The synergistic effect of high voltage discharge non‐thermal plasma(NTP)and photocatalysts on contaminant removal has repeatedly confirmed by plenty of researches.Most previous plasma‐photocatalyst synergistic syste...The synergistic effect of high voltage discharge non‐thermal plasma(NTP)and photocatalysts on contaminant removal has repeatedly confirmed by plenty of researches.Most previous plasma‐photocatalyst synergistic systems focused on the utilization of the ultraviolet light but ignored the visible light generated by high voltage discharge.Graphitic carbon nitride(g‐C3N4),a metal‐free semiconductor that exhibits high chemical stability,can utilize both the ultraviolet and visible light from high voltage discharge.However,the synergistic system of NTP and g‐C3N4 has been researched little.In this paper,the effect of NTP generated by dielectric barrier discharge(DBD)on g‐C3N4 is studied by comparing the photocatalytic activities,the surface physical structure and the surface chemical characteristics of pristine and plasma treated g‐C3N4.Experimental results indicate that the DBD plasma can change the physical structure and the chemical characteristics and to further affect the photocatalytic activity of g‐C3N4.The effect of NTP on g‐C3N4 is associated with the discharge intensity and the discharge time.For a long time scale,the effect of NTP on g‐C3N4 photocatalysts presents a periodic change trend.展开更多
Geological structures often exhibit smooth characteristics away from sharp discontinuities. One aim of geophysical inversion is to recover information about the smooth structures as well as about the sharp discontinui...Geological structures often exhibit smooth characteristics away from sharp discontinuities. One aim of geophysical inversion is to recover information about the smooth structures as well as about the sharp discontinuities. Because no specific operator can provide a perfect sparse representation of complicated geological models, hyper-parameter regularization inversion based on the iterative split Bregman method was used to recover the features of both smooth and sharp geological structures. A novel preconditioned matrix was proposed, which counteracted the natural decay of the sensitivity matrix and its inverse matrix was calculated easily. Application of the algorithm to synthetic data produces density models that are good representations of the designed models. The results show that the algorithm proposed is feasible and effective.展开更多
Flax fiber was used to reinforce Polypropylene (PP) owing to its lower impact on environment and suitable mechanical behaviors. To overcome the difficulty of penetrating fibers due to the high viscosity of thermo-pl...Flax fiber was used to reinforce Polypropylene (PP) owing to its lower impact on environment and suitable mechanical behaviors. To overcome the difficulty of penetrating fibers due to the high viscosity of thermo-plastic resin, PP filaments wrapping around the linen yam produced commingled yams, which were woven into fabrics as preforms to make laminates by optimum hot-pressing technology. The effects of fiber volume fraction, fabric density and structure on tensile properties of composites were researched through analyzing the tensile test results and the scanning electronic microscope (SEM) micrographs of fracture surface. Conclusions are drawn that the properties of laminates with fiber volume fraction of 0.50 are better than those with the other two fractions. For plain structure, the tensile properties in warp direction decrease according to the increase of weft density while in weft direction increase. For different fabric structures, properties of laminates with structures of plain 3, twill 2/2 and twill 3/1 increase gradually. And properties in weft direction are prior to those in warp direction for each laminate.展开更多
Cu?Ni nano-alloys were prepared using precursors synthesized by the citrate-gel method. The effects of initial solution pH value and calcination temperature on the composition, crystalline structure, purity, morpholog...Cu?Ni nano-alloys were prepared using precursors synthesized by the citrate-gel method. The effects of initial solution pH value and calcination temperature on the composition, crystalline structure, purity, morphology, homogeneity and grain size of Cu?Ni nanoparticles were investigated. Both the parameters significantly affect the crystalline structure, composition and grain size. Cu?Ni alloys prepared at pH value of 1 do not contain impurities, and their compositions are Cu0.42Ni0.58, Cu0.45Ni0.55 and Cu0.52Ni0.48 reduced at 300, 400 and 500 °C, respectively. The grain size grows with the increase of calcination temperature for the precursor prepared at pH values of 1.6 and 3. The Ni content of the alloys gradually increases with the increase of calcination temperature at pH value of 3.展开更多
Two-dimensional physical models of low crested breakwaters were tested to establish the effect of water depth, crest width, slope, stone size, core permeability and incident wave characteristics on the wave transforma...Two-dimensional physical models of low crested breakwaters were tested to establish the effect of water depth, crest width, slope, stone size, core permeability and incident wave characteristics on the wave transformation processes. The structure of the breakwaters can be used as coastal protection system by reducing the amount of incoming wave energy. Effect of slope, core permeability, water depth and incident wave characteristics on the stability was also studied. The breakwater model consisted of a core and two armour layers attacked by irregular waves. This paper discusses and compares the test results with the existing design equations. In general, the existing design equations do not seem to predict the wave transmission and reflection accurately for the range of test data. In the range of variable tested, it was observed that the water depth, crest width and wave period have a significant influence on wave transmission process. Further, results show strong influence of the water depth and wave period on the wave reflection process. The structural stability of low crested breakwaters is very much affected by the water depth and wave period.展开更多
In this work, the terahertz (THz) electromotive force (EMF) of the surface plasmon (SP) electric field and field strength was investigated in its propagation direction. Based on the nanowires structure, we intro...In this work, the terahertz (THz) electromotive force (EMF) of the surface plasmon (SP) electric field and field strength was investigated in its propagation direction. Based on the nanowires structure, we introduced physical models which were light wave energy of surface plasmon polariton (SPP) pulse and the variation of EMF changes in the active condition. Results of theory and verification showed SPP generated EMF with 10-2-10 V among wire radii of 5-30 nm; the electric field was up to 10^5-1066V/cm in the radius of 5 nm; the electric field intensity induced localization at λ=850 nm, and at the same time light intensity amplified 40 times. The characteristics which are femtosecond SPP pulse response and force-field amplifier in this work are significant for nonlinear spectroscopy research.展开更多
Black phosphorus (BP) is a good candidate for studying strain effects on two- dimensional (2D) materials beyond graphene and transition-metal dichalcogenides. This is because of its particular ability to sustain h...Black phosphorus (BP) is a good candidate for studying strain effects on two- dimensional (2D) materials beyond graphene and transition-metal dichalcogenides. This is because of its particular ability to sustain high strain and remarkably anisotropic mechanical properties resulting from its unique puckered structure. We here investigate the dependence of lattice vibrational frequencies on cry- stallographic orientations in uniaxially strained few-layer BP by in-situ strained Raman spectroscopy. The out-of-plane A1 mode is sensitive to uniaxial strain along the near-armchair direction whereas the in-plane B2g and A2 modes are sensitive to strain in the near-zigzag direction. For uniaxial strains applied away from these directions, all three phonon modes are linearly redshifted. Our experimental observation is explained by the anisotropic influence of uniaxial tensile strain on structural properties of BP using density functional theory. This study demonstrates the possibility of selective tuning of in-plane and out-of-plane phonon modes in BP by uniaxial strain and makes strain engineering a promising avenue for extensively modulating the optical and mechanical properties of 2D materials.展开更多
文摘The synergistic effect of high voltage discharge non‐thermal plasma(NTP)and photocatalysts on contaminant removal has repeatedly confirmed by plenty of researches.Most previous plasma‐photocatalyst synergistic systems focused on the utilization of the ultraviolet light but ignored the visible light generated by high voltage discharge.Graphitic carbon nitride(g‐C3N4),a metal‐free semiconductor that exhibits high chemical stability,can utilize both the ultraviolet and visible light from high voltage discharge.However,the synergistic system of NTP and g‐C3N4 has been researched little.In this paper,the effect of NTP generated by dielectric barrier discharge(DBD)on g‐C3N4 is studied by comparing the photocatalytic activities,the surface physical structure and the surface chemical characteristics of pristine and plasma treated g‐C3N4.Experimental results indicate that the DBD plasma can change the physical structure and the chemical characteristics and to further affect the photocatalytic activity of g‐C3N4.The effect of NTP on g‐C3N4 is associated with the discharge intensity and the discharge time.For a long time scale,the effect of NTP on g‐C3N4 photocatalysts presents a periodic change trend.
基金Projects(41174061,41374120)supported by the National Natural Science Foundation of China
文摘Geological structures often exhibit smooth characteristics away from sharp discontinuities. One aim of geophysical inversion is to recover information about the smooth structures as well as about the sharp discontinuities. Because no specific operator can provide a perfect sparse representation of complicated geological models, hyper-parameter regularization inversion based on the iterative split Bregman method was used to recover the features of both smooth and sharp geological structures. A novel preconditioned matrix was proposed, which counteracted the natural decay of the sensitivity matrix and its inverse matrix was calculated easily. Application of the algorithm to synthetic data produces density models that are good representations of the designed models. The results show that the algorithm proposed is feasible and effective.
文摘Flax fiber was used to reinforce Polypropylene (PP) owing to its lower impact on environment and suitable mechanical behaviors. To overcome the difficulty of penetrating fibers due to the high viscosity of thermo-plastic resin, PP filaments wrapping around the linen yam produced commingled yams, which were woven into fabrics as preforms to make laminates by optimum hot-pressing technology. The effects of fiber volume fraction, fabric density and structure on tensile properties of composites were researched through analyzing the tensile test results and the scanning electronic microscope (SEM) micrographs of fracture surface. Conclusions are drawn that the properties of laminates with fiber volume fraction of 0.50 are better than those with the other two fractions. For plain structure, the tensile properties in warp direction decrease according to the increase of weft density while in weft direction increase. For different fabric structures, properties of laminates with structures of plain 3, twill 2/2 and twill 3/1 increase gradually. And properties in weft direction are prior to those in warp direction for each laminate.
基金Universidad Nacional de San Luis, Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)Fondo para la Investigación Científica y Técnológica (FONCy T), Argentina,for their financial support
文摘Cu?Ni nano-alloys were prepared using precursors synthesized by the citrate-gel method. The effects of initial solution pH value and calcination temperature on the composition, crystalline structure, purity, morphology, homogeneity and grain size of Cu?Ni nanoparticles were investigated. Both the parameters significantly affect the crystalline structure, composition and grain size. Cu?Ni alloys prepared at pH value of 1 do not contain impurities, and their compositions are Cu0.42Ni0.58, Cu0.45Ni0.55 and Cu0.52Ni0.48 reduced at 300, 400 and 500 °C, respectively. The grain size grows with the increase of calcination temperature for the precursor prepared at pH values of 1.6 and 3. The Ni content of the alloys gradually increases with the increase of calcination temperature at pH value of 3.
文摘Two-dimensional physical models of low crested breakwaters were tested to establish the effect of water depth, crest width, slope, stone size, core permeability and incident wave characteristics on the wave transformation processes. The structure of the breakwaters can be used as coastal protection system by reducing the amount of incoming wave energy. Effect of slope, core permeability, water depth and incident wave characteristics on the stability was also studied. The breakwater model consisted of a core and two armour layers attacked by irregular waves. This paper discusses and compares the test results with the existing design equations. In general, the existing design equations do not seem to predict the wave transmission and reflection accurately for the range of test data. In the range of variable tested, it was observed that the water depth, crest width and wave period have a significant influence on wave transmission process. Further, results show strong influence of the water depth and wave period on the wave reflection process. The structural stability of low crested breakwaters is very much affected by the water depth and wave period.
基金supported by the National Natural Science Foundation of China (Grant No. 60877047)the Natural Science Foundation of Hebei Province,China (Grant No. F20100002002)
文摘In this work, the terahertz (THz) electromotive force (EMF) of the surface plasmon (SP) electric field and field strength was investigated in its propagation direction. Based on the nanowires structure, we introduced physical models which were light wave energy of surface plasmon polariton (SPP) pulse and the variation of EMF changes in the active condition. Results of theory and verification showed SPP generated EMF with 10-2-10 V among wire radii of 5-30 nm; the electric field was up to 10^5-1066V/cm in the radius of 5 nm; the electric field intensity induced localization at λ=850 nm, and at the same time light intensity amplified 40 times. The characteristics which are femtosecond SPP pulse response and force-field amplifier in this work are significant for nonlinear spectroscopy research.
文摘Black phosphorus (BP) is a good candidate for studying strain effects on two- dimensional (2D) materials beyond graphene and transition-metal dichalcogenides. This is because of its particular ability to sustain high strain and remarkably anisotropic mechanical properties resulting from its unique puckered structure. We here investigate the dependence of lattice vibrational frequencies on cry- stallographic orientations in uniaxially strained few-layer BP by in-situ strained Raman spectroscopy. The out-of-plane A1 mode is sensitive to uniaxial strain along the near-armchair direction whereas the in-plane B2g and A2 modes are sensitive to strain in the near-zigzag direction. For uniaxial strains applied away from these directions, all three phonon modes are linearly redshifted. Our experimental observation is explained by the anisotropic influence of uniaxial tensile strain on structural properties of BP using density functional theory. This study demonstrates the possibility of selective tuning of in-plane and out-of-plane phonon modes in BP by uniaxial strain and makes strain engineering a promising avenue for extensively modulating the optical and mechanical properties of 2D materials.