Photoelectrochemical(PEC)water splitting capable of reducing and oxidizing water into hydrogen and oxygen in a generation mode of spatial separation has gained extensive popularity.In order to effectively produce hydr...Photoelectrochemical(PEC)water splitting capable of reducing and oxidizing water into hydrogen and oxygen in a generation mode of spatial separation has gained extensive popularity.In order to effectively produce hydrogen at the photocathode of a PEC cell,the photoanode,where the oxygen evolution reaction occurs,should be systematically developed on priority.In particular,WO3 has been identified as one of the most promising photoanode materials owing to its narrow band gap and high valence band position.Its practical implementation,however,is still limited by excessive electron–hole recombination and poor water oxidation kinetics.This review presents the various strategies that have been studied for enhancing the PEC water oxidation performance of WO3,such as controlling the morphology,introducing defects,constructing a heterojunction,loading a cocatalyst,and exploiting the plasmonic effect.In addition,the possible future research directions are presented.展开更多
The vector transformation and pole reduction from the total-field anomaly are signifi cant for the interpretation.We examined these industry-standard processing procedures in the Fourier domain.We propose a novel iter...The vector transformation and pole reduction from the total-field anomaly are signifi cant for the interpretation.We examined these industry-standard processing procedures in the Fourier domain.We propose a novel iteration algorithm for regional magnetic anomalies transformations to derive the vertical-component data from the total-field measurements with the variation in the core-fi eld direction over the region.Additionally,we use the same algorithm to convert the calculated vertical-component data into the corresponding data at the pole and realize the processing of diff erential reduction to the pole(DRTP).Unlike Arkani-Hamed’s DRTP method,the two types of iterative algorithms have the same forms,and DRTP is realized by implementing this algorithm twice.The synthetic model’s calculation results show that the method has high accuracy,and the fi eld data processing confi rms its practicality.展开更多
基金financially supported by the National Natural Science Foundation of China (21808189, 21663027)the Science and Technology Support Project of Gansu Province (1504GKCA027)+2 种基金the Program for Innovative Research Team (NWNULKQN-15-2)the Opening Project of Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control (GKLECPC-12)the Opening Project of Key Laboratory of Green Catalysis of Sichuan Institutes of High Education (LYJ18205)~~
文摘Photoelectrochemical(PEC)water splitting capable of reducing and oxidizing water into hydrogen and oxygen in a generation mode of spatial separation has gained extensive popularity.In order to effectively produce hydrogen at the photocathode of a PEC cell,the photoanode,where the oxygen evolution reaction occurs,should be systematically developed on priority.In particular,WO3 has been identified as one of the most promising photoanode materials owing to its narrow band gap and high valence band position.Its practical implementation,however,is still limited by excessive electron–hole recombination and poor water oxidation kinetics.This review presents the various strategies that have been studied for enhancing the PEC water oxidation performance of WO3,such as controlling the morphology,introducing defects,constructing a heterojunction,loading a cocatalyst,and exploiting the plasmonic effect.In addition,the possible future research directions are presented.
基金supported by the National Key R&D Program of China (No. 2017YFC0602000)the China Geological Survey Project (Nos. DD20191001 and DD20189410)。
文摘The vector transformation and pole reduction from the total-field anomaly are signifi cant for the interpretation.We examined these industry-standard processing procedures in the Fourier domain.We propose a novel iteration algorithm for regional magnetic anomalies transformations to derive the vertical-component data from the total-field measurements with the variation in the core-fi eld direction over the region.Additionally,we use the same algorithm to convert the calculated vertical-component data into the corresponding data at the pole and realize the processing of diff erential reduction to the pole(DRTP).Unlike Arkani-Hamed’s DRTP method,the two types of iterative algorithms have the same forms,and DRTP is realized by implementing this algorithm twice.The synthetic model’s calculation results show that the method has high accuracy,and the fi eld data processing confi rms its practicality.
