Ag3PO4 is found to be a highly efficient photocatalyst and receives great attention. The high activity of the photocatalyst is credited to the intrinsic electronic structure. The morphology control and nano-composite ...Ag3PO4 is found to be a highly efficient photocatalyst and receives great attention. The high activity of the photocatalyst is credited to the intrinsic electronic structure. The morphology control and nano-composite fabrication are used to improve the performance and practicability. This paper reviews the structure, properties and some theoretical aspects of Ag3PO4 single crystal. Also, the major strategies, namely the morphology control and hetero-nanostructure construction, as ways to improve the performance of Ag3PO4-based photocatalysts, are summarized with the aid of some typical instances.展开更多
Two homogeneous photoelectrocatalytic systems composed of simple polypyridyl Co complexes[Co(tpy)2](PF6)2and[Co(bpy)3](PF6)2as electrocatalysts and a Si wafer as the photoelectrode were used for combined photoelectroc...Two homogeneous photoelectrocatalytic systems composed of simple polypyridyl Co complexes[Co(tpy)2](PF6)2and[Co(bpy)3](PF6)2as electrocatalysts and a Si wafer as the photoelectrode were used for combined photoelectrochemical reduction of CO2to CO.A high photocurrent density of1.4mA/cm2was observed for the system with the[Co(tpy)2](PF6)2catalyst and a photovoltage of400mV was generated.Faradaic efficiencies of CO were optimized to83%and94%for the[Co(tpy)2](PF6)2and[Co(bpy)3](PF6)2complexes,respectively,in acetonitrile solution with10%methanol(volume fraction,same below)as a protic additive.Addition of2%water volume fraction induced a large amount of non‐specific H2evolution by the Si photoelectrode.展开更多
This paper presents a novel remote controlled dexterous robot arm with 6 degrees of freedom (DOF). As a highly integrated mechatronics system, sensors and their signal processing system are integrated inside each jo...This paper presents a novel remote controlled dexterous robot arm with 6 degrees of freedom (DOF). As a highly integrated mechatronics system, sensors and their signal processing system are integrated inside each joint. To lighten the weight, almost all mechanical parts are made of aluminum and the robot control system is placed outside. The modular concept is adopted during the robot design process for time and cost saving. Considering the much greater torque acted on the two shoulder joints, the joint shells are strengthened in the design to increase joint stiffness and suppress system vibration. Meanwhile, to simplify the maintenance, a new spring pins electronic connector is designed to disassemble every joint, connector and link independently without cutting any cables. The teleoperation technology enables the robot to offer more convenient service definitely for people' s daily life. Virtual reality technology is used to solve the time delay problem during teleoperation. Finally, two typical daily chore experiments are implemented to prove the manipulation ability of the dexterous robot arm.展开更多
文摘Ag3PO4 is found to be a highly efficient photocatalyst and receives great attention. The high activity of the photocatalyst is credited to the intrinsic electronic structure. The morphology control and nano-composite fabrication are used to improve the performance and practicability. This paper reviews the structure, properties and some theoretical aspects of Ag3PO4 single crystal. Also, the major strategies, namely the morphology control and hetero-nanostructure construction, as ways to improve the performance of Ag3PO4-based photocatalysts, are summarized with the aid of some typical instances.
基金supported by the National Key R&D Program of China (2016YFB0600901)the Strategic Priority Research Program of the Chinese Academy of Sciences (XDB17030300)~~
文摘Two homogeneous photoelectrocatalytic systems composed of simple polypyridyl Co complexes[Co(tpy)2](PF6)2and[Co(bpy)3](PF6)2as electrocatalysts and a Si wafer as the photoelectrode were used for combined photoelectrochemical reduction of CO2to CO.A high photocurrent density of1.4mA/cm2was observed for the system with the[Co(tpy)2](PF6)2catalyst and a photovoltage of400mV was generated.Faradaic efficiencies of CO were optimized to83%and94%for the[Co(tpy)2](PF6)2and[Co(bpy)3](PF6)2complexes,respectively,in acetonitrile solution with10%methanol(volume fraction,same below)as a protic additive.Addition of2%water volume fraction induced a large amount of non‐specific H2evolution by the Si photoelectrode.
文摘This paper presents a novel remote controlled dexterous robot arm with 6 degrees of freedom (DOF). As a highly integrated mechatronics system, sensors and their signal processing system are integrated inside each joint. To lighten the weight, almost all mechanical parts are made of aluminum and the robot control system is placed outside. The modular concept is adopted during the robot design process for time and cost saving. Considering the much greater torque acted on the two shoulder joints, the joint shells are strengthened in the design to increase joint stiffness and suppress system vibration. Meanwhile, to simplify the maintenance, a new spring pins electronic connector is designed to disassemble every joint, connector and link independently without cutting any cables. The teleoperation technology enables the robot to offer more convenient service definitely for people' s daily life. Virtual reality technology is used to solve the time delay problem during teleoperation. Finally, two typical daily chore experiments are implemented to prove the manipulation ability of the dexterous robot arm.