利用CNKI《中国期刊全文数据库》,对2008年至2018年收录的相关文献从年度发文量、主要发文机构、被引频次与下载量等方面进行计量分析,并与Web of Science数据库该领域的研究成果进行对比分析。结果表明:统计范围内的相关文献发文总量...利用CNKI《中国期刊全文数据库》,对2008年至2018年收录的相关文献从年度发文量、主要发文机构、被引频次与下载量等方面进行计量分析,并与Web of Science数据库该领域的研究成果进行对比分析。结果表明:统计范围内的相关文献发文总量先上升后下降,发文数量最多的期刊为《环境科学与技术》和《环境科学学报》,中国科学院生态环境研究中心的发文量、综合影响力比较高,统计范围内的文献下载次数虽然多,但是篇均被引次数较低。“生态风险评价”、“沉积物”、“潜在生态风险”、“植物修复”等研究方向受关注度较高。展开更多
随着工农业的发展,河流重金属污染问题越来越受到人们的重视。近年来,全球对河流重金属污染的研究力度不断增大。利用Web of Science引文数据库,对1979—2016年间收录的相关文献进行了计量分析。结果表明:河流重金属污染研究的文献量增...随着工农业的发展,河流重金属污染问题越来越受到人们的重视。近年来,全球对河流重金属污染的研究力度不断增大。利用Web of Science引文数据库,对1979—2016年间收录的相关文献进行了计量分析。结果表明:河流重金属污染研究的文献量增长速度较快,西班牙、美国和法国等国的河流重金属污染研究论文综合影响力较高,中国发表论文的总量和总被引次数虽然最多,但篇平均被引次数较低。来自西班牙维尔瓦大学的Grande在该领域研究实力较强,Environmental Pollution是河流重金属污染研究领域最值得关注的期刊。研究的热点主要集中在河流沉积物,而汞、镉、铅、砷、锌、铜等是河流的主要重金属污染物,受关注度较高,同时基于生物监测的重金属污染评价也逐渐成为研究热点。展开更多
The Nanfei River （Anhui Province, China） is a severely polluted urban river that flows into Chaohu Lake. In the present study, sediments were collected from the river and analyzed for their heavy metal contents. Mul...The Nanfei River （Anhui Province, China） is a severely polluted urban river that flows into Chaohu Lake. In the present study, sediments were collected from the river and analyzed for their heavy metal contents. Multivariate statistics and the fuzzy comprehensive assessment method were used to determine the sources of pollution, the current pollution status, and spatial and temporal variations in heavy metal pollution in sediments. The concentrations of arsenic （As）, cadmium （Cd）, chromium （Cr）, copper （Cu）, mercury （Hg）, nickel （Ni）, lead （Pb）, and zinc （Zn） in sediments ranged from 5.67-113, 0.08-40.2, 41.6-524, 15.5-460, 0.03-4.84, 13.5-180, 18.8-250, and 47.9-1 996 mg/kg, and the average concentrations of each metal were 1.7, 38.7, 1.8, 5.5, l 8.8, 1.3, 2.5, and 11.1 times greater than the background values, respectively. Multivariate statistical analysis demonstrated that Hg, Cu, Cr, Cd, and Ni may have originated from industrial activities, whereas As and Pb came from agricultural activities. The fuzzy comprehensive assessment method, based on the fuzzy mathematics theory, was used to obtain a detailed assessment of the sediment quality in the Nanfei River watershed. The results indicated that the pollution was moderate in the downstream tributaries of the Nianbu and Dianbu Rivers, but was severe in the main channel of the Nanfei River and in the upstream tributaries of the Sill and Banqiao Rivers. Therefore, sediments in the Nanfei River watershed are heavily polluted and urgent measures should be taken to remedy the status.展开更多
Heavy metal pollutants are a worldwide concern due to slow decomposition, biocondensation, and negative effects on human health. We investigated seasonal and spatial variations of the five heavy metals and evaluated t...Heavy metal pollutants are a worldwide concern due to slow decomposition, biocondensation, and negative effects on human health. We investigated seasonal and spatial variations of the five heavy metals and evaluated their health risk in the Liaohe River, Northeast China. A total of 324 surface water samples collected from 2009 to 2010 were analyzed. Levels(high to low) of heavy metals in the Liaohe River were: zinc(Zn) > chromium(Cr) > copper(Cu) > cadmium(Cd) > mercury(Hg). Spatial and seasonal changes impacting concentrations of Cu and Zn were significant, but not significant for Cr, Cd and Hg. The highest concentrations of heavy metals were: Hg at Liuheqiao, Cu at Fudedian, Zn at Tongjiangkou, Cr at Mahushan, and Cd at Shenglitang. The highest concentrations of Hg and Cr were found in the wet period, Cu and Cd in the level period, and Zn in the dry period. The surface water of a tributary was an important accumulation site for heavy metals. Health risks from carcinogens and non-carcinogens increased from upstream to downstream in the mainstream of the Liaohe River. The total health risk for one person in the Liaohe River exceeded acceptable levels. The total health risk was the greatest during the wet period and least in the dry period. Among the five heavy metals in the Liaohe River, Cr posed the greatest single health risk.展开更多
Focusing on the origin of the heavy metal,this study aims to build an imputed method to estimate the heavy metal content in river water by making a distinction between the heavy metal of natural origins and that cause...Focusing on the origin of the heavy metal,this study aims to build an imputed method to estimate the heavy metal content in river water by making a distinction between the heavy metal of natural origins and that caused by human activities.Supported by GIS,Kosaka watershed within the Hokuroku basin was divided into several sub-watershed polygons and the outflows of water and Cu were calculated for each polygon.Compared with the natural origin,the dominant Cu emissions affected the river water more significantly in local.Based on the mass balance closure,the heavy metal content of Cu in the Kosaka River was estimated by the conflux accumulation of tributaries and mine drainages.The estimated Cu concentrations were checked by comparing with the actually measured values at monitoring points along the Kosaka River and the results are coincidence with each other in general.It is revealed that the mainstream water quality could be estimated by seizing the water quality of upstream tributaries and human drainages.展开更多
The main purpose of the research is to study the influence on shallow ground water by heavy metal in polluted river. In the lab-scale experiment polluted rivers were simulated by domestic sewage, and three kinds of na...The main purpose of the research is to study the influence on shallow ground water by heavy metal in polluted river. In the lab-scale experiment polluted rivers were simulated by domestic sewage, and three kinds of natural sand were chosen as infiltration medium, it was found that Cr（Ⅵ）penetrated on the 13th day and then had a removal ratio of 77%-99% in coarse sand,over 91% and 96% in two kinds of medium sand. From beginning to end in column 2 and column 3 the removal ratio of lead were greater than 97%. It is difficult for Cr（Ⅵ） and lead to enter ground water. In on-site test it indicates that the concentration of Cr（Ⅵ） in No.1-3 and coal yard well along the bank of Liangshui River is not greater than background concentration in groundwater, so Cr （Ⅵ） in Liangshui River has a little influence on ground water. The mechanism of Cr（Ⅵ） removal is reducing action and sedimentation. The removal mechanism of lead primarily is chemical adsorption and generation deposit. Cr（Ⅵ） mainly is transformed to precipitation by reducing action because of abundant reduction agent in the infiltration media, so the tests indicat that polluted river is not the source of Cr （Ⅵ） pollution in ground water. Generally lead may polluted soil, but not groundwater.展开更多
文摘利用CNKI《中国期刊全文数据库》,对2008年至2018年收录的相关文献从年度发文量、主要发文机构、被引频次与下载量等方面进行计量分析,并与Web of Science数据库该领域的研究成果进行对比分析。结果表明:统计范围内的相关文献发文总量先上升后下降,发文数量最多的期刊为《环境科学与技术》和《环境科学学报》,中国科学院生态环境研究中心的发文量、综合影响力比较高,统计范围内的文献下载次数虽然多,但是篇均被引次数较低。“生态风险评价”、“沉积物”、“潜在生态风险”、“植物修复”等研究方向受关注度较高。
文摘随着工农业的发展,河流重金属污染问题越来越受到人们的重视。近年来,全球对河流重金属污染的研究力度不断增大。利用Web of Science引文数据库,对1979—2016年间收录的相关文献进行了计量分析。结果表明:河流重金属污染研究的文献量增长速度较快,西班牙、美国和法国等国的河流重金属污染研究论文综合影响力较高,中国发表论文的总量和总被引次数虽然最多,但篇平均被引次数较低。来自西班牙维尔瓦大学的Grande在该领域研究实力较强,Environmental Pollution是河流重金属污染研究领域最值得关注的期刊。研究的热点主要集中在河流沉积物,而汞、镉、铅、砷、锌、铜等是河流的主要重金属污染物,受关注度较高,同时基于生物监测的重金属污染评价也逐渐成为研究热点。
基金Supported by the Major Science and Technology Program for Water Pollution Control and Treatment(No.2012ZX07103-005)
文摘The Nanfei River （Anhui Province, China） is a severely polluted urban river that flows into Chaohu Lake. In the present study, sediments were collected from the river and analyzed for their heavy metal contents. Multivariate statistics and the fuzzy comprehensive assessment method were used to determine the sources of pollution, the current pollution status, and spatial and temporal variations in heavy metal pollution in sediments. The concentrations of arsenic （As）, cadmium （Cd）, chromium （Cr）, copper （Cu）, mercury （Hg）, nickel （Ni）, lead （Pb）, and zinc （Zn） in sediments ranged from 5.67-113, 0.08-40.2, 41.6-524, 15.5-460, 0.03-4.84, 13.5-180, 18.8-250, and 47.9-1 996 mg/kg, and the average concentrations of each metal were 1.7, 38.7, 1.8, 5.5, l 8.8, 1.3, 2.5, and 11.1 times greater than the background values, respectively. Multivariate statistical analysis demonstrated that Hg, Cu, Cr, Cd, and Ni may have originated from industrial activities, whereas As and Pb came from agricultural activities. The fuzzy comprehensive assessment method, based on the fuzzy mathematics theory, was used to obtain a detailed assessment of the sediment quality in the Nanfei River watershed. The results indicated that the pollution was moderate in the downstream tributaries of the Nianbu and Dianbu Rivers, but was severe in the main channel of the Nanfei River and in the upstream tributaries of the Sill and Banqiao Rivers. Therefore, sediments in the Nanfei River watershed are heavily polluted and urgent measures should be taken to remedy the status.
基金Under the auspices of Major Science and Technology Program for Water Pollution Control and Treatment(No.2012ZX07202-004-05)National Natural Science Foundation of China(No.41401352)Science and Enterprise Competitive Selection Project of Shenyang City,Shenyang Science and Technology Plan Project(No.F14-133-9-00)
文摘Heavy metal pollutants are a worldwide concern due to slow decomposition, biocondensation, and negative effects on human health. We investigated seasonal and spatial variations of the five heavy metals and evaluated their health risk in the Liaohe River, Northeast China. A total of 324 surface water samples collected from 2009 to 2010 were analyzed. Levels(high to low) of heavy metals in the Liaohe River were: zinc(Zn) > chromium(Cr) > copper(Cu) > cadmium(Cd) > mercury(Hg). Spatial and seasonal changes impacting concentrations of Cu and Zn were significant, but not significant for Cr, Cd and Hg. The highest concentrations of heavy metals were: Hg at Liuheqiao, Cu at Fudedian, Zn at Tongjiangkou, Cr at Mahushan, and Cd at Shenglitang. The highest concentrations of Hg and Cr were found in the wet period, Cu and Cd in the level period, and Zn in the dry period. The surface water of a tributary was an important accumulation site for heavy metals. Health risks from carcinogens and non-carcinogens increased from upstream to downstream in the mainstream of the Liaohe River. The total health risk for one person in the Liaohe River exceeded acceptable levels. The total health risk was the greatest during the wet period and least in the dry period. Among the five heavy metals in the Liaohe River, Cr posed the greatest single health risk.
文摘Focusing on the origin of the heavy metal,this study aims to build an imputed method to estimate the heavy metal content in river water by making a distinction between the heavy metal of natural origins and that caused by human activities.Supported by GIS,Kosaka watershed within the Hokuroku basin was divided into several sub-watershed polygons and the outflows of water and Cu were calculated for each polygon.Compared with the natural origin,the dominant Cu emissions affected the river water more significantly in local.Based on the mass balance closure,the heavy metal content of Cu in the Kosaka River was estimated by the conflux accumulation of tributaries and mine drainages.The estimated Cu concentrations were checked by comparing with the actually measured values at monitoring points along the Kosaka River and the results are coincidence with each other in general.It is revealed that the mainstream water quality could be estimated by seizing the water quality of upstream tributaries and human drainages.
文摘The main purpose of the research is to study the influence on shallow ground water by heavy metal in polluted river. In the lab-scale experiment polluted rivers were simulated by domestic sewage, and three kinds of natural sand were chosen as infiltration medium, it was found that Cr（Ⅵ）penetrated on the 13th day and then had a removal ratio of 77%-99% in coarse sand,over 91% and 96% in two kinds of medium sand. From beginning to end in column 2 and column 3 the removal ratio of lead were greater than 97%. It is difficult for Cr（Ⅵ） and lead to enter ground water. In on-site test it indicates that the concentration of Cr（Ⅵ） in No.1-3 and coal yard well along the bank of Liangshui River is not greater than background concentration in groundwater, so Cr （Ⅵ） in Liangshui River has a little influence on ground water. The mechanism of Cr（Ⅵ） removal is reducing action and sedimentation. The removal mechanism of lead primarily is chemical adsorption and generation deposit. Cr（Ⅵ） mainly is transformed to precipitation by reducing action because of abundant reduction agent in the infiltration media, so the tests indicat that polluted river is not the source of Cr （Ⅵ） pollution in ground water. Generally lead may polluted soil, but not groundwater.
