The careers of three Chinese physicists,Hu Ning,Ma Shijun,and Peng Huanwu at the Dublin Institute for Advance Studies in the 1940s,and later,are described.A brief history of the foundation and operations of the instit...The careers of three Chinese physicists,Hu Ning,Ma Shijun,and Peng Huanwu at the Dublin Institute for Advance Studies in the 1940s,and later,are described.A brief history of the foundation and operations of the institute,as well as the roles in it of Erwin Schrodinger,Walter Heitler,Max Born,and others are included.Some details are given of the works carried out there.The three men's post-institute careers are described,Ma eventually in Australia,and Hu and Peng in the People's Republic of China where they became distinguished leaders of theoretical physics research.展开更多
The microstructures and growth process characteristics precipitation-crystallization method were investigated by SEM, TEM of spherical Ni(OH)2 particles synthesized by the aqueous and XRD, and their growth mechanism...The microstructures and growth process characteristics precipitation-crystallization method were investigated by SEM, TEM of spherical Ni(OH)2 particles synthesized by the aqueous and XRD, and their growth mechanism was discussed. With the reaction beginning and continuing, amorphous Ni(OH)2 nano-crystallites grow up to spherical micron-particles with radially arranged crystallites. The nucleation, crystallization and re-crystallization led by Ostwald ripening simultaneously take place through the whole growth processes. With the course from reversible aggregation to irreversible agglomeration, the Ni(OH)2 particles tend to grow according to the template growth model: the growth on the crystallite templates stretching in the radius directions is free and quick, while the growth rate for crystallites in other directions is confined due to lower monomers concentration and tends to dissolve So it is only the radially arranged crystallites that predominate in the particle and lead to characteristic microstructures.展开更多
As a clean and renewable future energy source, hydrogen fuel can be produced via solar water splitting. Two-dimensional (2D) black phosphorene (black-P) can harvest visible light due to the desirable band gap, which p...As a clean and renewable future energy source, hydrogen fuel can be produced via solar water splitting. Two-dimensional (2D) black phosphorene (black-P) can harvest visible light due to the desirable band gap, which promises it as a metal-free photocatalyst. However, black-P can be only used to produce hydrogen since the oxidation potential of water locates lower than the position of the valence band maximum. To improve the photocatalytic performance of black-P, here, using black-P and blue phosphorene (blue-P) monolayers, we propose a 2D van der Waals (vdW) heterojunction. Theoretical results, including the band structures, density of states, Bader charge population, charge density di erence, and optical absorption spectra, clearly reveal that the visible light absorption ability is obviously improved, and the band edge alignment of the proposed vdW heterojunction displays a typical type-II feature to effectively separate the photogenerated carriers. At the same time, the built-in interfacial electric field prevents the electron-hole recombination. These predictions suggest that the examined phosphorene-based vdW heterojunction is an efficient photocatalyst for solar water splitting.展开更多
In this paper we transfer the van der Waerden problem into a problem of solving special systems of equations and give some properties of the solutions for the systems.
Hydrogen-Metal pure at thousand thousandth in ingots is a superconductive metal. The sole "additive" which is bounding to the molecules and to the atoms of Hydrogen is an "inert" gas which is a new isotope of H an...Hydrogen-Metal pure at thousand thousandth in ingots is a superconductive metal. The sole "additive" which is bounding to the molecules and to the atoms of Hydrogen is an "inert" gas which is a new isotope of H and which is as the property of holding them together without modifying their characteristics, which means that the forces of Van der Waals and especially the forces of repulsion annihilate themselves: The molecules do not move apart from each other when pressure is lowering. That is the secret of the production of Hydrogen-Metal stable at High Pressure-Low Pressure and High Temperature 6-Low Temperature. In 2007, at the ICENES 2007 conference, it was supposed to be officially announced the existence of the first two Hydrogen-Metal ingots, pure at thousand thousandth and stable at ambient temperature. If in a certain scientific club this reality was communicated but since the strategic importance of such a discovery in the military as well as the financial domain and considering also its civil application, according to my will, it was not officially publicized until November 2007 at the INCANSE 2007 conference in Bandung.展开更多
The van der Waals force originates from the electromagnetic interaction between quantum fluctuationinduced charges. It is a ubiquitous but subtle force which plays an important role and has a wide range of application...The van der Waals force originates from the electromagnetic interaction between quantum fluctuationinduced charges. It is a ubiquitous but subtle force which plays an important role and has a wide range of applications in surface related phenomena like adhesion, friction,and colloidal stability. Calculating the van der Waals force between closely spaced metallic nanoparticles is very challenging due to the strong concentration of electromagnetic fields at the nanometric gap. Especially, at such a small length scale, the macroscopic description of the dielectric properties no longer suffices. The diffuse nonlocal nature of the induced surface electrons which are smeared out near the boundary has to be considered. Here,we review the recent progress on using three-dimensional transformation optics to study the van der Waals forces between closely spaced nanostructures. Through mapping a seemingly asymmetric system to a more symmetric counterpart, transformation optics enables us to look into the behavior of van der Waals forces at extreme length scales,where the effect of nonlocality is found to dramatically weaken the van der Waals interactions.展开更多
Atomically thin transition-metal dichalcogenide(TMDC) nanostructures are predicted to exhibit novel physical properties that make them attractive candidates for the fabrication of electronic and optoelectronic devices...Atomically thin transition-metal dichalcogenide(TMDC) nanostructures are predicted to exhibit novel physical properties that make them attractive candidates for the fabrication of electronic and optoelectronic devices. However, TMDCs tend to grow in the form of two-dimensional nanoplates(NPs) rather than one-dimensional nanoribbons(NRs) due to their native layered structure. Herein, we have developed a space-confined and substrate-directed chemical vapor deposition strategy for the controllable synthesis of WS2, WSe2, MoSe2, MoS2, WS2(1-x)Se2x NPs and NRs. TMDC NRs with lengths ranging from several micrometers to 100 μm have been obtained and the widths of TMDC NRs can be effectively tuned.Moreover, we found that TMDC NRs show different growth behaviors on van der Waals(vdW) and nonvd W substrates. The micro-nano structures, optical and electronic properties of synthesized TMDC NRs have been systematically investigated. This approach provides a general strategy for controllable synthesis of TMDC NRs, which makes these materials easily accessible as functional building blocks for novel optoelectronic devices.展开更多
High-precision sensing of vectorial forces has broad impact on both fundamental research and technological applications such as the examination of vacuum fluctuations and the detection of surface roughness of nanostru...High-precision sensing of vectorial forces has broad impact on both fundamental research and technological applications such as the examination of vacuum fluctuations and the detection of surface roughness of nanostructures.Recent years have witnessed much progress on sensing alternating electromagnetic forces for the rapidly advancing quantum technology-orders of magnitude improvement has been accomplished on the detection sensitivity with atomic sensors,whereas such high-precision measurements for static electromagnetic forces have rarely been demonstrated.Here,based on quantum atomic matter waves confined by a two-dimensional optical lattice,we perform precision measurement of static electromagnetic forces by imaging coherent wave mechanics in the reciprocal space.The lattice confinement causes a decoupling between real-space and reciprocal dynamics,and provides a rigid coordinate frame for calibrating the wavevector accumulation of the matter wave.With that we achieve a stateof-the-art sensitivity of 2.30(8)×10^(-26) N/√Hz.Long-term stabilities on the order of 10^(-28) N are observed in the two spatial components of a force,which allows probing atomic Van der Waals forces at one millimeter distance.As a further illustrative application,we use our atomic sensor to calibrate the control precision of an alternating electromagnetic force applied in the experiment.Future developments of this method hold promise for delivering unprecedented atom-based quantum force sensing technologies.展开更多
Inspired by the great success of ultrathin two-dimensional(2D)layered crystals,more and more attention is being paid to preparing 2D nanostructures from non-layered materials.They can significantly enrich the 2D mater...Inspired by the great success of ultrathin two-dimensional(2D)layered crystals,more and more attention is being paid to preparing 2D nanostructures from non-layered materials.They can significantly enrich the 2D materials and 2D heterostructures family,extend their application prospects,and bring us distinct properties from their bulk counterparts due to the strong 2D confinement effect.However,the realization of 2D non-layered semiconductors with strong light-harvesting capability and the ability to construct high-performance 2D heterostructures is still a critical challenge.Herein,we successfully synthesized 2D PbSe semiconductors with a large lateral dimension and ultrathin thickness via van der Waals epitaxy.The fabricated 2D PbSe device exhibits good electrical conductivity and superior multi-wavelength photoresponse performance with high responsivity(∼10^(3) A/W)and impressive detectivity(∼2×10^(11) Jones).Furthermore,we demonstrate that 2D PbSe nanosheets can serve as component units for constructing high-performance heterostructure devices.With our strategy,ultrahigh current on/off ratio(∼10^(8))and rectification ratio(∼10^()6),as well as high responsivity(∼3×10^(3) A/W)and detectivity(∼7×10^(12) Jones),can be achieved in PbSe/MoS_(2) back-gated transistors.These results indicate that 2D PbSe nanosheets and their heterostructures have tremendous applications potential in electrical and optoelectronic devices.展开更多
文摘The careers of three Chinese physicists,Hu Ning,Ma Shijun,and Peng Huanwu at the Dublin Institute for Advance Studies in the 1940s,and later,are described.A brief history of the foundation and operations of the institute,as well as the roles in it of Erwin Schrodinger,Walter Heitler,Max Born,and others are included.Some details are given of the works carried out there.The three men's post-institute careers are described,Ma eventually in Australia,and Hu and Peng in the People's Republic of China where they became distinguished leaders of theoretical physics research.
基金Project(50134020) supported by the National Natural Science Foundation of ChinaProject supported by Postdoctoral Fund of Central South University
文摘The microstructures and growth process characteristics precipitation-crystallization method were investigated by SEM, TEM of spherical Ni(OH)2 particles synthesized by the aqueous and XRD, and their growth mechanism was discussed. With the reaction beginning and continuing, amorphous Ni(OH)2 nano-crystallites grow up to spherical micron-particles with radially arranged crystallites. The nucleation, crystallization and re-crystallization led by Ostwald ripening simultaneously take place through the whole growth processes. With the course from reversible aggregation to irreversible agglomeration, the Ni(OH)2 particles tend to grow according to the template growth model: the growth on the crystallite templates stretching in the radius directions is free and quick, while the growth rate for crystallites in other directions is confined due to lower monomers concentration and tends to dissolve So it is only the radially arranged crystallites that predominate in the particle and lead to characteristic microstructures.
基金supported by the National Natural Science Foundation of China (No.21473168 and No.21873088)the Natural Science Foundation of the Anhui Higher Education Institutions (No.KJ2016A144)
文摘As a clean and renewable future energy source, hydrogen fuel can be produced via solar water splitting. Two-dimensional (2D) black phosphorene (black-P) can harvest visible light due to the desirable band gap, which promises it as a metal-free photocatalyst. However, black-P can be only used to produce hydrogen since the oxidation potential of water locates lower than the position of the valence band maximum. To improve the photocatalytic performance of black-P, here, using black-P and blue phosphorene (blue-P) monolayers, we propose a 2D van der Waals (vdW) heterojunction. Theoretical results, including the band structures, density of states, Bader charge population, charge density di erence, and optical absorption spectra, clearly reveal that the visible light absorption ability is obviously improved, and the band edge alignment of the proposed vdW heterojunction displays a typical type-II feature to effectively separate the photogenerated carriers. At the same time, the built-in interfacial electric field prevents the electron-hole recombination. These predictions suggest that the examined phosphorene-based vdW heterojunction is an efficient photocatalyst for solar water splitting.
文摘In this paper we transfer the van der Waerden problem into a problem of solving special systems of equations and give some properties of the solutions for the systems.
文摘Hydrogen-Metal pure at thousand thousandth in ingots is a superconductive metal. The sole "additive" which is bounding to the molecules and to the atoms of Hydrogen is an "inert" gas which is a new isotope of H and which is as the property of holding them together without modifying their characteristics, which means that the forces of Van der Waals and especially the forces of repulsion annihilate themselves: The molecules do not move apart from each other when pressure is lowering. That is the secret of the production of Hydrogen-Metal stable at High Pressure-Low Pressure and High Temperature 6-Low Temperature. In 2007, at the ICENES 2007 conference, it was supposed to be officially announced the existence of the first two Hydrogen-Metal ingots, pure at thousand thousandth and stable at ambient temperature. If in a certain scientific club this reality was communicated but since the strategic importance of such a discovery in the military as well as the financial domain and considering also its civil application, according to my will, it was not officially publicized until November 2007 at the INCANSE 2007 conference in Bandung.
基金partially supported by the Gordon and Betty Moore Foundation (J. B. P.)the Royal Commission for the Exhibition of 1851 (R. Z.)+2 种基金the Leverhulme Trust (Y. L. and J. B. P.)the MOE Ac RF Tier 2 (Y. L.)the Program Grant (11235150003) from NTU-A*STAR Silicon Technologies Centre of Excellence (Y. L.)
文摘The van der Waals force originates from the electromagnetic interaction between quantum fluctuationinduced charges. It is a ubiquitous but subtle force which plays an important role and has a wide range of applications in surface related phenomena like adhesion, friction,and colloidal stability. Calculating the van der Waals force between closely spaced metallic nanoparticles is very challenging due to the strong concentration of electromagnetic fields at the nanometric gap. Especially, at such a small length scale, the macroscopic description of the dielectric properties no longer suffices. The diffuse nonlocal nature of the induced surface electrons which are smeared out near the boundary has to be considered. Here,we review the recent progress on using three-dimensional transformation optics to study the van der Waals forces between closely spaced nanostructures. Through mapping a seemingly asymmetric system to a more symmetric counterpart, transformation optics enables us to look into the behavior of van der Waals forces at extreme length scales,where the effect of nonlocality is found to dramatically weaken the van der Waals interactions.
基金supported by the National Natural Science Foundation of China(11974301,11404274,11574395,11702236,61804050)the support from National Natural Science Foundation of China(21673054 and 11874130)+4 种基金the Science and Technology Project of Hunan Province(2019JJ30021,2018JJ3489)Grant from Education Commission of Hunan Province(18B084)Degree and Postgraduate Education Reform Project of Hunan Province(JG2018B045)the Program for Changjiang Scholars and Innovative Research Team in University(IRT13093)financial support from the research project of National University of Defense Technology(ZK18-03-38)。
文摘Atomically thin transition-metal dichalcogenide(TMDC) nanostructures are predicted to exhibit novel physical properties that make them attractive candidates for the fabrication of electronic and optoelectronic devices. However, TMDCs tend to grow in the form of two-dimensional nanoplates(NPs) rather than one-dimensional nanoribbons(NRs) due to their native layered structure. Herein, we have developed a space-confined and substrate-directed chemical vapor deposition strategy for the controllable synthesis of WS2, WSe2, MoSe2, MoS2, WS2(1-x)Se2x NPs and NRs. TMDC NRs with lengths ranging from several micrometers to 100 μm have been obtained and the widths of TMDC NRs can be effectively tuned.Moreover, we found that TMDC NRs show different growth behaviors on van der Waals(vdW) and nonvd W substrates. The micro-nano structures, optical and electronic properties of synthesized TMDC NRs have been systematically investigated. This approach provides a general strategy for controllable synthesis of TMDC NRs, which makes these materials easily accessible as functional building blocks for novel optoelectronic devices.
基金supported by the National Program on Key Basic Research Project of China (2018YFA0305601, 2021YFA07183012021YFA1400900)+4 种基金the National Natural Science Foundation of China (61727819, 11934002, and 11874073)Shanghai Municipal Science and Technology Major Project (2019SHZDZCX01)the Chinese Academy of Sciences Priority Research Program(XDB35020100)the Science and Technology Major Project of Shanxi (202101030201022)the Space Application System of China Manned Space Program
文摘High-precision sensing of vectorial forces has broad impact on both fundamental research and technological applications such as the examination of vacuum fluctuations and the detection of surface roughness of nanostructures.Recent years have witnessed much progress on sensing alternating electromagnetic forces for the rapidly advancing quantum technology-orders of magnitude improvement has been accomplished on the detection sensitivity with atomic sensors,whereas such high-precision measurements for static electromagnetic forces have rarely been demonstrated.Here,based on quantum atomic matter waves confined by a two-dimensional optical lattice,we perform precision measurement of static electromagnetic forces by imaging coherent wave mechanics in the reciprocal space.The lattice confinement causes a decoupling between real-space and reciprocal dynamics,and provides a rigid coordinate frame for calibrating the wavevector accumulation of the matter wave.With that we achieve a stateof-the-art sensitivity of 2.30(8)×10^(-26) N/√Hz.Long-term stabilities on the order of 10^(-28) N are observed in the two spatial components of a force,which allows probing atomic Van der Waals forces at one millimeter distance.As a further illustrative application,we use our atomic sensor to calibrate the control precision of an alternating electromagnetic force applied in the experiment.Future developments of this method hold promise for delivering unprecedented atom-based quantum force sensing technologies.
基金supported by the National Key R&D Program of China(2018YFA0703700)the National Natural Science Foundation of China(91964203,62104171,62104172,and 62004142)+2 种基金the Natural Science Foundation of Hubei Province(2021CFB037)the Strategic Priority Research Program of Chinese Academy of Sciences(XDB44000000)the Fundamental Research Funds for the Central Universities(2042021kf0067)。
文摘Inspired by the great success of ultrathin two-dimensional(2D)layered crystals,more and more attention is being paid to preparing 2D nanostructures from non-layered materials.They can significantly enrich the 2D materials and 2D heterostructures family,extend their application prospects,and bring us distinct properties from their bulk counterparts due to the strong 2D confinement effect.However,the realization of 2D non-layered semiconductors with strong light-harvesting capability and the ability to construct high-performance 2D heterostructures is still a critical challenge.Herein,we successfully synthesized 2D PbSe semiconductors with a large lateral dimension and ultrathin thickness via van der Waals epitaxy.The fabricated 2D PbSe device exhibits good electrical conductivity and superior multi-wavelength photoresponse performance with high responsivity(∼10^(3) A/W)and impressive detectivity(∼2×10^(11) Jones).Furthermore,we demonstrate that 2D PbSe nanosheets can serve as component units for constructing high-performance heterostructure devices.With our strategy,ultrahigh current on/off ratio(∼10^(8))and rectification ratio(∼10^()6),as well as high responsivity(∼3×10^(3) A/W)and detectivity(∼7×10^(12) Jones),can be achieved in PbSe/MoS_(2) back-gated transistors.These results indicate that 2D PbSe nanosheets and their heterostructures have tremendous applications potential in electrical and optoelectronic devices.