To obtain carbon dioxide （CO2） flux between water-air interface of Taihu lake, monthly water samplers at 14 sites and the local meteorological data of the lake were collected and analyzed in 1998. Carbon dioxide par...To obtain carbon dioxide （CO2） flux between water-air interface of Taihu lake, monthly water samplers at 14 sites and the local meteorological data of the lake were collected and analyzed in 1998. Carbon dioxide partial pressures （pCO2） at air-water interface in the lake were calculated using alkalinity, pH, ionic strength, active coefficient, and water temperature. The carbon fluxes at different sublakes and areas were estimated by concentration gradient between water and air in consideration of Schmidt numbers of 600 and daily mean windspeed at 10 m above water surface. The results indicated that the mean values of pCO2 in Wuli Lake,Meiliang Bay, hydrophyte area, west littoral zone, riverine mouths, and the open lake areas were 1 807.8±1 071.4（mean±standard deviation）μatm （latm=1.013 25×10^5pa）, 416.3±217.0μatm, 576.5±758.8μatm, 304.2±9.43.5μatm, 1 933.6±1 144.7 μatm, and 448.5±202.6μatm, respectively. Maximum and minimum pCO2 values were found in the hypertrophic （4 053.7μatm） and the eutrophic （3.2 μatm） areas. The riverine mouth areas have the maximum fluxes （82.0±62.8 mmol/m^2a）. But there was no significant difference between eutrophic and mesotrophic areas in pCO2 and the flux of CO2. The hydrophyte area, however, has the minimum （--0.58±12.9mmol/m^2a）. In respect to CO2 equilibrium, input of the rivers will obviously influence inorganic carbon distribution in the riverine estuary. For example, the annual mean CO2 flux in Zhihugang River estuary was 19 times of that in Meiliang Bay, although the former is only a part of the latter. The sites in the body of the lake show a clear seasonal cycle with pCO2 higher than atmospheric equilibrium in winter, and much lower than atmospheric in summer due to CO2 consumption by photosynthesis. The CO2 amount of the net annual evasion that enters the atmosphere is 28.42×10^4 t/a, of which those from the west littoral zone and the open lake account for 53.8% and 36.7%, respectively.展开更多
To clarify temporal changes in the transboundary pollution, we analyzed SCPs （spheroidal carbonaceous particles） in bottom sediments of lakes in China, South Korea and Japan. SCPs provide an unambiguous record of an...To clarify temporal changes in the transboundary pollution, we analyzed SCPs （spheroidal carbonaceous particles） in bottom sediments of lakes in China, South Korea and Japan. SCPs provide an unambiguous record of anthropogenic atmospheric pollution in bottom sediments. Recently deposited SCPs in air and unmelted snow on Mt. Fuji were also characterized. The concentrarion and characteristics of SCPs reflected the environmental and industrial history of the area. Evidence of transboundary air pollution was observed after the 1980s in Yashagaike and Kotaniike ponds in Japan, which are located on the coast of the Sea of Japan. The concentration suggests that the pollutants originated from continental Asia, particularly after the 1980s. The chemical composition of the SCPs allowed the source of emissions to be identified. Chinese SCPs were found at Yashagaike and Kotaniike ponds in Japan, and at Songiiho and Urimji lakes in Korea. The size distributions showed that small SCPs are transported over long distances. On the summit of Mr. Fuji, SCPs transported by the prevailing westerlies from China were found in addition to SCPs emitted in Japan.展开更多
基金This research was supported by the Knowledge Innovation Project of Chinese Academy of Sciences (KZCX1-SW-01-15) and (KZCX1- SW-12)
文摘To obtain carbon dioxide （CO2） flux between water-air interface of Taihu lake, monthly water samplers at 14 sites and the local meteorological data of the lake were collected and analyzed in 1998. Carbon dioxide partial pressures （pCO2） at air-water interface in the lake were calculated using alkalinity, pH, ionic strength, active coefficient, and water temperature. The carbon fluxes at different sublakes and areas were estimated by concentration gradient between water and air in consideration of Schmidt numbers of 600 and daily mean windspeed at 10 m above water surface. The results indicated that the mean values of pCO2 in Wuli Lake,Meiliang Bay, hydrophyte area, west littoral zone, riverine mouths, and the open lake areas were 1 807.8±1 071.4（mean±standard deviation）μatm （latm=1.013 25×10^5pa）, 416.3±217.0μatm, 576.5±758.8μatm, 304.2±9.43.5μatm, 1 933.6±1 144.7 μatm, and 448.5±202.6μatm, respectively. Maximum and minimum pCO2 values were found in the hypertrophic （4 053.7μatm） and the eutrophic （3.2 μatm） areas. The riverine mouth areas have the maximum fluxes （82.0±62.8 mmol/m^2a）. But there was no significant difference between eutrophic and mesotrophic areas in pCO2 and the flux of CO2. The hydrophyte area, however, has the minimum （--0.58±12.9mmol/m^2a）. In respect to CO2 equilibrium, input of the rivers will obviously influence inorganic carbon distribution in the riverine estuary. For example, the annual mean CO2 flux in Zhihugang River estuary was 19 times of that in Meiliang Bay, although the former is only a part of the latter. The sites in the body of the lake show a clear seasonal cycle with pCO2 higher than atmospheric equilibrium in winter, and much lower than atmospheric in summer due to CO2 consumption by photosynthesis. The CO2 amount of the net annual evasion that enters the atmosphere is 28.42×10^4 t/a, of which those from the west littoral zone and the open lake account for 53.8% and 36.7%, respectively.
文摘To clarify temporal changes in the transboundary pollution, we analyzed SCPs （spheroidal carbonaceous particles） in bottom sediments of lakes in China, South Korea and Japan. SCPs provide an unambiguous record of anthropogenic atmospheric pollution in bottom sediments. Recently deposited SCPs in air and unmelted snow on Mt. Fuji were also characterized. The concentrarion and characteristics of SCPs reflected the environmental and industrial history of the area. Evidence of transboundary air pollution was observed after the 1980s in Yashagaike and Kotaniike ponds in Japan, which are located on the coast of the Sea of Japan. The concentration suggests that the pollutants originated from continental Asia, particularly after the 1980s. The chemical composition of the SCPs allowed the source of emissions to be identified. Chinese SCPs were found at Yashagaike and Kotaniike ponds in Japan, and at Songiiho and Urimji lakes in Korea. The size distributions showed that small SCPs are transported over long distances. On the summit of Mr. Fuji, SCPs transported by the prevailing westerlies from China were found in addition to SCPs emitted in Japan.
