^99Sr concentrations, resulting from the Chernobyl NPP accident, were determined in the salt lakes of the Crimea （Lakes Kiyatskoe, Kirleutskoe, Kizil-Yar, Bakalskoe and Donuzlav）, together with the redistribution be...^99Sr concentrations, resulting from the Chernobyl NPP accident, were determined in the salt lakes of the Crimea （Lakes Kiyatskoe, Kirleutskoe, Kizil-Yar, Bakalskoe and Donuzlav）, together with the redistribution between the components of the ecosystems. The content of mercury in the waters of the studied reservoirs was also established. Vertical distributions of natural radionuclide activities （^238U, ^232Th, ^226Ra, ^210pb, ^40K） and anthropogenic ^137Cs concentrations （as radiotracers） were determined in the bottom sediments of the Koyashskoe salt lake （located in the south-eastern Crimea） to evaluate the long- term dynamics and biogeochemical processes. Radiochemical and chemical analysis was undertaken and radiotracer and statistical methods were applied to the analytical data. The highest concentrations of ^99Sr in the water of Lake Kiyatskoe （350.5 and 98.0 Bq/m^3） and Lake Kirleutskoe （121.3 Bq/m^3） were due to the discharge of the Dnieper water from the North-Crimean Canal. The high content of mercury in Lake Kiyatskoe （363.2 ng/L） and in seawater near Lake Kizil-Yar （364 ng/L） exceeded the maximum permissible concentration （3.5 times the maximum）. Natural radionuclides provide the main contribution to the total radioactivity （artificial and natural combined） in the bottom sediments of Lake Koyashskoe. The significant concentration of ^210pb in the upper layer of bottom sediments of the lake indicates an active inflow of its parent radionuclide-gaseous ^222Rn from the lower layers of the bottom sediment. The average sedimentation rates in Lake Koyashskoe, determined using ^210pb and ^137Cs data, were 0.117 and 0.109 cm per year, respectively.展开更多
Here I collected natural gas samples from 41 industrial gas wells in the Tarim Basin,and studied the mercury distribution in the area.My data show that there is certain regularity in the distribution of mercury in the...Here I collected natural gas samples from 41 industrial gas wells in the Tarim Basin,and studied the mercury distribution in the area.My data show that there is certain regularity in the distribution of mercury in the Tarim Basin.Generally,the mercury concentration is high at the edge of the basin and low in the central basin.The highest mercury concentration occurs in the Southwest Depression,ranging from 15428.5 to 296763.0ng/m3 with an average of 156095.7ng/m3,followed by the Kuqa Depression ranging from 15.0 to 56964.3ng/m3 with an average of 11793.7ng/m3,and the Hade oil and gas field in the North Depression has the lowest mercury concentration ranging from 17.7 to 3339.5ng/m3 with an average of 1678.6ng/m3.The mercury concentrations in the natural gases of different structural units are various,with the highest mercury concentration in the zone of strong structural activity of Southwest Depression.It is profitable of Hg accumulation in the self sourced and self accumulated gas reservoirs or volcanic existence;in contrast,the low Hg concentration exists in the secondary gas reservoir.The mercury concentration in the natural gas generated under continental depositional environment is higher than that in marine gas.Therefore,the mercury concentration in the natural gases is constrained by gas genesis,depositional environment of source rocks,tectonic activity,and volcanic activity,and the tectonic activity is the main factor for the mercury concentration in the natural gas,followed by volcanic activity and depositional environments.展开更多
文摘^99Sr concentrations, resulting from the Chernobyl NPP accident, were determined in the salt lakes of the Crimea （Lakes Kiyatskoe, Kirleutskoe, Kizil-Yar, Bakalskoe and Donuzlav）, together with the redistribution between the components of the ecosystems. The content of mercury in the waters of the studied reservoirs was also established. Vertical distributions of natural radionuclide activities （^238U, ^232Th, ^226Ra, ^210pb, ^40K） and anthropogenic ^137Cs concentrations （as radiotracers） were determined in the bottom sediments of the Koyashskoe salt lake （located in the south-eastern Crimea） to evaluate the long- term dynamics and biogeochemical processes. Radiochemical and chemical analysis was undertaken and radiotracer and statistical methods were applied to the analytical data. The highest concentrations of ^99Sr in the water of Lake Kiyatskoe （350.5 and 98.0 Bq/m^3） and Lake Kirleutskoe （121.3 Bq/m^3） were due to the discharge of the Dnieper water from the North-Crimean Canal. The high content of mercury in Lake Kiyatskoe （363.2 ng/L） and in seawater near Lake Kizil-Yar （364 ng/L） exceeded the maximum permissible concentration （3.5 times the maximum）. Natural radionuclides provide the main contribution to the total radioactivity （artificial and natural combined） in the bottom sediments of Lake Koyashskoe. The significant concentration of ^210pb in the upper layer of bottom sediments of the lake indicates an active inflow of its parent radionuclide-gaseous ^222Rn from the lower layers of the bottom sediment. The average sedimentation rates in Lake Koyashskoe, determined using ^210pb and ^137Cs data, were 0.117 and 0.109 cm per year, respectively.
基金supported by the National Natural Science Foundation of China (Grant Nos. 40802028 & 41173035)the China National Key Fundamental Research and Development Project (Grant Nos. 2012CB214800 & 2005CB422108)the National Science & Technology Special Project (Grant No. 2011ZX05005)
文摘Here I collected natural gas samples from 41 industrial gas wells in the Tarim Basin,and studied the mercury distribution in the area.My data show that there is certain regularity in the distribution of mercury in the Tarim Basin.Generally,the mercury concentration is high at the edge of the basin and low in the central basin.The highest mercury concentration occurs in the Southwest Depression,ranging from 15428.5 to 296763.0ng/m3 with an average of 156095.7ng/m3,followed by the Kuqa Depression ranging from 15.0 to 56964.3ng/m3 with an average of 11793.7ng/m3,and the Hade oil and gas field in the North Depression has the lowest mercury concentration ranging from 17.7 to 3339.5ng/m3 with an average of 1678.6ng/m3.The mercury concentrations in the natural gases of different structural units are various,with the highest mercury concentration in the zone of strong structural activity of Southwest Depression.It is profitable of Hg accumulation in the self sourced and self accumulated gas reservoirs or volcanic existence;in contrast,the low Hg concentration exists in the secondary gas reservoir.The mercury concentration in the natural gas generated under continental depositional environment is higher than that in marine gas.Therefore,the mercury concentration in the natural gases is constrained by gas genesis,depositional environment of source rocks,tectonic activity,and volcanic activity,and the tectonic activity is the main factor for the mercury concentration in the natural gas,followed by volcanic activity and depositional environments.
