Smart flexible electronics with underwater motion detection have become a promising research aspect in intelligent perception.Inspired by the strong adaptability of marine creatures to complex underwater environments,...Smart flexible electronics with underwater motion detection have become a promising research aspect in intelligent perception.Inspired by the strong adaptability of marine creatures to complex underwater environments,conventional biocompatible hydrogels are worth developing into organogels with preferred underwater adhesive properties,hydrophobic and antiswelling performance,and motion perception ability.Herein,a highly sensitive organogel sensor exhibiting good hydrophobicity,electromechanical properties,and adhesion properties was prepared for underwater utilization by regulating the chemical components and internal interactions.The synergistic effect of massive reversible noncovalent bonds ensures the organogel’s excellent underwater adhesion to multifarious substrates.Meanwhile,the interactions of hydrophobic conductive fillers and the dynamic hydrophobic associations in the organogel endow it with satisfactory hydrophobic performance(contact angle of111.8°)and antiswelling property(equilibrium swelling ratio of-31%after 15-day immersion).The fabricated flexible organogel strain sensor exhibits high sensitivity(gauge factor of1.96),ultrafast response rate(79.1 ms),low limit of detection(0.45 Pa),and excellent cyclic stability(1044 tensile cycles followed by 3981 compressive cycles).Results demonstrate the proposed organogel’s precise perception of sophisticated human motions in air and underwater,which expands its application scenarios.展开更多
There has been ongoing keen interest to mold electronic devices into desired shapes and be laid on desired configurable surfaces. In specific, the ability to design materials that can bend, twist, compress and stretch...There has been ongoing keen interest to mold electronic devices into desired shapes and be laid on desired configurable surfaces. In specific, the ability to design materials that can bend, twist, compress and stretch repeatedly, while still able to maintain its full capability as conductors or electrodes, has led to numerous efforts to develop flexible and stretchable (bio)devices that are both technologically challenging and environmentally friendly (e.g. biodegradable). In this review, we highlight several recent significant results that have made impacts toward the field of flexible and stretchable electronics, sensors and power sources.展开更多
The advancement of technology has had a profound impact on all areas of life, with an ever more intimate integration of the digital and biological spheres, but it may also be accompanied by an environmental crisis cau...The advancement of technology has had a profound impact on all areas of life, with an ever more intimate integration of the digital and biological spheres, but it may also be accompanied by an environmental crisis caused by the abuse of large quantities of electronics and petrochemicals.Next-generation "green" electronics or iontronics with high biocompatibility, biodegradation, low cost and mechanical compliance promise to mitigate these adverse effects, but are often limited by the finite choices of materials and strategies.Herein, maltose syrup, a traditional water-dissolvable saccharide food called "JiaoJiao" in Chinese, is engineered to replace unsustainable conductive components of current electronic devices. After churning and pulling with two chopsticks, known as aeration, the aerated maltose syrup has optimized viscoelasticity, mechanical adaptation, robustness,remodeling and self-healing capability, yet with transient behavior. Moreover, the structural and viscoelastic evolution during aeration is also analyzed to maximize the contribution from structures. As a proof-of-concept, a type of "green" skinlike iontronics is prepared, which exhibits reliable strain sensing ability and is subsequently applied for intelligent information encryption and transmission based on a novel concept of sending Morse code. This work greatly extends the current material choice and is expected to shed light on the development of a sustainable future.展开更多
基金supported by the Natural Science Foundation of Jiangsu Province(BK20190688)the Natural Science Foundation of Jiangsu Higher Education Institutions(21KJB430039)Taishan Scholar Construction Special Fund of Shandong Province。
文摘Smart flexible electronics with underwater motion detection have become a promising research aspect in intelligent perception.Inspired by the strong adaptability of marine creatures to complex underwater environments,conventional biocompatible hydrogels are worth developing into organogels with preferred underwater adhesive properties,hydrophobic and antiswelling performance,and motion perception ability.Herein,a highly sensitive organogel sensor exhibiting good hydrophobicity,electromechanical properties,and adhesion properties was prepared for underwater utilization by regulating the chemical components and internal interactions.The synergistic effect of massive reversible noncovalent bonds ensures the organogel’s excellent underwater adhesion to multifarious substrates.Meanwhile,the interactions of hydrophobic conductive fillers and the dynamic hydrophobic associations in the organogel endow it with satisfactory hydrophobic performance(contact angle of111.8°)and antiswelling property(equilibrium swelling ratio of-31%after 15-day immersion).The fabricated flexible organogel strain sensor exhibits high sensitivity(gauge factor of1.96),ultrafast response rate(79.1 ms),low limit of detection(0.45 Pa),and excellent cyclic stability(1044 tensile cycles followed by 3981 compressive cycles).Results demonstrate the proposed organogel’s precise perception of sophisticated human motions in air and underwater,which expands its application scenarios.
基金funding from the Bill and Melinda Gates Foundation Grand Challenge Award (OPP1032970)
文摘There has been ongoing keen interest to mold electronic devices into desired shapes and be laid on desired configurable surfaces. In specific, the ability to design materials that can bend, twist, compress and stretch repeatedly, while still able to maintain its full capability as conductors or electrodes, has led to numerous efforts to develop flexible and stretchable (bio)devices that are both technologically challenging and environmentally friendly (e.g. biodegradable). In this review, we highlight several recent significant results that have made impacts toward the field of flexible and stretchable electronics, sensors and power sources.
基金supported by the National Natural Science Foundation of China (51733003)。
文摘The advancement of technology has had a profound impact on all areas of life, with an ever more intimate integration of the digital and biological spheres, but it may also be accompanied by an environmental crisis caused by the abuse of large quantities of electronics and petrochemicals.Next-generation "green" electronics or iontronics with high biocompatibility, biodegradation, low cost and mechanical compliance promise to mitigate these adverse effects, but are often limited by the finite choices of materials and strategies.Herein, maltose syrup, a traditional water-dissolvable saccharide food called "JiaoJiao" in Chinese, is engineered to replace unsustainable conductive components of current electronic devices. After churning and pulling with two chopsticks, known as aeration, the aerated maltose syrup has optimized viscoelasticity, mechanical adaptation, robustness,remodeling and self-healing capability, yet with transient behavior. Moreover, the structural and viscoelastic evolution during aeration is also analyzed to maximize the contribution from structures. As a proof-of-concept, a type of "green" skinlike iontronics is prepared, which exhibits reliable strain sensing ability and is subsequently applied for intelligent information encryption and transmission based on a novel concept of sending Morse code. This work greatly extends the current material choice and is expected to shed light on the development of a sustainable future.