The photodissociation of NO+ at c3∏(v′=0) state is studied by threshold photoelectron- photoion coincidence imaging method. By some assumptions, the relations between velocity in center of mass (CM) coordinates...The photodissociation of NO+ at c3∏(v′=0) state is studied by threshold photoelectron- photoion coincidence imaging method. By some assumptions, the relations between velocity in center of mass (CM) coordinates and most probable center of mass (MPCM) coordinates, time of flight and displacement in the velocity map image of fragment ions are derived using vector addition of velocity and displacement on the condition of perpendicular molecular beam. Using these relations the velocity in CM coordinates, the velocity and angular distri- bution of N+ fragment ions in MPCM coordinates are obtained and discussed, respectively.展开更多
Threshold photoelectron-photoion coincidence (TPEPICO) is a powerful method to prepare and analyze internal energy- or state-selected ions. Here, we review the state-of-the-art TPEPICO imaging technique combining with...Threshold photoelectron-photoion coincidence (TPEPICO) is a powerful method to prepare and analyze internal energy- or state-selected ions. Here, we review the state-of-the-art TPEPICO imaging technique combining with tunable vacuum ultraviolet (VUV) synchrotron radiation and its recent applications at Hefei Light Source (HLS), especially on the fundamental data measurement and the dissociation dynamics of ions. By applying the double velocity map imaging for both electrons and ions in coincidence, the collection efficiency of the charged particles, the electron energy resolution and the resolving power of the released kinetic energy in dissociation have been greatly improved. The kinetic energy and the angular distributions of fragment ions dissociated from parent ions with definitive internal energy or state have been acquired directly from TPEPICO images. Some dissociation mechanisms involving non-adiabatic quantum effects, like conical intersection and internal conversion, have been revealed. Moreover, the mass-selected threshold photoelectron spectroscopy (MS-TPES) shows tremendous advantages in isomer-specific analysis of complex systems.展开更多
The class of bi-directional optimal velocity models can describe the bi-directional looking effect that usually exists in the reality and is even enhanced with the development of the connected vehicle technologies. It...The class of bi-directional optimal velocity models can describe the bi-directional looking effect that usually exists in the reality and is even enhanced with the development of the connected vehicle technologies. Its combined string stability condition can be obtained through the method of the ring-road based string stability analysis. However, the partial string stability about traffic fluctuation propagated backward or forward was neglected, which will be analyzed in detail in this work by the method of transfer function and its H∞ norm from the viewpoint of control theory. Then, through comparing the conditions of combined and partial string stabilities, their relationships can make traffic flow be divided into three distinguishable regions, displaying various combined and partial string stability performance. Finally, the numerical experiments verify the theoretical results and find that the final displaying string stability or instability performance results from the accumulated and offset effects of traffic fluctuations propagated from different directions.展开更多
Combining Adomian decomposition method (ADM) with Pade approximants, we solve two differentiaidifference equations (DDEs): the relativistic Toda lattice equation and the modified Volterra lattice equation. With t...Combining Adomian decomposition method (ADM) with Pade approximants, we solve two differentiaidifference equations (DDEs): the relativistic Toda lattice equation and the modified Volterra lattice equation. With the help of symbolic computation Maple, the results obtained by ADM-Pade technique are compared with those obtained by using ADM alone. The numerical results demonstrate that ADM-Pade technique give the approximate solution with faster convergence rate and higher accuracy and relative in larger domain of convergence than using ADM.展开更多
文摘The photodissociation of NO+ at c3∏(v′=0) state is studied by threshold photoelectron- photoion coincidence imaging method. By some assumptions, the relations between velocity in center of mass (CM) coordinates and most probable center of mass (MPCM) coordinates, time of flight and displacement in the velocity map image of fragment ions are derived using vector addition of velocity and displacement on the condition of perpendicular molecular beam. Using these relations the velocity in CM coordinates, the velocity and angular distri- bution of N+ fragment ions in MPCM coordinates are obtained and discussed, respectively.
基金supported by the Instrument Developing Project of the Chinese Academy of Sciences (No.YZ200763)the National Natural Science Foundation of China (No.21027005, No.21573210 and No.21873089)+2 种基金the National Key Research and Development program (No.2016YFF0200502)the National Key Basic Research Foundation (No.2013CB834602)the Chinese Postdoctoral Foundation (No.2018M632535)
文摘Threshold photoelectron-photoion coincidence (TPEPICO) is a powerful method to prepare and analyze internal energy- or state-selected ions. Here, we review the state-of-the-art TPEPICO imaging technique combining with tunable vacuum ultraviolet (VUV) synchrotron radiation and its recent applications at Hefei Light Source (HLS), especially on the fundamental data measurement and the dissociation dynamics of ions. By applying the double velocity map imaging for both electrons and ions in coincidence, the collection efficiency of the charged particles, the electron energy resolution and the resolving power of the released kinetic energy in dissociation have been greatly improved. The kinetic energy and the angular distributions of fragment ions dissociated from parent ions with definitive internal energy or state have been acquired directly from TPEPICO images. Some dissociation mechanisms involving non-adiabatic quantum effects, like conical intersection and internal conversion, have been revealed. Moreover, the mass-selected threshold photoelectron spectroscopy (MS-TPES) shows tremendous advantages in isomer-specific analysis of complex systems.
基金Projects(51108465,71371192)supported by the National Natural Science Foundation of ChinaProject(2014M552165)supported by China Postdoctoral Science FoundationProject(20113187851460)supported by Technology Project of the Ministry of Transport of China
文摘The class of bi-directional optimal velocity models can describe the bi-directional looking effect that usually exists in the reality and is even enhanced with the development of the connected vehicle technologies. Its combined string stability condition can be obtained through the method of the ring-road based string stability analysis. However, the partial string stability about traffic fluctuation propagated backward or forward was neglected, which will be analyzed in detail in this work by the method of transfer function and its H∞ norm from the viewpoint of control theory. Then, through comparing the conditions of combined and partial string stabilities, their relationships can make traffic flow be divided into three distinguishable regions, displaying various combined and partial string stability performance. Finally, the numerical experiments verify the theoretical results and find that the final displaying string stability or instability performance results from the accumulated and offset effects of traffic fluctuations propagated from different directions.
基金supported by the National Natural Science Foundation of China under Grant No. 10735030Shanghai Leading Academic Discipline Project under Grant No. B412Program for Changjiang Scholars and Innovative Research Team in University under Grant No. IRT0734
文摘Combining Adomian decomposition method (ADM) with Pade approximants, we solve two differentiaidifference equations (DDEs): the relativistic Toda lattice equation and the modified Volterra lattice equation. With the help of symbolic computation Maple, the results obtained by ADM-Pade technique are compared with those obtained by using ADM alone. The numerical results demonstrate that ADM-Pade technique give the approximate solution with faster convergence rate and higher accuracy and relative in larger domain of convergence than using ADM.