The seasonal variations of the Kuroshio intrusion pathways northeast of Taiwan were investigated using observational data from satellite-tracked sea surface drifters and a numerical particle-tracking experiment based ...The seasonal variations of the Kuroshio intrusion pathways northeast of Taiwan were investigated using observational data from satellite-tracked sea surface drifters and a numerical particle-tracking experiment based on a high-resolution numerical ocean model. The results of sea surface drifter data observed from 1989 to 2013 indicate that the Kuroshio surface intrusion follows two distinct pathways: one is a northwestward intrusion along the northern coast of Taiwan Island, and the other is a direct intrusion near the turn of the shelf break. The former occurs primarily in the winter, while the latter exists year round. A particle-tracking experiment in the high-resolution numerical model reproduces the two observed intrusion paths by the sea surface drifters. The three-dimensional structure of the Kuroshio intrusion is revealed by the model results. The pathways, features and possible dynamic mechanisms of the subsurface intrusion are also discussed.展开更多
Isolation and purification of single-walled carbon nanotubes （SWCNTs） are prerequisites for their implementation in various applications. In this work, we present a fast （-5 min）, low-cost, and easily scalable ben...Isolation and purification of single-walled carbon nanotubes （SWCNTs） are prerequisites for their implementation in various applications. In this work, we present a fast （-5 min）, low-cost, and easily scalable bench-top approach to the extraction of high-quality isolated SWCNTs from bundles and impurities in an aqueous dispersion. The extraction procedure, based on aqueous two-phase （ATP） separation, is widely applicable to any SWCNT source （tested on samples up to 1.7 nm in diameter） and independent of defect density, purity, diameter, and length. The extracted dispersions demonstrate that the removal of large aggregates, small bundles, and impurities is comparable to that by density gradient ultracentrifugation, but without the need for high-end instrumentation. Raman and fluorescence-excitation spectroscopy, single-nanotube fluorescence imaging, atomic force and transmission electron microscopy, and thermogravimetric analysis all confirm the high purity of the isolated SWCNTs. By predispersing the SWCNTs without sonication （only gentle stirring）, full-length, pristine SWCNTs can be isolated （tested up to 20 μm）. Hence, this simple ATP method will find immediate application in the generation of SWCNT materials for all levels of nanotube research and applications, from fundamental studies to high-performance devices.展开更多
基金supported by the National Basic Research Program of China(Grant Nos.2013CB430302&2014CB-745000)the National Natural Science Foundation of China(Grant Nos.41321004+5 种基金911282044110602041476022&41490643)the Scientific Research Fund of the Second Institute of OceanographySOA(Grant No.JT1205)the National Program on Global Change and Air-Sea Interaction(Grant No.GASI-03-IPOVAI-05)
文摘The seasonal variations of the Kuroshio intrusion pathways northeast of Taiwan were investigated using observational data from satellite-tracked sea surface drifters and a numerical particle-tracking experiment based on a high-resolution numerical ocean model. The results of sea surface drifter data observed from 1989 to 2013 indicate that the Kuroshio surface intrusion follows two distinct pathways: one is a northwestward intrusion along the northern coast of Taiwan Island, and the other is a direct intrusion near the turn of the shelf break. The former occurs primarily in the winter, while the latter exists year round. A particle-tracking experiment in the high-resolution numerical model reproduces the two observed intrusion paths by the sea surface drifters. The three-dimensional structure of the Kuroshio intrusion is revealed by the model results. The pathways, features and possible dynamic mechanisms of the subsurface intrusion are also discussed.
文摘Isolation and purification of single-walled carbon nanotubes （SWCNTs） are prerequisites for their implementation in various applications. In this work, we present a fast （-5 min）, low-cost, and easily scalable bench-top approach to the extraction of high-quality isolated SWCNTs from bundles and impurities in an aqueous dispersion. The extraction procedure, based on aqueous two-phase （ATP） separation, is widely applicable to any SWCNT source （tested on samples up to 1.7 nm in diameter） and independent of defect density, purity, diameter, and length. The extracted dispersions demonstrate that the removal of large aggregates, small bundles, and impurities is comparable to that by density gradient ultracentrifugation, but without the need for high-end instrumentation. Raman and fluorescence-excitation spectroscopy, single-nanotube fluorescence imaging, atomic force and transmission electron microscopy, and thermogravimetric analysis all confirm the high purity of the isolated SWCNTs. By predispersing the SWCNTs without sonication （only gentle stirring）, full-length, pristine SWCNTs can be isolated （tested up to 20 μm）. Hence, this simple ATP method will find immediate application in the generation of SWCNT materials for all levels of nanotube research and applications, from fundamental studies to high-performance devices.
