The magnetization reduction of hematite using biomass waste can effectively utilize waste and reduce CO_(2) emission to achieve the goals of carbon peaking and carbon neutrality.The effects of temperatures on suspensi...The magnetization reduction of hematite using biomass waste can effectively utilize waste and reduce CO_(2) emission to achieve the goals of carbon peaking and carbon neutrality.The effects of temperatures on suspension magnetization roasting of hematite using biomass waste for evolved gases have been investigated using TG-FTIR,Py-GC/MS and gas composition analyzer.The mixture reduction process is divided into four stages.In the temperature range of 200-450℃ for mixture,the release of CO_(2),acids,and ketones is dominated in gases products.The yield and concentration of small molecules reducing gases increase when the temperature increases from 450 to 900℃.At 700℃,the volume concentrations of CO,H_(2) and CH_(4) peak at 8.91%,8.90% and 4.91%,respectively.During the suspension magnetization roasting process,an optimal iron concentrate with an iron grade of 70.86%,a recovery of 98.66% and a magnetic conversion of 45.70% is obtained at 700℃.Therefore,the magnetization reduction could react greatly in the temperature range of 600 to 700℃ owing to the suitable reducing gases.This study shows a detail gaseous evolution of roasting temperature and provides a new insight for studying the reduction process of hematite using biomass waste.展开更多
The formation and evolution of secondary minerals during bioleaching of chalcopyrite by thermoacidophilic Archaea Acidianus manzaensis were analyzed by combining synchrotron radiation X-ray diffraction(SR-XRD) and S...The formation and evolution of secondary minerals during bioleaching of chalcopyrite by thermoacidophilic Archaea Acidianus manzaensis were analyzed by combining synchrotron radiation X-ray diffraction(SR-XRD) and S, Fe and Cu Kα X-ray absorption near edge structure(XANES) spectroscopy. Leaching experiment showed that 82.4% of Cu2+ was dissolved by A. manzaensis after 10 d. The surface of chalcopyrite was corroded apparently and covered with leaching products. During bioleaching, the formation and evolution of secondary minerals were as follows: 1) little elemental sulfur, jarosite, bornite and chalcocite were found at days 2 and 4; and 2) bornite and chalcocite disappeared, covellite formed, and jarosite gradually became the main component at days 6 and 10. These results indicated that metal-deficiency sulfides chalcocite and bornite were first formed with a low redox potential value(360-461 m V), and then gradually transformed to covellite with a high redox potential value(461-531 m V).展开更多
Environmental characteristics are often the factors that determine the distribution of species in nature. However, species response vis-A-vis these factors differs. For a better understanding of the phenomenon, we hav...Environmental characteristics are often the factors that determine the distribution of species in nature. However, species response vis-A-vis these factors differs. For a better understanding of the phenomenon, we have conducted this study which consists of following the spatio-temporal evolution of two species of Oribatida (Scheloribates sp. and Galumna sp.). The sites which have been the subject of this study, are situated in different bioclimatic zones presenting a very different climatic, edaphic, nutritional, and altitudinal characteristics. The variability of ecological factors showed that the behavior of two species differs. Indeed, Scheloribates sp. is present in all sites except in Biskra whereas Galumna sp. is present only in sites belonging to humid and sub humid bioclimatic zones. Moreover, Scheloribates sp. appears more tolerant of environmental changes while Galumna sp. is more stringent and its presence is marked only in the sites where ecological conditions are better. Thus, it can be noted that the spatial and temporal distribution of oribatid is not only conditioned solely by environmental factors but also by intrinsic factors specific to each species. The specific behavior of Galumna sp. and the tolerance of Scheloribates sp. are interesting and can be the subject of bioindicator species that can inform us about the changes that effect whether natural or anthropogenic environment.展开更多
基金Project(52022019)supported by the National Natural Science Foundation of China。
文摘The magnetization reduction of hematite using biomass waste can effectively utilize waste and reduce CO_(2) emission to achieve the goals of carbon peaking and carbon neutrality.The effects of temperatures on suspension magnetization roasting of hematite using biomass waste for evolved gases have been investigated using TG-FTIR,Py-GC/MS and gas composition analyzer.The mixture reduction process is divided into four stages.In the temperature range of 200-450℃ for mixture,the release of CO_(2),acids,and ketones is dominated in gases products.The yield and concentration of small molecules reducing gases increase when the temperature increases from 450 to 900℃.At 700℃,the volume concentrations of CO,H_(2) and CH_(4) peak at 8.91%,8.90% and 4.91%,respectively.During the suspension magnetization roasting process,an optimal iron concentrate with an iron grade of 70.86%,a recovery of 98.66% and a magnetic conversion of 45.70% is obtained at 700℃.Therefore,the magnetization reduction could react greatly in the temperature range of 600 to 700℃ owing to the suitable reducing gases.This study shows a detail gaseous evolution of roasting temperature and provides a new insight for studying the reduction process of hematite using biomass waste.
基金Project(U1232103)supported by the Joint Funds of National Natural Science Foundation of China and Large Scientific Facility Foundation of Chinese Academy of SciencesProject(51274257)supported by the National Natural Science Foundation of China+2 种基金Project(CX2014B092)supported by Hunan Provincial Innovation Foundation For Postgraduate,ChinaProject(VR-12419)supported by Beijing Synchrotron Radiation Facility Public User Program,ChinaProjects(13SRBL15U13024,13SRBL14B13023)supported by the Open Funds of Shanghai Synchrotron Radiation Facility,China
文摘The formation and evolution of secondary minerals during bioleaching of chalcopyrite by thermoacidophilic Archaea Acidianus manzaensis were analyzed by combining synchrotron radiation X-ray diffraction(SR-XRD) and S, Fe and Cu Kα X-ray absorption near edge structure(XANES) spectroscopy. Leaching experiment showed that 82.4% of Cu2+ was dissolved by A. manzaensis after 10 d. The surface of chalcopyrite was corroded apparently and covered with leaching products. During bioleaching, the formation and evolution of secondary minerals were as follows: 1) little elemental sulfur, jarosite, bornite and chalcocite were found at days 2 and 4; and 2) bornite and chalcocite disappeared, covellite formed, and jarosite gradually became the main component at days 6 and 10. These results indicated that metal-deficiency sulfides chalcocite and bornite were first formed with a low redox potential value(360-461 m V), and then gradually transformed to covellite with a high redox potential value(461-531 m V).
文摘Environmental characteristics are often the factors that determine the distribution of species in nature. However, species response vis-A-vis these factors differs. For a better understanding of the phenomenon, we have conducted this study which consists of following the spatio-temporal evolution of two species of Oribatida (Scheloribates sp. and Galumna sp.). The sites which have been the subject of this study, are situated in different bioclimatic zones presenting a very different climatic, edaphic, nutritional, and altitudinal characteristics. The variability of ecological factors showed that the behavior of two species differs. Indeed, Scheloribates sp. is present in all sites except in Biskra whereas Galumna sp. is present only in sites belonging to humid and sub humid bioclimatic zones. Moreover, Scheloribates sp. appears more tolerant of environmental changes while Galumna sp. is more stringent and its presence is marked only in the sites where ecological conditions are better. Thus, it can be noted that the spatial and temporal distribution of oribatid is not only conditioned solely by environmental factors but also by intrinsic factors specific to each species. The specific behavior of Galumna sp. and the tolerance of Scheloribates sp. are interesting and can be the subject of bioindicator species that can inform us about the changes that effect whether natural or anthropogenic environment.