Here, we report a trap-assisted photomultiplication (PM) phenomenon in solution-processed organic photodetectors (OPDs) using poly(3-hexylthiophene) (P3HT): indene-C60 bisadduct (ICBA) as the active layer. ...Here, we report a trap-assisted photomultiplication (PM) phenomenon in solution-processed organic photodetectors (OPDs) using poly(3-hexylthiophene) (P3HT): indene-C60 bisadduct (ICBA) as the active layer. The maximum external quantum efficiency (EQE) is 685% for the device with 2% ICBA doping ratio, which is much higher than that of OPDs with P3HT:ICBA (1:1) as the active layer. The PM phenomenon is attributed to the hole tunneling injection assisted by trapped electron in ICBA near A1 cathode, which can be demonstrated from the EQE spectra and transient photocurrent curves of OPDs with different ICBA doping ratios.展开更多
In this work, we study an entanglement concentration scheme in a 3-mode optomechanical system. The scheme is based on phonon counting measurements, which can be performed through photon counting of an auxiliary cavity...In this work, we study an entanglement concentration scheme in a 3-mode optomechanical system. The scheme is based on phonon counting measurements, which can be performed through photon counting of an auxiliary cavity connected to the mechanical resonator. The amount of entanglement between the two cavity output modes is found to increase logarithmically with the number of detected phonons(photons). Such an entanglement concentration scheme is deterministic since, independently of the number of detected phonons(photons), the measurement always leads to an increase in output entanglement. Besides numerical simulations,we provide analytical results and physical insight for the improved entanglement and the concentration efficiency.展开更多
The aim of this study was to evaluate the influence of different entrance surface treatments of the scintillator on the intrinsic spatial resolution of a scintillation camera.The primary scintillation light reflection...The aim of this study was to evaluate the influence of different entrance surface treatments of the scintillator on the intrinsic spatial resolution of a scintillation camera.The primary scintillation light reflection on the entrance surface of a scintillator may be affected by the optical coating of the entrance surface,resulting in either spatial resolution or system detection efficiency degradation.A Monte Carlo simulation model,based on Geant4 codes,was developed in order to study the scintillation light transportation in the scintillator with an entrance surface of various optical coatings.The results demonstrated that the application of retro-reflector on entrance surface of the scintillation crystal can significantly improve the intrinsic spatial resolution of the scintillation camera.The physical mechanism of the improvement of spatial resolution is explored.展开更多
This work presents the study of optical constants and film thickness of blended organic thin films, emphasizing on the modeling procedure with modified genetic algorithm aided by absorption or transmittance spectra of...This work presents the study of optical constants and film thickness of blended organic thin films, emphasizing on the modeling procedure with modified genetic algorithm aided by absorption or transmittance spectra of both pure materials and the blends. Taking the blending of copper phthalocyanine(Cu Pc) and fullerene(C60) as an example, a simple, convenient and low-cost method for the determination of the optical constants and film thickness of blended organic thin films was demonstrated. New scheme for optical modeling of blended organic thin film was proposed by introducing peak energies of Cody-Lorentz oscillators of the pure materials, which were determined by fitting the film absorption of pure materials. These oscillators of pure materials could be recognized in the transmittance spectrum of their blends, and were further used as the initial searching ranges in the simulation of blended films. As a result, the constraint bounds of the unknown parameters were significantly reduced and modeling efficiency as well as fitting accuracy was improved. For instance, the fitting of the transmittance curves of blended films with different blending ratios reached reliable results in comparison with extinction coefficients obtained from experiment.展开更多
Due to distinctive lattice and electronic properties,the thiocyanate anion(SCN-)perovskite as an alluring two-dimensional(2D)material system,can be applied in optoelectronic devices.Herein,both photovoltaic and photod...Due to distinctive lattice and electronic properties,the thiocyanate anion(SCN-)perovskite as an alluring two-dimensional(2D)material system,can be applied in optoelectronic devices.Herein,both photovoltaic and photodetection performances of the 2D Cs2Pb(SCN)2I2 have been investigated.Compared with the conventional cationic 2D perovskites,Cs2Pb(SCN)2I2 possesses ultra-small interlayer spacing,additional interlayer nano channels,which is thus beneficial for charge transport ability.The planar heterojunction solar cell based on Cs2Pb(SCN)2I2 as the light absorber,has presented the highest power conversion efficiency among long-chain-cation-based 2D perovskite devices.Besides,the Cs2Pb(SCN)2I2-based photodetector also exhibits much higher photodetection performance(i.e.quantum efficiency,on/off ratio,responsivity,detectivity,response speed,polarization sensitivity and detection stability).It is thus suggested that these outstanding photoelectric characteristics of Cs2Pb(SCN)2I2 could bring huge opportunities for its more abundant optoelectronic applications,such as field-effect transistor and light-emitting diodes.展开更多
基金supported by the National Training Program of Innovation and Entrepreneurship for Undergraduates,Fundamental Research Funds for the Central Universities(Grant No.2014JBZ017)National Natural Science Foundation of China(Grant No.613770029)Beijing Natural Science Foundation(Grant No.2122050)
文摘Here, we report a trap-assisted photomultiplication (PM) phenomenon in solution-processed organic photodetectors (OPDs) using poly(3-hexylthiophene) (P3HT): indene-C60 bisadduct (ICBA) as the active layer. The maximum external quantum efficiency (EQE) is 685% for the device with 2% ICBA doping ratio, which is much higher than that of OPDs with P3HT:ICBA (1:1) as the active layer. The PM phenomenon is attributed to the hole tunneling injection assisted by trapped electron in ICBA near A1 cathode, which can be demonstrated from the EQE spectra and transient photocurrent curves of OPDs with different ICBA doping ratios.
基金supported by the Chinese Youth 1000 Talents Program and the National Natural Science Foundation of China(Grant No.11434011)
文摘In this work, we study an entanglement concentration scheme in a 3-mode optomechanical system. The scheme is based on phonon counting measurements, which can be performed through photon counting of an auxiliary cavity connected to the mechanical resonator. The amount of entanglement between the two cavity output modes is found to increase logarithmically with the number of detected phonons(photons). Such an entanglement concentration scheme is deterministic since, independently of the number of detected phonons(photons), the measurement always leads to an increase in output entanglement. Besides numerical simulations,we provide analytical results and physical insight for the improved entanglement and the concentration efficiency.
文摘The aim of this study was to evaluate the influence of different entrance surface treatments of the scintillator on the intrinsic spatial resolution of a scintillation camera.The primary scintillation light reflection on the entrance surface of a scintillator may be affected by the optical coating of the entrance surface,resulting in either spatial resolution or system detection efficiency degradation.A Monte Carlo simulation model,based on Geant4 codes,was developed in order to study the scintillation light transportation in the scintillator with an entrance surface of various optical coatings.The results demonstrated that the application of retro-reflector on entrance surface of the scintillation crystal can significantly improve the intrinsic spatial resolution of the scintillation camera.The physical mechanism of the improvement of spatial resolution is explored.
基金supported by the National Natural Foundation of China(Grant Nos.61077021 and 61076016)the Fund of Nanjing University of Posts and Telecommunications(Grant Nos.NY212076 and NY212050)
文摘This work presents the study of optical constants and film thickness of blended organic thin films, emphasizing on the modeling procedure with modified genetic algorithm aided by absorption or transmittance spectra of both pure materials and the blends. Taking the blending of copper phthalocyanine(Cu Pc) and fullerene(C60) as an example, a simple, convenient and low-cost method for the determination of the optical constants and film thickness of blended organic thin films was demonstrated. New scheme for optical modeling of blended organic thin film was proposed by introducing peak energies of Cody-Lorentz oscillators of the pure materials, which were determined by fitting the film absorption of pure materials. These oscillators of pure materials could be recognized in the transmittance spectrum of their blends, and were further used as the initial searching ranges in the simulation of blended films. As a result, the constraint bounds of the unknown parameters were significantly reduced and modeling efficiency as well as fitting accuracy was improved. For instance, the fitting of the transmittance curves of blended films with different blending ratios reached reliable results in comparison with extinction coefficients obtained from experiment.
基金supported by the National Key R&D Program of China(2018YFB1500101)the National Natural Science Foundation of China(11874402,51421002,51627803,91733301 and 51761145042)the International Partnership Program of Chinese Academy of Sciences(112111KYSB20170089)。
文摘Due to distinctive lattice and electronic properties,the thiocyanate anion(SCN-)perovskite as an alluring two-dimensional(2D)material system,can be applied in optoelectronic devices.Herein,both photovoltaic and photodetection performances of the 2D Cs2Pb(SCN)2I2 have been investigated.Compared with the conventional cationic 2D perovskites,Cs2Pb(SCN)2I2 possesses ultra-small interlayer spacing,additional interlayer nano channels,which is thus beneficial for charge transport ability.The planar heterojunction solar cell based on Cs2Pb(SCN)2I2 as the light absorber,has presented the highest power conversion efficiency among long-chain-cation-based 2D perovskite devices.Besides,the Cs2Pb(SCN)2I2-based photodetector also exhibits much higher photodetection performance(i.e.quantum efficiency,on/off ratio,responsivity,detectivity,response speed,polarization sensitivity and detection stability).It is thus suggested that these outstanding photoelectric characteristics of Cs2Pb(SCN)2I2 could bring huge opportunities for its more abundant optoelectronic applications,such as field-effect transistor and light-emitting diodes.