Liquid phase axial mixing was measured with the tracer technique in a packed column with inner diameter of 0.15m, in which the structured packing, Mellapak 350Y, was installed. Tap water as the liquid phase flowed dow...Liquid phase axial mixing was measured with the tracer technique in a packed column with inner diameter of 0.15m, in which the structured packing, Mellapak 350Y, was installed. Tap water as the liquid phase flowed down through the column and stagnant gas was at elevated pressure ranging from atmospheric to 2.0MPa. The model parameters of Bo and 9 were estimated with the least square method in the time domain. As liquid flow rate was increased, the liquid axial mixing decreased. Under our experimental conditions, the effect of pressure on Bo number on single liquid phase was negligible, and eddy diffusion was believed to be the primary cause of axial mixing in liquid phase.展开更多
An experimental study of the extent of axial backmixing in both gas and liquid phases was conducted in a 150 mm ID column packed with Mellapak 250Y corrugated structured packing. The column was operated at pressures r...An experimental study of the extent of axial backmixing in both gas and liquid phases was conducted in a 150 mm ID column packed with Mellapak 250Y corrugated structured packing. The column was operated at pressures ranging from 0.3 MPa to 2.0MPa with nitrogen and water flowing countercurrently through the packing. The amount of axial backmixing was experimentally evaluated by the pulse response techniques using hydrogen in gas phase and an aqueous solution of NaCl in liquid phase as inert tracers. The response of the tracer was monitored by means of thermal conductivity in the gas phase and electrical conductance in the liquid phase. The experimentally determined residence time distribution (RTD) curves were interpreted in terms of the diffusion-type modei. The results indicated that the axial backmixing in the gas increased notably with gas flowrate and slightly with operating pressure and liquid flowrate. The liquid-phase axial backmixing was an increasing function of both gas and liquid flowrates and insensitive to pressure. Various correlations were developed for reproducing the experimental mixing data. The agreement between experimental and correlated data appeared to be acceptable and within ±20% of difference.展开更多
基金Supported by the National Natural Science Foundation of China (No. 20136010).
文摘Liquid phase axial mixing was measured with the tracer technique in a packed column with inner diameter of 0.15m, in which the structured packing, Mellapak 350Y, was installed. Tap water as the liquid phase flowed down through the column and stagnant gas was at elevated pressure ranging from atmospheric to 2.0MPa. The model parameters of Bo and 9 were estimated with the least square method in the time domain. As liquid flow rate was increased, the liquid axial mixing decreased. Under our experimental conditions, the effect of pressure on Bo number on single liquid phase was negligible, and eddy diffusion was believed to be the primary cause of axial mixing in liquid phase.
基金National Natural Science Foundation of China(No. 20136010)
文摘An experimental study of the extent of axial backmixing in both gas and liquid phases was conducted in a 150 mm ID column packed with Mellapak 250Y corrugated structured packing. The column was operated at pressures ranging from 0.3 MPa to 2.0MPa with nitrogen and water flowing countercurrently through the packing. The amount of axial backmixing was experimentally evaluated by the pulse response techniques using hydrogen in gas phase and an aqueous solution of NaCl in liquid phase as inert tracers. The response of the tracer was monitored by means of thermal conductivity in the gas phase and electrical conductance in the liquid phase. The experimentally determined residence time distribution (RTD) curves were interpreted in terms of the diffusion-type modei. The results indicated that the axial backmixing in the gas increased notably with gas flowrate and slightly with operating pressure and liquid flowrate. The liquid-phase axial backmixing was an increasing function of both gas and liquid flowrates and insensitive to pressure. Various correlations were developed for reproducing the experimental mixing data. The agreement between experimental and correlated data appeared to be acceptable and within ±20% of difference.
