properties.And their nonlinear optical properties were studied through the Zscan technique and the two-photon excited fluorescence method.The stimulated emission properties including oneand two-photon pumped ASE have been realized from FAPbBr_(3) NCs.With large two-photon absorption coefficient(0.27 cm/GW)and high non-linear absorption cross-section(7.52×10^(5) GM),ASE with threshold as low as 9.8μJ/cm^(2) and 487μJ/cm^(2) have been obtained from colloidal FAPbBr_(3) NCs using one-and two-photon excitations.These results indicate that as a new possible green-emitting frequency-upconversion material with low thresholds,FAPbBr_(3) NCs hold great potential in the development of high-performance two-photon pump lasers.展开更多
[ Objective] The aim was to provide strategies for development of rare earth and control of environmental pollution. [ Method] Responses of membrane lipid peroxidation and endogenous hormones of soybean seedlings to U...[ Objective] The aim was to provide strategies for development of rare earth and control of environmental pollution. [ Method] Responses of membrane lipid peroxidation and endogenous hormones of soybean seedlings to UV-B radiation and rare earth were studied through hydroponics in laboratory. [ Result] The results showed that under irradiation of UV-B（ T1-0.15 W/m^2 and T2-0.45 W/m^2）, chlorophyll and indole-3-acetic acid（IAA） contents firstly decreased during the stress phase （1 -5 d） and then increased during the restoration phase （6 -9 d） while contents of malonadialdehyde（MDA） and abscisic acid（ABA） gradually increased during the imposition of UV-B radiation （1 -5 d） and subsequently decreased during recovery from UV-B stress （6 -9 d） . With adding of La （III） with the concentration of 20 mg · L^-1 , the decline/dse trend of chlorophyll, IAA, MDA and ABA contents was slowed down during the stress period while the rise/decline speed was accelerated during the recovery period. [ Conclusion] It suggests that the regulation of La （ III ） on membrane lipid peroxidation and endogenous hormones could increase chlorophyll and IAA contents, improve the metabolism of reactive oxygen species （ ROS）, inhibit membrane lipid peroxidation, decrease the accumulation amount of ABA and alleviate injury of UV-B radiation to soybean seedlings. Further, the protective potential of La （ III ） was better under low UV-B radiation than under high one.展开更多
The thermal infrared channel (IRS4) of HJ-1B satellite obtains view zenith angles (VZA) up to ±33°. The view angle should be taken into account when retrieving land surface temperature (LST) from IRS4 data. ...The thermal infrared channel (IRS4) of HJ-1B satellite obtains view zenith angles (VZA) up to ±33°. The view angle should be taken into account when retrieving land surface temperature (LST) from IRS4 data. This study aims at improving the mono-window algorithm for retrieving LST from IRS4 data. Based on atmospheric radiative transfer simulations,a model for correcting the VZA effects on atmospheric transmittance is proposed. In addition,a generalized model for calculating the effective mean atmospheric temperature is developed. Validation with the simulated dataset based on standard atmospheric profiles reveals that the improved mono-window algorithm for IRS4 obtains high accuracy for LST retrieval,with the mean absolute error (MAE) and root mean square error (RMSE) being 1.0 K and 1.1 K,respectively. Numerical experiment with the radiosonde profile acquired in Beijing in winter demonstrates that the improved mono-window algorithm exhibits excellent ability for LST retrieval,with MAE and RMSE being 0.6 K and 0.6 K,respectively. Further application in Qinghai Lake and comparison with the Moderate-Resolution Imaging Spectroradiometer (MODIS) LST product suggest that the improved mono-window algorithm is applicable and feasible in actual conditions.展开更多
Mt. Qomolangma （Everest）, the highest mountain peak in the world, has little been studied extensively from a meteorological perspective, mostly because of the remoteness of the region and the resultant lack of meteo...Mt. Qomolangma （Everest）, the highest mountain peak in the world, has little been studied extensively from a meteorological perspective, mostly because of the remoteness of the region and the resultant lack of meteorological data. An automatic weather station （AWS）, the highest in the world, was set up on 27 April 2005 at the Ruopula Pass （6523 m asl） on the northern slope of Mt. Qomolangma by the team of integrated scientific expedition to Mt. Qomolangma. Here its meteorological characteristics were analyzed according to the lo-minute-averaged and 24-hour records of air temperature, relative humidity, air pressure and wind from 1 May to 22 July 2005. It is shown that at 6523 m of Mt. Qomolangma, these meteorological elements display very obvious diurnal variations, and the character of averaged diurnal variation is one-peak-and-one-vale for air temperature, one-vale for relative humidity, two-peak-and-two-vale for air pressure, and one-peak with day-night asymmetry for wind speed. In the 83 days, all the air temperature, relative humidity and air pressure increased with some different fluctuations, while wind speed decreased gradually and wind direction turned from north to south. The variations of relative humidity had great fluctuations and obvious local differences. Then the paper discusses the reason for the characters of diurnal and daily variations. Compared with the corresponding records in May 1960, 5-day-averaged maximums, minimums and diurnal variations of air temperature in May 2005 were apparently lower.展开更多
文摘Formamidinium lead bromide(FAPbBr_(3))nanocrystals(NCs)have been considered to be a good optoelectronic material due to their pure green emission,excellent stability and superior carrier transport characteristics.However,two-photon pumped amplified spontaneous emission(ASE)and the corresponding nonlinear optical properties of FAPbBr_(3) NCs are scarcely revealed.Herein,we synthesized colloidal FAPbBr_(3) NCs with different sizes by changing the molar ratio of FABr/PbBr_(2) in the precursor solution,using ligand assisted precipitation(LARP)technology at room temperature.Photoluminescence(PL)and time resolved photoluminescence(TRPL)spectroscopy were measured to characterize their ASE properties.And their nonlinear optical properties were studied through the Zscan technique and the two-photon excited fluorescence method.The stimulated emission properties including oneand two-photon pumped ASE have been realized from FAPbBr_(3) NCs.With large two-photon absorption coefficient(0.27 cm/GW)and high non-linear absorption cross-section(7.52×10^(5) GM),ASE with threshold as low as 9.8μJ/cm^(2) and 487μJ/cm^(2) have been obtained from colloidal FAPbBr_(3) NCs using one-and two-photon excitations.These results indicate that as a new possible green-emitting frequency-upconversion material with low thresholds,FAPbBr_(3) NCs hold great potential in the development of high-performance two-photon pump lasers.
基金Supported by the Foundation of State Developing and ReformingCommittee(No.IFZ20051210)the National Natural Science Foundationof China(No.30570323,No.20471030)the Programsin Science and Technology of Nantong(No.DE2009006,No.S2009019)~~
文摘[ Objective] The aim was to provide strategies for development of rare earth and control of environmental pollution. [ Method] Responses of membrane lipid peroxidation and endogenous hormones of soybean seedlings to UV-B radiation and rare earth were studied through hydroponics in laboratory. [ Result] The results showed that under irradiation of UV-B（ T1-0.15 W/m^2 and T2-0.45 W/m^2）, chlorophyll and indole-3-acetic acid（IAA） contents firstly decreased during the stress phase （1 -5 d） and then increased during the restoration phase （6 -9 d） while contents of malonadialdehyde（MDA） and abscisic acid（ABA） gradually increased during the imposition of UV-B radiation （1 -5 d） and subsequently decreased during recovery from UV-B stress （6 -9 d） . With adding of La （III） with the concentration of 20 mg · L^-1 , the decline/dse trend of chlorophyll, IAA, MDA and ABA contents was slowed down during the stress period while the rise/decline speed was accelerated during the recovery period. [ Conclusion] It suggests that the regulation of La （ III ） on membrane lipid peroxidation and endogenous hormones could increase chlorophyll and IAA contents, improve the metabolism of reactive oxygen species （ ROS）, inhibit membrane lipid peroxidation, decrease the accumulation amount of ABA and alleviate injury of UV-B radiation to soybean seedlings. Further, the protective potential of La （ III ） was better under low UV-B radiation than under high one.
基金Under the auspices of Opening Funding of State Key Laboratory for Remote Sensing ScienceNational High-tech Research and Development Program (863 Program) (No. 2007AA120205, 2007AA120306)
文摘The thermal infrared channel (IRS4) of HJ-1B satellite obtains view zenith angles (VZA) up to ±33°. The view angle should be taken into account when retrieving land surface temperature (LST) from IRS4 data. This study aims at improving the mono-window algorithm for retrieving LST from IRS4 data. Based on atmospheric radiative transfer simulations,a model for correcting the VZA effects on atmospheric transmittance is proposed. In addition,a generalized model for calculating the effective mean atmospheric temperature is developed. Validation with the simulated dataset based on standard atmospheric profiles reveals that the improved mono-window algorithm for IRS4 obtains high accuracy for LST retrieval,with the mean absolute error (MAE) and root mean square error (RMSE) being 1.0 K and 1.1 K,respectively. Numerical experiment with the radiosonde profile acquired in Beijing in winter demonstrates that the improved mono-window algorithm exhibits excellent ability for LST retrieval,with MAE and RMSE being 0.6 K and 0.6 K,respectively. Further application in Qinghai Lake and comparison with the Moderate-Resolution Imaging Spectroradiometer (MODIS) LST product suggest that the improved mono-window algorithm is applicable and feasible in actual conditions.
基金partially funded by the National Nature Science Foundation of China(Grant No.40501015)the Chinese Academy of Science(Grant No.KZCX3-SW-354 and KZCX3-SW-344).
文摘Mt. Qomolangma （Everest）, the highest mountain peak in the world, has little been studied extensively from a meteorological perspective, mostly because of the remoteness of the region and the resultant lack of meteorological data. An automatic weather station （AWS）, the highest in the world, was set up on 27 April 2005 at the Ruopula Pass （6523 m asl） on the northern slope of Mt. Qomolangma by the team of integrated scientific expedition to Mt. Qomolangma. Here its meteorological characteristics were analyzed according to the lo-minute-averaged and 24-hour records of air temperature, relative humidity, air pressure and wind from 1 May to 22 July 2005. It is shown that at 6523 m of Mt. Qomolangma, these meteorological elements display very obvious diurnal variations, and the character of averaged diurnal variation is one-peak-and-one-vale for air temperature, one-vale for relative humidity, two-peak-and-two-vale for air pressure, and one-peak with day-night asymmetry for wind speed. In the 83 days, all the air temperature, relative humidity and air pressure increased with some different fluctuations, while wind speed decreased gradually and wind direction turned from north to south. The variations of relative humidity had great fluctuations and obvious local differences. Then the paper discusses the reason for the characters of diurnal and daily variations. Compared with the corresponding records in May 1960, 5-day-averaged maximums, minimums and diurnal variations of air temperature in May 2005 were apparently lower.
