It is a great advantage to design advanced materials with outstanding porosity and controllable band gab. In this study, （Fe, Ti）-containing mesoporous silica （x Fe/Ti-HMS） nanoparticles were prepared by a photo-a...It is a great advantage to design advanced materials with outstanding porosity and controllable band gab. In this study, （Fe, Ti）-containing mesoporous silica （x Fe/Ti-HMS） nanoparticles were prepared by a photo-assisted deposition PAD technique, where x is a nominal composition ofFe （l to 4 wt%））. The prepared samples were characterized by DR-UV, XRD, and TEM techniques. The results showed the insertion of Fe into intra-framework of Ti-HMS resulted in a gradual narrowing of the band gap of Ti-HMS samples with increment of Fe wt%. TEM observations reveal that Fe nanoparticles are evenly distributed within Ti-HSM matrix at different Fe wt%. Such results indicate the possibility to control the band gap of a single-site photocatalyst （Ti-HMS） by coupling it with the conventional nano-sized Fe catalysts.展开更多
Multi-lasers are proposed to enhance the proton acceleration in laser plasma interaction. A rear-holed target is illuminated by three lasers from different directions. The scheme is demonstrated by two-dimensional par...Multi-lasers are proposed to enhance the proton acceleration in laser plasma interaction. A rear-holed target is illuminated by three lasers from different directions. The scheme is demonstrated by two-dimensional particlein-cell simulations. The electron cloud shape is controlled well and the electron density is improved significantly. The electrons accelerated by the three lasers induce an enhanced target normal sheath acceleration(TNSA) which suppresses the proton beam divergence and improves the maximum proton energy. The maximum proton energy is 22.9 Me V, which increased significantly than that of a single-laser target interaction. Meanwhile, the average divergence angle(22.3?) is reduced. The dependence of the proton beam on the length of sidewall is investigated in detail and the optimal length is obtained.展开更多
文摘It is a great advantage to design advanced materials with outstanding porosity and controllable band gab. In this study, （Fe, Ti）-containing mesoporous silica （x Fe/Ti-HMS） nanoparticles were prepared by a photo-assisted deposition PAD technique, where x is a nominal composition ofFe （l to 4 wt%））. The prepared samples were characterized by DR-UV, XRD, and TEM techniques. The results showed the insertion of Fe into intra-framework of Ti-HMS resulted in a gradual narrowing of the band gap of Ti-HMS samples with increment of Fe wt%. TEM observations reveal that Fe nanoparticles are evenly distributed within Ti-HSM matrix at different Fe wt%. Such results indicate the possibility to control the band gap of a single-site photocatalyst （Ti-HMS） by coupling it with the conventional nano-sized Fe catalysts.
文摘Multi-lasers are proposed to enhance the proton acceleration in laser plasma interaction. A rear-holed target is illuminated by three lasers from different directions. The scheme is demonstrated by two-dimensional particlein-cell simulations. The electron cloud shape is controlled well and the electron density is improved significantly. The electrons accelerated by the three lasers induce an enhanced target normal sheath acceleration(TNSA) which suppresses the proton beam divergence and improves the maximum proton energy. The maximum proton energy is 22.9 Me V, which increased significantly than that of a single-laser target interaction. Meanwhile, the average divergence angle(22.3?) is reduced. The dependence of the proton beam on the length of sidewall is investigated in detail and the optimal length is obtained.
