Unveiling the pore-size performance of metal organic frameworks(MOFs)is imperative for controllable design of sophisticated catalysts.Herein,UiO-66 with distinct macropores and mesopores were intentionally created and...Unveiling the pore-size performance of metal organic frameworks(MOFs)is imperative for controllable design of sophisticated catalysts.Herein,UiO-66 with distinct macropores and mesopores were intentionally created and served as substrates to create advanced CdS/UiO-66 catalysts.The pore size impacted the spatial distribution of CdS nanoparticles(NPs):CdS tended to deposit on the external surface of mesoporous UiO-66,but spontaneously penetrated into the large cavity of macroporous UiO-66 nanocage.Normalized to unit amount of CdS,the photocatalytic reaction constant of macroporous CdS/UiO-66 over 4-nitroaniline reduction was~3 folds of that of mesoporous counterpart,and outperformed many other reported state-of-art CdS-based catalysts.A confinement effect of CdS NPs within UiO-66 cage could respond for its high activity,which could shorten the electron-transport distance of NPs-MOFs-reactant,and protect the active CdS NPs from photocorrosion.The finding here provides a straightforward paradigm and mechanism to rationally fabricate advance NPs/MOFs for diverse applications.展开更多
The paper begins with a brief review of the research history of earthquake size measurement. On this basis, the author pointed out the following points： ① In recent decades, ML, mb （mH ）, Ms magnitude scales are w...The paper begins with a brief review of the research history of earthquake size measurement. On this basis, the author pointed out the following points： ① In recent decades, ML, mb （mH ）, Ms magnitude scales are widely used as measures of earthquake size. However, these magnitude scales have a deficiency of ＂overgeneralization＂ and ＂magnitude saturation＂. Moreover, since they do not fully take into account the regional difference of seismic attenuation, especially the difference of site effects on the amplification of ground motion, these magnitude scales are but inaccurate measures of earthquake size. ② Seismic moment M0 not only has clear physical meaning, but also overcomes the deficiencies existing in ML, mb （mB ） and Ms magnitude scales, so it is the most suitable physical quantity for measuring earthquake size scientifically. In order to continue to use the term ＂magnitude＂, Kanamori defined the moment magnitude scale Act. Although its prerequisite assumptions remain to be studied, it is still a reasonable scale used as a measure of the relative size of an earthquake. ③ For measuring the earthquake size more scientifically, we must make full use of a large amount of waveform data from modern regional digital seismograph networks, strengthen the research on seismic wave attenuation characteristics, site effect, calculation of source parameters and the related scaling relations. In improving the measurement methods for ML, mb （mB ） and Ms magnitude, we should focus on the improvement of Mw scale and carry forward the work as gradually taking Mw magnitude scale as the uniform physical quantity to measure the relative size of earthquakes, so as to lay a more solid foundation for research in earthquake science and earthquake prediction.展开更多
Conventional correlation matching algorithms waste great time in invalid area search. This paper proposes a color tracking method based on correlation search area optimization on target characteristic hue decision. By...Conventional correlation matching algorithms waste great time in invalid area search. This paper proposes a color tracking method based on correlation search area optimization on target characteristic hue decision. By quantifying and reducing dimensions of HSV（ hue saturation value） color space, a one-dimensional hue space is constructed. In the space, the target characteristic hue granule set is constructed, which contains attributes such as value, area and average distance between pixels and aiming center. By using granular computing method, the similarity between target and search blocks is obtained and the invalid search areas can be removed. The color tracking experiment has proved that the algorithm can improve real time performance for conventional matching algorithms without precision lost.展开更多
The enumerating algorithm has been introduced into the fitting procedure of the ASR model. Based on the detailed study of 21 large earthquakes with M≥6. 8 in the Chinese Mainland,the statistical features of seismic s...The enumerating algorithm has been introduced into the fitting procedure of the ASR model. Based on the detailed study of 21 large earthquakes with M≥6. 8 in the Chinese Mainland,the statistical features of seismic strain release before large earthquakes have been summarized. In the mass,the strain release models can be divided into five types. The first is the DA model,in which the strain release accelerates in broader areas and decelerates in small areas around the epicenter. Approximately 38% of earthquake samples are of this type. The second is the AD model,in which the strain release decelerates in broader areas and accelerates in smaller areas around the epicenter with an occupying ratioof approximately 19%. The third is ASR,in which only accelerating strain release can be observed. Cases of this model amount to about 14%. The fourth is DSR,in which only decelerating strain release can be checked,amounting to about 24%. There is only one earthquake sample of the fifth type (LSR),which shows a linear strain release. There is a 3～6 years difference in the duration of pre-shock sequences between the accelerating and decelerating models. This means that seismic quiescence against a background of increased seismicity of small earthquakes before large earthquakes are a typical feature in general. For the DA model,the average size of critical regions for steady accelerating and decelerating strain release is about 260km to 400km and 100km to 200km,respectively,3 to 5 times and 1 to 2 times the rupture size of an earthquake of magnitude 7. 0. The AD model is the opposite of the DA model. The model parameter,m value,has good stability. The ratio of ASR is about the same for accelerating seismic strain release phenomena,no matter what the strain release models are,or how large the strain release quantity is. With regard to decelerating seismic strain release phenomena, the DA model has the most distinctive decelerating strain release characteristic and is the typical feature of seismic strain release,i. e. "decelerating in-accelerating out seismic strain model".展开更多
In this paper we study a negatively charged exciton （NCE）, which is trapped by a two-dimensional （2D） parabolic potential. By using matrix diagonalization techniques, the correlation energies of the low-lying stat...In this paper we study a negatively charged exciton （NCE）, which is trapped by a two-dimensional （2D） parabolic potential. By using matrix diagonalization techniques, the correlation energies of the low-lying states with L=0, 1, and 2 are calculated as a function of confinement strength. We find that the size effects of different states are different. This phenomenon can be explained as a hidden symmetry, which is originated purely from symmetry. Based on symmetry, the features of the low-lying states are discussed in the influence of the 2D parabolic potential well. It is found that the confinement may cause accidental degeneracies between levels with different low-excited states. It is shown that the effect of quantum confinement on the binding energy of the heavy hole is stronger than that of a light hole.展开更多
文摘Unveiling the pore-size performance of metal organic frameworks(MOFs)is imperative for controllable design of sophisticated catalysts.Herein,UiO-66 with distinct macropores and mesopores were intentionally created and served as substrates to create advanced CdS/UiO-66 catalysts.The pore size impacted the spatial distribution of CdS nanoparticles(NPs):CdS tended to deposit on the external surface of mesoporous UiO-66,but spontaneously penetrated into the large cavity of macroporous UiO-66 nanocage.Normalized to unit amount of CdS,the photocatalytic reaction constant of macroporous CdS/UiO-66 over 4-nitroaniline reduction was~3 folds of that of mesoporous counterpart,and outperformed many other reported state-of-art CdS-based catalysts.A confinement effect of CdS NPs within UiO-66 cage could respond for its high activity,which could shorten the electron-transport distance of NPs-MOFs-reactant,and protect the active CdS NPs from photocorrosion.The finding here provides a straightforward paradigm and mechanism to rationally fabricate advance NPs/MOFs for diverse applications.
基金funded by the Basic R&D Special Fund of Institute of Earthquake Science,CEA(2012IES0204)
文摘The paper begins with a brief review of the research history of earthquake size measurement. On this basis, the author pointed out the following points： ① In recent decades, ML, mb （mH ）, Ms magnitude scales are widely used as measures of earthquake size. However, these magnitude scales have a deficiency of ＂overgeneralization＂ and ＂magnitude saturation＂. Moreover, since they do not fully take into account the regional difference of seismic attenuation, especially the difference of site effects on the amplification of ground motion, these magnitude scales are but inaccurate measures of earthquake size. ② Seismic moment M0 not only has clear physical meaning, but also overcomes the deficiencies existing in ML, mb （mB ） and Ms magnitude scales, so it is the most suitable physical quantity for measuring earthquake size scientifically. In order to continue to use the term ＂magnitude＂, Kanamori defined the moment magnitude scale Act. Although its prerequisite assumptions remain to be studied, it is still a reasonable scale used as a measure of the relative size of an earthquake. ③ For measuring the earthquake size more scientifically, we must make full use of a large amount of waveform data from modern regional digital seismograph networks, strengthen the research on seismic wave attenuation characteristics, site effect, calculation of source parameters and the related scaling relations. In improving the measurement methods for ML, mb （mB ） and Ms magnitude, we should focus on the improvement of Mw scale and carry forward the work as gradually taking Mw magnitude scale as the uniform physical quantity to measure the relative size of earthquakes, so as to lay a more solid foundation for research in earthquake science and earthquake prediction.
文摘Conventional correlation matching algorithms waste great time in invalid area search. This paper proposes a color tracking method based on correlation search area optimization on target characteristic hue decision. By quantifying and reducing dimensions of HSV（ hue saturation value） color space, a one-dimensional hue space is constructed. In the space, the target characteristic hue granule set is constructed, which contains attributes such as value, area and average distance between pixels and aiming center. By using granular computing method, the similarity between target and search blocks is obtained and the invalid search areas can be removed. The color tracking experiment has proved that the algorithm can improve real time performance for conventional matching algorithms without precision lost.
基金supported by a grant from the National Key Technology R&D Program in the Eleventh"Five-year Plan"Period ( 20070403-2006BAC01B03-02-02)fund for earthquake research (200708020),China
文摘The enumerating algorithm has been introduced into the fitting procedure of the ASR model. Based on the detailed study of 21 large earthquakes with M≥6. 8 in the Chinese Mainland,the statistical features of seismic strain release before large earthquakes have been summarized. In the mass,the strain release models can be divided into five types. The first is the DA model,in which the strain release accelerates in broader areas and decelerates in small areas around the epicenter. Approximately 38% of earthquake samples are of this type. The second is the AD model,in which the strain release decelerates in broader areas and accelerates in smaller areas around the epicenter with an occupying ratioof approximately 19%. The third is ASR,in which only accelerating strain release can be observed. Cases of this model amount to about 14%. The fourth is DSR,in which only decelerating strain release can be checked,amounting to about 24%. There is only one earthquake sample of the fifth type (LSR),which shows a linear strain release. There is a 3～6 years difference in the duration of pre-shock sequences between the accelerating and decelerating models. This means that seismic quiescence against a background of increased seismicity of small earthquakes before large earthquakes are a typical feature in general. For the DA model,the average size of critical regions for steady accelerating and decelerating strain release is about 260km to 400km and 100km to 200km,respectively,3 to 5 times and 1 to 2 times the rupture size of an earthquake of magnitude 7. 0. The AD model is the opposite of the DA model. The model parameter,m value,has good stability. The ratio of ASR is about the same for accelerating seismic strain release phenomena,no matter what the strain release models are,or how large the strain release quantity is. With regard to decelerating seismic strain release phenomena, the DA model has the most distinctive decelerating strain release characteristic and is the typical feature of seismic strain release,i. e. "decelerating in-accelerating out seismic strain model".
基金supported by National Natural Science Foundation of China under Grant No.10775035
文摘In this paper we study a negatively charged exciton （NCE）, which is trapped by a two-dimensional （2D） parabolic potential. By using matrix diagonalization techniques, the correlation energies of the low-lying states with L=0, 1, and 2 are calculated as a function of confinement strength. We find that the size effects of different states are different. This phenomenon can be explained as a hidden symmetry, which is originated purely from symmetry. Based on symmetry, the features of the low-lying states are discussed in the influence of the 2D parabolic potential well. It is found that the confinement may cause accidental degeneracies between levels with different low-excited states. It is shown that the effect of quantum confinement on the binding energy of the heavy hole is stronger than that of a light hole.
