本文从非线性耦合波理论的观点分析了单模光纤中受激喇曼散射瞬态过程,给出了解答的解析表达式。由此得到稳态过程的解答,并分析了该稳态过程。该稳态分析所得结论与 Yariv 等从光子转换理论所得稳态结论相一致,并对 Smith 的小信号解...本文从非线性耦合波理论的观点分析了单模光纤中受激喇曼散射瞬态过程,给出了解答的解析表达式。由此得到稳态过程的解答,并分析了该稳态过程。该稳态分析所得结论与 Yariv 等从光子转换理论所得稳态结论相一致,并对 Smith 的小信号解答作了进一步完善。展开更多
Real-time continuous-wave terahertz imaging is demonstrated with a 1.63 THz (184.31 lam) optically-pumped terahertz laser (OPTL) and a 124 × 124 element room-temperature pyroelectric camera. Transmission-mode...Real-time continuous-wave terahertz imaging is demonstrated with a 1.63 THz (184.31 lam) optically-pumped terahertz laser (OPTL) and a 124 × 124 element room-temperature pyroelectric camera. Transmission-mode THz imaging is presented for the samples hidden in various wrapping materials. These experimental results reveal the possibility to construct a simple real-time THz imaging system applied to nondestructive inspection.展开更多
Resonance enhancement has been increasingly employed in the emergent felntosecond stimu- lated Raman spectroscopy (FSRS) to selectively monitor molecular structure and dynamics with improved spectral and temporal re...Resonance enhancement has been increasingly employed in the emergent felntosecond stimu- lated Raman spectroscopy (FSRS) to selectively monitor molecular structure and dynamics with improved spectral and temporal resolutions and signal-to-noise ratios. Such joint eflforts by the technique- and application-oriented scientists and engineers have laid the foundation for exploiting the tunable FSRS methodology to investigate a great variety of photosensitive systems and elucidate the underlying functional mechanisms on molecular time scales. Dur- ing spectral analysis, peak line shapes remain a major concern with an intricate dependence on resonance conditions. Here, we present a comprehensive study of line shapes by tuning the Rarnan pump wavelength from red to blue side of the ground-state absorption band of the fluorescent dye rhodarnine 6G in solution. Distinct line shape patterns in Stokes and anti-Stokes FSRS as well as from the low to high-frequency modes highlight the competition between multiple third-order and higher-order nonlinear pathways, governed by difl^rent res- onance conditions achieved by Raman pump and probe pulses. In particular, the resonance condition of probe wavelength is revealed to play an important role in generating circular line shape changes through oppositely phased dispersion via hot luminescence (HL) pathways. Meanwhile, on-resonance conditions of the Rarnan pump could promote excited-state vibrational modes which are broadened and red-shifted from the coincident ground-state vibrational modes, posing challenges for spectral analysis. Certain strategies in tuning the Raman pump and probe to characteristic regions across an electronic transition band are discussed to improve the FSRS usability and versatility as a powerful structural dynamics toolset to advance chemical, physical, materials, and biological sciences.展开更多
The energy levels, wave functions and the second-order nonlinear susceptibilities are calculated in GaAs/Al0.2Ga0.8As/Al0.5Ga0.5As asymmetric quantum well (AQW) by using an asymmetric model based on the parabolic an...The energy levels, wave functions and the second-order nonlinear susceptibilities are calculated in GaAs/Al0.2Ga0.8As/Al0.5Ga0.5As asymmetric quantum well (AQW) by using an asymmetric model based on the parabolic and non-parabolic band. The influence of non-parabolicity can not be neglected when analyzing the phenomena in narrow quantum wells and in higher lying subband edges in wider wells. The numerical results show that under double resonance (DR) conditions, the second- order difference frequency generation (DFG) and optical rectification (OR) generation susceptibilities in the AQW reach 2.5019 μm/V and 13.208 μm/V, respectively, which are much larger than those of the bulk GaAs. Besides, we calculate the absorption coefficient of AQW and find out the two pump wavelengths correspond to the maximum absorption, so appropriate pump beams must be selected to generate terahertz (THz) radiation by DFG.展开更多
A polarization-dependent supercontinuum spectrum source of light from the UV to infrared region has been generated in our photonic crystal fiber with birefringence B=2.23×10 3.By tuning the polarization direction...A polarization-dependent supercontinuum spectrum source of light from the UV to infrared region has been generated in our photonic crystal fiber with birefringence B=2.23×10 3.By tuning the polarization direction of the input pulse,it is found that the width of the supercontinuum spectrum changes dramatically with the input polarization directions.At the same time,we qualitatively explain the blue-shift peak and the red-shift peak in the experimental spectrum using phase matching conditions on dispersive waves,stoke waves and the pump wave.In addition,we also found that supercontinuum spectrum generation,to some extent,is dependent on the pump wavelength and average power of the pump.The spectrum is broadened with the increase of average power,but unchanged after average power reaches a certain value;when the pump wavelength is located in the anomalous dispersion and further away from the zero-dispersion wavelength,the spectrum of the supercontinuum is wider.展开更多
We demonstrate a laser-diode (LD) pumped actively Q-switched laser with Nd:Sc0.2Y0.5SiO5 (Nd:SYSO) crystal for the first time. A stable actively Q-switched laser is obtained at dual wavelengths of 1 075.2 nm and...We demonstrate a laser-diode (LD) pumped actively Q-switched laser with Nd:Sc0.2Y0.5SiO5 (Nd:SYSO) crystal for the first time. A stable actively Q-switched laser is obtained at dual wavelengths of 1 075.2 nm and 1 078.2 nm. The maximum average output power of 720 mW is obtained at the repetition rate of 15 kHz under the pump power of 8.7 W. The minimum pulse width of 58 ns is obtained at the repetition rate of 5 kHz under the pump power of 8.7 W, corresponding to the peak power of 1.9 kW and the pulse energy of 112 μJ.展开更多
An all-solid-state Pr:KY3F10(Pr:KYF) laser pumped by blue laser(471 nm) has been demonstrated.With the incident pump power of 2.6 W,the maximum output power at 610 nm is 213 mW.Moreover,the intracavity second-harmonic...An all-solid-state Pr:KY3F10(Pr:KYF) laser pumped by blue laser(471 nm) has been demonstrated.With the incident pump power of 2.6 W,the maximum output power at 610 nm is 213 mW.Moreover,the intracavity second-harmonic generation(SHG) is also achieved with the maximum ultraviolet(UV) power at 305 nm of 11 mW by using a β-BaB2O4(BBO) nonlinear crystal.展开更多
文摘Real-time continuous-wave terahertz imaging is demonstrated with a 1.63 THz (184.31 lam) optically-pumped terahertz laser (OPTL) and a 124 × 124 element room-temperature pyroelectric camera. Transmission-mode THz imaging is presented for the samples hidden in various wrapping materials. These experimental results reveal the possibility to construct a simple real-time THz imaging system applied to nondestructive inspection.
基金supported by the U.S.National Science Foundation CAREER grant(CHE-1455353)the Oregon State University(OSU) Research Equipment Reserve Fund(Spring 2014)to C.Fang(USTC9603)the Wei Family Private Foundation in supporting C.Chen(USTC 0903) during his graduate studies at OSU Chemistry
文摘Resonance enhancement has been increasingly employed in the emergent felntosecond stimu- lated Raman spectroscopy (FSRS) to selectively monitor molecular structure and dynamics with improved spectral and temporal resolutions and signal-to-noise ratios. Such joint eflforts by the technique- and application-oriented scientists and engineers have laid the foundation for exploiting the tunable FSRS methodology to investigate a great variety of photosensitive systems and elucidate the underlying functional mechanisms on molecular time scales. Dur- ing spectral analysis, peak line shapes remain a major concern with an intricate dependence on resonance conditions. Here, we present a comprehensive study of line shapes by tuning the Rarnan pump wavelength from red to blue side of the ground-state absorption band of the fluorescent dye rhodarnine 6G in solution. Distinct line shape patterns in Stokes and anti-Stokes FSRS as well as from the low to high-frequency modes highlight the competition between multiple third-order and higher-order nonlinear pathways, governed by difl^rent res- onance conditions achieved by Raman pump and probe pulses. In particular, the resonance condition of probe wavelength is revealed to play an important role in generating circular line shape changes through oppositely phased dispersion via hot luminescence (HL) pathways. Meanwhile, on-resonance conditions of the Rarnan pump could promote excited-state vibrational modes which are broadened and red-shifted from the coincident ground-state vibrational modes, posing challenges for spectral analysis. Certain strategies in tuning the Raman pump and probe to characteristic regions across an electronic transition band are discussed to improve the FSRS usability and versatility as a powerful structural dynamics toolset to advance chemical, physical, materials, and biological sciences.
基金supported by the National Basic Research Program of China (No.2007CB310403)the National Natural Science Foundation of China (Nos.60801017 and 61172010)the Science and Technology Committee of Tianjin (No.11JCYBJC01100)
文摘The energy levels, wave functions and the second-order nonlinear susceptibilities are calculated in GaAs/Al0.2Ga0.8As/Al0.5Ga0.5As asymmetric quantum well (AQW) by using an asymmetric model based on the parabolic and non-parabolic band. The influence of non-parabolicity can not be neglected when analyzing the phenomena in narrow quantum wells and in higher lying subband edges in wider wells. The numerical results show that under double resonance (DR) conditions, the second- order difference frequency generation (DFG) and optical rectification (OR) generation susceptibilities in the AQW reach 2.5019 μm/V and 13.208 μm/V, respectively, which are much larger than those of the bulk GaAs. Besides, we calculate the absorption coefficient of AQW and find out the two pump wavelengths correspond to the maximum absorption, so appropriate pump beams must be selected to generate terahertz (THz) radiation by DFG.
基金supported by the National Natural Science Foundation of China (Grant No.10874145)Specialized Research Fund for the Doctoral Program of Higher Education (Grant No.20091333110010)+1 种基金the Natural Science Foundation of Hebei Province (Grant No.F2009000481)the China Postdoctoral Science Foundation (Grant Nos.20080440014 and 200902046)
文摘A polarization-dependent supercontinuum spectrum source of light from the UV to infrared region has been generated in our photonic crystal fiber with birefringence B=2.23×10 3.By tuning the polarization direction of the input pulse,it is found that the width of the supercontinuum spectrum changes dramatically with the input polarization directions.At the same time,we qualitatively explain the blue-shift peak and the red-shift peak in the experimental spectrum using phase matching conditions on dispersive waves,stoke waves and the pump wave.In addition,we also found that supercontinuum spectrum generation,to some extent,is dependent on the pump wavelength and average power of the pump.The spectrum is broadened with the increase of average power,but unchanged after average power reaches a certain value;when the pump wavelength is located in the anomalous dispersion and further away from the zero-dispersion wavelength,the spectrum of the supercontinuum is wider.
基金supported by the National Natural Science Foundation of China(No.11104161)the High School Science and Technology Planning Project of Shandong Province in China(No.J11LA12)the Open Project of State Key Laboratory of Crystal Materials(No.KF1103)
文摘We demonstrate a laser-diode (LD) pumped actively Q-switched laser with Nd:Sc0.2Y0.5SiO5 (Nd:SYSO) crystal for the first time. A stable actively Q-switched laser is obtained at dual wavelengths of 1 075.2 nm and 1 078.2 nm. The maximum average output power of 720 mW is obtained at the repetition rate of 15 kHz under the pump power of 8.7 W. The minimum pulse width of 58 ns is obtained at the repetition rate of 5 kHz under the pump power of 8.7 W, corresponding to the peak power of 1.9 kW and the pulse energy of 112 μJ.
基金supported by the National Natural Science Foundation of China (No.61108029)
文摘An all-solid-state Pr:KY3F10(Pr:KYF) laser pumped by blue laser(471 nm) has been demonstrated.With the incident pump power of 2.6 W,the maximum output power at 610 nm is 213 mW.Moreover,the intracavity second-harmonic generation(SHG) is also achieved with the maximum ultraviolet(UV) power at 305 nm of 11 mW by using a β-BaB2O4(BBO) nonlinear crystal.