In order to recognize one's intention from the communication, both the meaning and the emotion are necessary to be interpreted correctly. But until now the study of fine-grained theory of emotion is still full of cha...In order to recognize one's intention from the communication, both the meaning and the emotion are necessary to be interpreted correctly. But until now the study of fine-grained theory of emotion is still full of challenges. This paper analy- zes emotion category according to the statistics of Affective Word (AW) hierarchy and descries an e- motion ontology from Chinese knowledge resource semi-automatically created for human machine in- teraction. The emotion hierarchy is called complex emotion. Firstly, over 7 000 AWs have been annota- ted and theft detailed explanations had been collected for an affective lexicon and then the consistent rela- tionships are automatically parsed and a serial of e- motion hierarchical structures are built up. More than 50 affective categories are extracted by a lexical clustering algorithm and about 5 000 nouns and ad- jectives and 2 000 verbs are categorized into the predicate hierarchy. The results have been evaluated to be valid by two metrics.展开更多
In this work grand canonical Monte Carlo simulations were performed to study gas separation in three pairs of isoreticular metal-organic frameworks (IRMOFs) with and without catenation at room temperature.Mixture comp...In this work grand canonical Monte Carlo simulations were performed to study gas separation in three pairs of isoreticular metal-organic frameworks (IRMOFs) with and without catenation at room temperature.Mixture composed of CO2 and H2 was selected as the model system to separate.The results show that CO2 selectivity in catenated MOFs with multi-porous frameworks is much higher than their non-catenated counterparts.The simulations also show that the electrostatic interactions are very important for the selectivity,and the contributions of different electrostatic interactions are different,depending on pore size,pressure and mixture composition.In fact,changing the electrostatic interactions can even qualitatively change the adsorption behavior.A general conclusion is that the electrostatic interactions between adsorbate molecules and the framework atoms play a dominant role at low pressures,and these interactions in catenated MOFs have much more pronounced effects than those in their non-catenated counterparts,while the electrostatic interactions between adsorbate molecules become evident with increasing pressure,and eventually dominant.展开更多
We report a theoretic study on modulating the spin polarization of charge current in a mesoscopic fourterminal device of cross structure by using the inverse spin hall effect. The scattering region of device is a two-...We report a theoretic study on modulating the spin polarization of charge current in a mesoscopic fourterminal device of cross structure by using the inverse spin hall effect. The scattering region of device is a two-dimensional electron gas (2DEG) with Rashba spin orbital interaction (RSOI), one of lead is ferromagnetic metal and other three leads are spin-degenerate normal metals. By using Landauer-Biittiker formalism, we found that when a longitudinal charge current flows through 2DEG scattering region from FM lead by external bias, the transverse current can be either a pure spin current or full-polarized charge current due to the combined effect of spin hall effect and its inverse process, and the polarization of this transverse current can be easily controlled by several device parameters such as the Fermi energy, ferromagnetic magnetization, and the RSOI constant. Our method may pave a new way to control the spin polarization of a charge current.展开更多
Electrochemical reductive exfoliation of graphite to few layered graphene(FLG) in presence of 1-ethyl-2,3-dimethyl imidazolium bis(trifluoromethylsulfonyl) imide ionic liquid and redox ionic liquid based ferrocene has...Electrochemical reductive exfoliation of graphite to few layered graphene(FLG) in presence of 1-ethyl-2,3-dimethyl imidazolium bis(trifluoromethylsulfonyl) imide ionic liquid and redox ionic liquid based ferrocene has been investigated. Thus, by applying a mild negative potential(-2.7 V vs. Fc/Fc^+) to carbon electrode in ionic liquid graphene flakes could be generated. The generated materials have been characterized by X-ray photoelectron spectroscopy, Raman spectroscopy, high resolution transmission electron microscopy and atomic force microscopy. XPS and Raman analysis show that the electrochemical reductive exfoliation provides the formation of FLG. The thickness of the resulting FLG was found to be ranged between 4 and1 nm. HR-TEM images reveal the formation of few graphene layers and in some cases single graphene layer was observed.Moreover, this electrochemical route conduces to the formation of ionic liquid functionalized FLG. Finally, the reductive exfoliation was further investigated in the presence of redox ionic liquid. XPS and electrochemical measurements confirm the presence of ferrocene.展开更多
This paper presents suggestions in aspects(which should meet the standards) such as alarm indication, system setup and system security during the designing process of alarm system in medical electrical equipment, whic...This paper presents suggestions in aspects(which should meet the standards) such as alarm indication, system setup and system security during the designing process of alarm system in medical electrical equipment, which can be used as a reference for manufacturers.展开更多
基金supported by the Ministry of Education,Science,Sports and Culture,Grant-in-Aid for Scientific Research under Grant No.22240021the Grant-in-Aid for Challenging Exploratory Research under Grant No.21650030
文摘In order to recognize one's intention from the communication, both the meaning and the emotion are necessary to be interpreted correctly. But until now the study of fine-grained theory of emotion is still full of challenges. This paper analy- zes emotion category according to the statistics of Affective Word (AW) hierarchy and descries an e- motion ontology from Chinese knowledge resource semi-automatically created for human machine in- teraction. The emotion hierarchy is called complex emotion. Firstly, over 7 000 AWs have been annota- ted and theft detailed explanations had been collected for an affective lexicon and then the consistent rela- tionships are automatically parsed and a serial of e- motion hierarchical structures are built up. More than 50 affective categories are extracted by a lexical clustering algorithm and about 5 000 nouns and ad- jectives and 2 000 verbs are categorized into the predicate hierarchy. The results have been evaluated to be valid by two metrics.
基金Supported by the National Natural Science Foundation of China (20725622, 20706002, and 20876006), Beijing Nova Program (2008B15) and the Dutch STW/CW Separation Technology Program (700.56.655-DPC.6243).
文摘In this work grand canonical Monte Carlo simulations were performed to study gas separation in three pairs of isoreticular metal-organic frameworks (IRMOFs) with and without catenation at room temperature.Mixture composed of CO2 and H2 was selected as the model system to separate.The results show that CO2 selectivity in catenated MOFs with multi-porous frameworks is much higher than their non-catenated counterparts.The simulations also show that the electrostatic interactions are very important for the selectivity,and the contributions of different electrostatic interactions are different,depending on pore size,pressure and mixture composition.In fact,changing the electrostatic interactions can even qualitatively change the adsorption behavior.A general conclusion is that the electrostatic interactions between adsorbate molecules and the framework atoms play a dominant role at low pressures,and these interactions in catenated MOFs have much more pronounced effects than those in their non-catenated counterparts,while the electrostatic interactions between adsorbate molecules become evident with increasing pressure,and eventually dominant.
基金Supported by National Natural Science Foundation of China under Grant No.10704016Natural Science Foundation of Jiangsu Province under Grant Nos.BK2007100Ministry of Education of China under Grant No.MEC-20070286036
文摘We report a theoretic study on modulating the spin polarization of charge current in a mesoscopic fourterminal device of cross structure by using the inverse spin hall effect. The scattering region of device is a two-dimensional electron gas (2DEG) with Rashba spin orbital interaction (RSOI), one of lead is ferromagnetic metal and other three leads are spin-degenerate normal metals. By using Landauer-Biittiker formalism, we found that when a longitudinal charge current flows through 2DEG scattering region from FM lead by external bias, the transverse current can be either a pure spin current or full-polarized charge current due to the combined effect of spin hall effect and its inverse process, and the polarization of this transverse current can be easily controlled by several device parameters such as the Fermi energy, ferromagnetic magnetization, and the RSOI constant. Our method may pave a new way to control the spin polarization of a charge current.
基金supported by the European Community Seventh Framework Programme(266391)
文摘Electrochemical reductive exfoliation of graphite to few layered graphene(FLG) in presence of 1-ethyl-2,3-dimethyl imidazolium bis(trifluoromethylsulfonyl) imide ionic liquid and redox ionic liquid based ferrocene has been investigated. Thus, by applying a mild negative potential(-2.7 V vs. Fc/Fc^+) to carbon electrode in ionic liquid graphene flakes could be generated. The generated materials have been characterized by X-ray photoelectron spectroscopy, Raman spectroscopy, high resolution transmission electron microscopy and atomic force microscopy. XPS and Raman analysis show that the electrochemical reductive exfoliation provides the formation of FLG. The thickness of the resulting FLG was found to be ranged between 4 and1 nm. HR-TEM images reveal the formation of few graphene layers and in some cases single graphene layer was observed.Moreover, this electrochemical route conduces to the formation of ionic liquid functionalized FLG. Finally, the reductive exfoliation was further investigated in the presence of redox ionic liquid. XPS and electrochemical measurements confirm the presence of ferrocene.
文摘This paper presents suggestions in aspects(which should meet the standards) such as alarm indication, system setup and system security during the designing process of alarm system in medical electrical equipment, which can be used as a reference for manufacturers.