We report the preparation of D2 molecules in v=2 level in molecular beam condition. A single longitudinal mode laser system was used for excitation of D2 from （v=0, j=0） to （v=2, j=0） with the scheme of stimulated...We report the preparation of D2 molecules in v=2 level in molecular beam condition. A single longitudinal mode laser system was used for excitation of D2 from （v=0, j=0） to （v=2, j=0） with the scheme of stimulated Raman pumping. An excitation efficiency of 25.2% has been achieved, which was determined by the scheme of resonance-enhanced multiphoton ion- ization. Dependence of relative excitation efficiency on laser energy has been measured. We found that the increasing rate of excitation efficiency became slower as pulse energy of Stokes laser increase, while the excitation efficiency still increases approximately linearly with pump pulse energies up to 60 mJ. The spectral line shapes of Raman transition was also measured at different laser energies and considerable dynamical Stark effect was observed. A single peak was found on the three dimension surface of relative excitation efficiency, indicating the process occurred in the present study is a process of stimulated Raman pumping instead of stimulated adiabatic Raman passage.展开更多
We study the statistics of the emitted filed from Rydberg atom confined inside a microcavity and interacting with a pump laser in the strong coupling regime. We explore the manifestation of the antibunching in connect...We study the statistics of the emitted filed from Rydberg atom confined inside a microcavity and interacting with a pump laser in the strong coupling regime. We explore the manifestation of the antibunching in connection with the internal system parameters.展开更多
In a Gaussian laser beam pumped single-photon frequency up-conversion system, the spatial distribution of the con- version efficiency is calculated, which strongly depends on the intensity distribution of the pump bea...In a Gaussian laser beam pumped single-photon frequency up-conversion system, the spatial distribution of the con- version efficiency is calculated, which strongly depends on the intensity distribution of the pump beam and leads to a spatial modulation of the output single photons. As a result, by simply varying the Gauss/an pump beam intensity and the beam size, the converted photons could be modulated spatially and exhibit a programmable distribution. This will be meaningful for the researches on quantum communication and quantum manipulation based on frequency up-conversion svstem.展开更多
文摘We report the preparation of D2 molecules in v=2 level in molecular beam condition. A single longitudinal mode laser system was used for excitation of D2 from （v=0, j=0） to （v=2, j=0） with the scheme of stimulated Raman pumping. An excitation efficiency of 25.2% has been achieved, which was determined by the scheme of resonance-enhanced multiphoton ion- ization. Dependence of relative excitation efficiency on laser energy has been measured. We found that the increasing rate of excitation efficiency became slower as pulse energy of Stokes laser increase, while the excitation efficiency still increases approximately linearly with pump pulse energies up to 60 mJ. The spectral line shapes of Raman transition was also measured at different laser energies and considerable dynamical Stark effect was observed. A single peak was found on the three dimension surface of relative excitation efficiency, indicating the process occurred in the present study is a process of stimulated Raman pumping instead of stimulated adiabatic Raman passage.
文摘We study the statistics of the emitted filed from Rydberg atom confined inside a microcavity and interacting with a pump laser in the strong coupling regime. We explore the manifestation of the antibunching in connection with the internal system parameters.
基金supported by the National Natural Science Foundation of China(Nos.61127014,61378033 and 11434005)the National Key Scientific Instrument Project(No.2012YQ150092)+2 种基金the Program of Introducing Talents of Discipline to Universities(No.B12024)the Shanghai Rising-Star Program(No.13QA1401300)the Shanghai International Cooperation Project(No.13520720700)
文摘In a Gaussian laser beam pumped single-photon frequency up-conversion system, the spatial distribution of the con- version efficiency is calculated, which strongly depends on the intensity distribution of the pump beam and leads to a spatial modulation of the output single photons. As a result, by simply varying the Gauss/an pump beam intensity and the beam size, the converted photons could be modulated spatially and exhibit a programmable distribution. This will be meaningful for the researches on quantum communication and quantum manipulation based on frequency up-conversion svstem.
