The spatial distributions and interannual variations of aerosol concentrations, aerosol optical depth （AOD）, aerosol direct radiative forcings, and their responses to heterogeneous reactions on dust surfaces over Ea...The spatial distributions and interannual variations of aerosol concentrations, aerosol optical depth （AOD）, aerosol direct radiative forcings, and their responses to heterogeneous reactions on dust surfaces over East Asia in March 2006-10 were investigated by utilizing a regional coupled climate-chemistry/aerosol model. Anthropogenic aerosol concentrations （inorganic ＋ carbonaceous） were higher in March 2006 and 2008, whereas soil dust reached its highest levels in March 2006 and 2010, resulting in stronger aerosol radiative forcings in these periods. The domain and five-year （2006-10） monthly mean concentrations of anthropogenic and dust aerosols, AOD, and radiative forcings at the surface （SURF） and at the top of the atmosphere （TOA） in March were 2.4 μg m 3 13.1 lag m^-3, 0.18, -19.0 W m^-2, and -7.4 W m^-2, respectively. Heterogeneous reactions led to an increase of total inorganic aerosol concentration; however, the ambient inorganic aerosol concentration decreased, resulting in a smaller AOD and weaker aerosol radiative forcings. In March 2006 and 2010, the changes in ambient inorganic aerosols, AOD, and aerosol radiative forcings were more evident. In terms of the domain and five-year averages, the total inorganic aerosol concentrations increased by 13.7% （0.17 μg m^-3） due to heterogeneous reactions, but the ambient inorganic aerosol concentrations were reduced by 10.5% （0.13 lag m-3）. As a result, the changes in AOD, SURF and TOA radiative forcings were estimated to be -3.9% （-0.007）, -1.7% （0.34 W m^-2）, and -4.3% （0.34 W m^-2）, respectively, in March over East Asia.展开更多
The thermodynamic state of the tropical atmosphere plays an important role in the development of tropical cyclone(TC)intensity.This study reports new results that demonstrate a negative association between eastern Pac...The thermodynamic state of the tropical atmosphere plays an important role in the development of tropical cyclone(TC)intensity.This study reports new results that demonstrate a negative association between eastern Pacific TC intensity in offshore regions and dust aerosol optical depth(AOD)for the years 1980–2019.At the same time,a negative response of cloud water in the lower troposphere to dust AOD is reported by analyzing MERRA-2 reanalysis data and GCM simulations from CMIP6.This response can be explained by the dust semi-direct effect,in which dust aerosols absorb solar radiation,promoting the evaporation of clouds.In principle,this aerosol-driven vaporization modification could affect the enthalpy of the air surrounding a TC.Using potential intensity theory,the authors demonstrate that change in TC intensity related to dust AOD conditions is a consequence of the anomalous enthalpy of the air surrounding a TC caused by the dust semi-direct effect.展开更多
The air quality modeling system RAMS (Regional Atmospheric Modeling System)-CMAQ (Models-3 Community Multi-scale Air Quality) is developed to simulate the aerosol optical depth (AOD) and aerosol direct forcing (DF). T...The air quality modeling system RAMS (Regional Atmospheric Modeling System)-CMAQ (Models-3 Community Multi-scale Air Quality) is developed to simulate the aerosol optical depth (AOD) and aerosol direct forcing (DF). The aerosol-specific extinction, single scattering albedo, and asymmetry factor are parameterized based on Mie theory taking into account the aerosol size distribution, composition, refractive index, and water uptake of solution particles. A two-stream solar radiative model considers all gaseous molecular absorption, Rayleigh scattering, and aerosols and clouds. RAMSCMAQ is applied to simulate all major aerosol concentrations (e.g., sulfate, nitrate, ammonium, organic carbon, black carbon, fine soil, and sea salt) and AOD and DF over East Asia in 2005. To evaluate its performance, the simulated AOD values were compared with ground-based in situ measurements. The comparison shows that RAMSCMAQ performed well in most of the model domain and generally captured the observed variations. High AOD values (0.2 1.0) mainly appear in the Sichuan Basin as well as in central and southeastern China. The geographic distribution of DF generally follows the AOD distribution patterns, and the DF at the top-of-the-atmosphere is less than 25 and 20 W m 2 in clear-sky and all-sky over the Sichuan Basin. Both AOD and DF exhibit seasonal variations with lower values in July and higher ones in January The DF could obviously be impacted by high cloud fractions.展开更多
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences(Grant No. KZCX2-YW-Q11-03)the National Basic Research Program of China(Grant No.2010CB950804)100 Talents Program of the Chinese Academy of Sciences
文摘The spatial distributions and interannual variations of aerosol concentrations, aerosol optical depth （AOD）, aerosol direct radiative forcings, and their responses to heterogeneous reactions on dust surfaces over East Asia in March 2006-10 were investigated by utilizing a regional coupled climate-chemistry/aerosol model. Anthropogenic aerosol concentrations （inorganic ＋ carbonaceous） were higher in March 2006 and 2008, whereas soil dust reached its highest levels in March 2006 and 2010, resulting in stronger aerosol radiative forcings in these periods. The domain and five-year （2006-10） monthly mean concentrations of anthropogenic and dust aerosols, AOD, and radiative forcings at the surface （SURF） and at the top of the atmosphere （TOA） in March were 2.4 μg m 3 13.1 lag m^-3, 0.18, -19.0 W m^-2, and -7.4 W m^-2, respectively. Heterogeneous reactions led to an increase of total inorganic aerosol concentration; however, the ambient inorganic aerosol concentration decreased, resulting in a smaller AOD and weaker aerosol radiative forcings. In March 2006 and 2010, the changes in ambient inorganic aerosols, AOD, and aerosol radiative forcings were more evident. In terms of the domain and five-year averages, the total inorganic aerosol concentrations increased by 13.7% （0.17 μg m^-3） due to heterogeneous reactions, but the ambient inorganic aerosol concentrations were reduced by 10.5% （0.13 lag m-3）. As a result, the changes in AOD, SURF and TOA radiative forcings were estimated to be -3.9% （-0.007）, -1.7% （0.34 W m^-2）, and -4.3% （0.34 W m^-2）, respectively, in March over East Asia.
基金This work was supported by National Natural Science Foundation of China[grant numbers 41675062 and 41375096]the Research Grants Council of the Hong Kong Special Administrative Region,China[project numbers CityU 11306417 and 11335316].
文摘The thermodynamic state of the tropical atmosphere plays an important role in the development of tropical cyclone(TC)intensity.This study reports new results that demonstrate a negative association between eastern Pacific TC intensity in offshore regions and dust aerosol optical depth(AOD)for the years 1980–2019.At the same time,a negative response of cloud water in the lower troposphere to dust AOD is reported by analyzing MERRA-2 reanalysis data and GCM simulations from CMIP6.This response can be explained by the dust semi-direct effect,in which dust aerosols absorb solar radiation,promoting the evaporation of clouds.In principle,this aerosol-driven vaporization modification could affect the enthalpy of the air surrounding a TC.Using potential intensity theory,the authors demonstrate that change in TC intensity related to dust AOD conditions is a consequence of the anomalous enthalpy of the air surrounding a TC caused by the dust semi-direct effect.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (KZCX2-YW-Q11-04)the National Basic research Program of China (2006CB403702 and 2007CB407303)
文摘The air quality modeling system RAMS (Regional Atmospheric Modeling System)-CMAQ (Models-3 Community Multi-scale Air Quality) is developed to simulate the aerosol optical depth (AOD) and aerosol direct forcing (DF). The aerosol-specific extinction, single scattering albedo, and asymmetry factor are parameterized based on Mie theory taking into account the aerosol size distribution, composition, refractive index, and water uptake of solution particles. A two-stream solar radiative model considers all gaseous molecular absorption, Rayleigh scattering, and aerosols and clouds. RAMSCMAQ is applied to simulate all major aerosol concentrations (e.g., sulfate, nitrate, ammonium, organic carbon, black carbon, fine soil, and sea salt) and AOD and DF over East Asia in 2005. To evaluate its performance, the simulated AOD values were compared with ground-based in situ measurements. The comparison shows that RAMSCMAQ performed well in most of the model domain and generally captured the observed variations. High AOD values (0.2 1.0) mainly appear in the Sichuan Basin as well as in central and southeastern China. The geographic distribution of DF generally follows the AOD distribution patterns, and the DF at the top-of-the-atmosphere is less than 25 and 20 W m 2 in clear-sky and all-sky over the Sichuan Basin. Both AOD and DF exhibit seasonal variations with lower values in July and higher ones in January The DF could obviously be impacted by high cloud fractions.
