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青藏高原林线森林汞的空间分布格局及对大气环境汞污染的指示 被引量:7
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作者 吴飞 王训 +1 位作者 罗辑 李秋华 《环境化学》 CAS CSCD 北大核心 2019年第7期1619-1627,共9页
汞是引人关注的全球性污染物,偏远地区汞的源汇关系是当前研究的重点.由于其特殊的地理环境与大面积在线监测的不便,青藏高原大气汞的污染特征尚不明确.本研究根据青藏高原季风的传播路径,设置了云南-西藏与四川-西藏两条采样带,通过测... 汞是引人关注的全球性污染物,偏远地区汞的源汇关系是当前研究的重点.由于其特殊的地理环境与大面积在线监测的不便,青藏高原大气汞的污染特征尚不明确.本研究根据青藏高原季风的传播路径,设置了云南-西藏与四川-西藏两条采样带,通过测定样带上林线森林各个组分的汞含量,来反演大气汞的污染状况.研究结果表明,青藏高原林线区域的冷杉凋落物、树叶树皮与表层土壤的汞含量均表现为越靠近青藏高原腹地,汞浓度越低.特别冷杉凋落物在云南与西藏、四川与西藏的交界区域汞浓度为60—70 ng·g-1,而昌都地区汞浓度仅为20—30 ng·g-1.此外还发现,凋落物与表层土壤的总汞含量在空间分布上与经度正相关,与纬度负相关.通过综合分析排放清单与大气环流资料,其原因可总结为:越靠近青藏高原腹地,局地源的汞排放与大气环流输送的汞均显著减少,使得大气环境汞含量降低,进而导致植被与土壤汞含量相应下降.本研究表明了凋落物中的总汞含量可作为大气环境汞污染的指示指标,证实了南亚、东南亚及我国的四川盆地与云贵高原是青藏高原大气汞污染的潜在排放源. 展开更多
关键词 青藏高原 大气汞污染 季风传输 凋落物汞 土壤汞
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Factors Limiting the Forecast Skill of the Boreal Summer Intraseasonal Oscillation in a Subseasonal-to-Seasonal Model 被引量:1
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作者 Zheng HE Pangchi HSU +2 位作者 Xiangwen LIU Tongwen WU Yingxia GAO 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2019年第1期104-118,共15页
In this study,we evaluate the forecast skill of the subseasonal-to-seasonal(S2S)prediction model of the Beijing Climate Center(BCC)for the boreal summer intraseasonal oscillation(BSISO).We also discuss the key factors... In this study,we evaluate the forecast skill of the subseasonal-to-seasonal(S2S)prediction model of the Beijing Climate Center(BCC)for the boreal summer intraseasonal oscillation(BSISO).We also discuss the key factors that inhibit the BSISO forecast skill in this model.Based on the bivariate anomaly correlation coefficient(ACC)of the BSISO index,defined by the first two EOF modes of outgoing longwave radiation and 850-hPa zonal wind anomalies over the Asian monsoon region,we found that the hindcast skill degraded as the lead time increased.The ACC dropped to below 0.5for lead times of 11 days and longer when the predicted BSISO showed weakened strength and insignificant northward propagation.To identify what causes the weakened forecast skill of BSISO at the forecast lead time of 11 days,we diagnosed the main mechanisms responsible for the BSISO northward propagation.The same analysis was also carried out using the observations and the outputs of the four-day forecast lead that successfully predicted the observed northward-propagating BSISO.We found that the lack of northward propagation at the 11-day forecast lead was due to insufficient increases in low-level cyclonic vorticity,moistening and warm temperature anomalies to the north of the convection,which were induced by the interaction between background mean flows and BSISO-related anomalous fields.The BCC S2S model can predict the background monsoon circulations,such as the low-level southerly and the northerly and easterly vertical shears,but has limited capability in forecasting the distributions of circulation and moisture anomalies. 展开更多
关键词 BCC S2S model boreal summer intraseasonal oscillation forecast skill northward propagation
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