The collective Bamiltonian up to the fourth order for multi-O（4） model is derived based on the self-consistent collective-coordinate （SCC） method, which is formulated in the framework of the time-dependent Hartree...The collective Bamiltonian up to the fourth order for multi-O（4） model is derived based on the self-consistent collective-coordinate （SCC） method, which is formulated in the framework of the time-dependent Hartree-Bogoliubov （TDHB） theory. The validity of the collective Hamiltonian is checked in the two special cases of the multi-O（4） model： the case where the number of the shells is equal to one （a single j-shell case）, and the case where the Hartree-Bogoliubov equilibrium point is spherical （the spherical case）. The collective Hamiltonian constitutes a good starting point to study nuclear shape coexistence.展开更多
The effective action for spin-1 bosonic atom in an optical lattice is derived. The quasiparticle and quasihole dispersions are calculated for different cases by using a functional integral formalism. For all cases, th...The effective action for spin-1 bosonic atom in an optical lattice is derived. The quasiparticle and quasihole dispersions are calculated for different cases by using a functional integral formalism. For all cases, the excitation spectra are analyzed. All the quasiparticle and quasihole excitations start with a gap.展开更多
OBJECTIVE To examine the influence of tumor osseous metastasis on the patients undergoing autoiogous peripheral blood stem ceil collection. METHODS A total of 36 patients with malignant diseases who received an autoio...OBJECTIVE To examine the influence of tumor osseous metastasis on the patients undergoing autoiogous peripheral blood stem ceil collection. METHODS A total of 36 patients with malignant diseases who received an autoiogous peripheral blood stem ceil transplantation, during a period from April 2004 to June 2006, were chosen. The patients were divided into two groups, i.e. group A were patients with a complication of tumor osseous metastasis, and group B were without metastasis. Both groups were treated with Taxotere 120 mg/m^2 plus granuiocyte colony-stimulating factor （G-CSF） 5 μg/kg/d, for a mobilization regimen. A blood ceil separator was used to collect the mononuciear ceils. The proportion of harvested CD34＋ ceils in the peripheral blood and the collected mononuciear ceils were detected by flow cytometry. The number of CD34＋ ceils was used to determine the difference in the nature of the collections between the two groups. RESULTS After mobilization in groups A and B, the number of the peripheral blood mononuciear ceils （PBMC） was 39.3±14.7% and 41.1±12.4 % and the proportion of CD34＋ ceils was 0.16±0.07% and 0.17±0.10%, respectively. Following administration of the drugs, there was no significant difference between the number of harvested PBMC and CD34＋ cells of the two groups, i.e., 3.47±1.16×10^8/Kg and 2.52±1.43×10^6/Kg in group A and 4.02±1.31×10^8/Kg and 2.73±1.87×10^6/Kg in group B, respectively. CONCLUSION Osseous metastasis, as a single factor, may have no impact on mobilization and harvesting of hematopoietic stem ceils and their engraftment after autotransplantation.展开更多
A novel mixed-valent heterometallic pentanuclear CoⅢ3 CoⅡ Dy Ⅲ cluster has been rationally assembled taking advantage of a bifunctional ligand with o-vanillin and tripodal tris(hydroxymethyl)aminomethane units. Thi...A novel mixed-valent heterometallic pentanuclear CoⅢ3 CoⅡ Dy Ⅲ cluster has been rationally assembled taking advantage of a bifunctional ligand with o-vanillin and tripodal tris(hydroxymethyl)aminomethane units. This unique heterometallic cluster represents a rare example of T-shaped molecules exhibiting slow magnetic relaxation.展开更多
The rapid transition between spherical and γ-soft shapes in Zn isotopes in the mass A 70 region,is analyzed using excitation spectra and collective wave functions obtained by diagonalization of a five-dimensional Ham...The rapid transition between spherical and γ-soft shapes in Zn isotopes in the mass A 70 region,is analyzed using excitation spectra and collective wave functions obtained by diagonalization of a five-dimensional Hamiltonian for quadrupole vibrational and rotational degrees of freedom,with parameters determined by constrained self-consistent relativistic mean-field calculations for triaxial shapes.The microscopic potential energy surfaces,together with the characteristic collective observables,illustrate a rapid transition from near spherical shape at the N = 40 subshell,to γ-soft deformed shapes for lighter isotopes.The calculated spectra display fingerprints of a second-order shape phase transition that can be approximately described by the E(5) analytic solution.展开更多
We present here a brief summary of a National Natural Science Foundation Major Project entitled "Theoretical study of the low-lying electronic excited state for molecular aggregates". The project focuses on ...We present here a brief summary of a National Natural Science Foundation Major Project entitled "Theoretical study of the low-lying electronic excited state for molecular aggregates". The project focuses on theoretical investigation of the electronic structures and dynamic processes upon photo-and electric-excitation for molecules and aggregates. We aim to develop reliable methodology to predict the optoelectronic properties of molecular materials related to the electronic excitations and to apply in the experiments. We identify two essential scientific challenges: (i) nature of intramolecular and intermolecular electronic excited states; (ii) theoretical description of the dynamic processes of the coupled motion of electronic excitations and nucleus. We propose the following four subjects of research: (i) linear scaling time-dependent density-functional theory and its application to open shell system; (ii) computational method development of electronic excited state for molecular aggregates; (iii) theoretical investigation of the time evolution of the excited state dynamics; (iv) methods to predict the optoelectronic properties starting from electronic excited state investigation for organic materials and experimental verifications.展开更多
In the past three decades, molecular magnetism has been a rapidly growing interdisciplinary field in chemistry, phys- ics and materials sciences. It covers diverse range of topics including inorganic/organic/hybrid ma...In the past three decades, molecular magnetism has been a rapidly growing interdisciplinary field in chemistry, phys- ics and materials sciences. It covers diverse range of topics including inorganic/organic/hybrid magnetic molecular ma- terials, multifunctional and/or switchable magnetic molecu- lar materials, molecular nanomagnets, nanostructural mo- lecular magnets, molecular spintronics and biomagnetism. Much research on molecular magnetism has been carried out in China both before and after we organized the Interna- tional Conference on Molecule-Based Magnets 2010 （ICMM 2010） in Beijing.展开更多
基金The project supported by the Director Foundation from the Department of Nuclear Physics of China Institute of Atomic Energy under Grant Nos. 11SZZ200501 and 11SZZ200601 0ne of the authors （J.Z. Gu） is grateful to H. Aiba, K. Hagino, K. Matsuyanagi, S. Mizutori, F. Sakata, and Y.Z. Zhuo for valuable discussions on this subject. He also acknowledges support from Postdoctoral Fellowship for Foreign Researchers of the Japan Society for the Promotion of Science with thanks.
文摘The collective Bamiltonian up to the fourth order for multi-O（4） model is derived based on the self-consistent collective-coordinate （SCC） method, which is formulated in the framework of the time-dependent Hartree-Bogoliubov （TDHB） theory. The validity of the collective Hamiltonian is checked in the two special cases of the multi-O（4） model： the case where the number of the shells is equal to one （a single j-shell case）, and the case where the Hartree-Bogoliubov equilibrium point is spherical （the spherical case）. The collective Hamiltonian constitutes a good starting point to study nuclear shape coexistence.
基金The project supported in part by National Natural Science Foundation of China under Grant Nos. 10547107, 10447125, and Doctoral Starting Fund from Southeast University under Grant No. 9207022244
文摘The effective action for spin-1 bosonic atom in an optical lattice is derived. The quasiparticle and quasihole dispersions are calculated for different cases by using a functional integral formalism. For all cases, the excitation spectra are analyzed. All the quasiparticle and quasihole excitations start with a gap.
文摘OBJECTIVE To examine the influence of tumor osseous metastasis on the patients undergoing autoiogous peripheral blood stem ceil collection. METHODS A total of 36 patients with malignant diseases who received an autoiogous peripheral blood stem ceil transplantation, during a period from April 2004 to June 2006, were chosen. The patients were divided into two groups, i.e. group A were patients with a complication of tumor osseous metastasis, and group B were without metastasis. Both groups were treated with Taxotere 120 mg/m^2 plus granuiocyte colony-stimulating factor （G-CSF） 5 μg/kg/d, for a mobilization regimen. A blood ceil separator was used to collect the mononuciear ceils. The proportion of harvested CD34＋ ceils in the peripheral blood and the collected mononuciear ceils were detected by flow cytometry. The number of CD34＋ ceils was used to determine the difference in the nature of the collections between the two groups. RESULTS After mobilization in groups A and B, the number of the peripheral blood mononuciear ceils （PBMC） was 39.3±14.7% and 41.1±12.4 % and the proportion of CD34＋ ceils was 0.16±0.07% and 0.17±0.10%, respectively. Following administration of the drugs, there was no significant difference between the number of harvested PBMC and CD34＋ cells of the two groups, i.e., 3.47±1.16×10^8/Kg and 2.52±1.43×10^6/Kg in group A and 4.02±1.31×10^8/Kg and 2.73±1.87×10^6/Kg in group B, respectively. CONCLUSION Osseous metastasis, as a single factor, may have no impact on mobilization and harvesting of hematopoietic stem ceils and their engraftment after autotransplantation.
基金supported by the National Natural Science Foundation of China (91022009, 20921002)
文摘A novel mixed-valent heterometallic pentanuclear CoⅢ3 CoⅡ Dy Ⅲ cluster has been rationally assembled taking advantage of a bifunctional ligand with o-vanillin and tripodal tris(hydroxymethyl)aminomethane units. This unique heterometallic cluster represents a rare example of T-shaped molecules exhibiting slow magnetic relaxation.
基金supported in part by the Major State Basic Research Developing Program (Grant No 2007CB815000)the National Natural Science Foundation of China (Grant Nos 11005004, 10775004 and 10975008)+1 种基金the Southwest University Initial Research Foundation Grant to Doctor (Grant No.SWU110039)MZOS (Grant No 1191005-1010)
文摘The rapid transition between spherical and γ-soft shapes in Zn isotopes in the mass A 70 region,is analyzed using excitation spectra and collective wave functions obtained by diagonalization of a five-dimensional Hamiltonian for quadrupole vibrational and rotational degrees of freedom,with parameters determined by constrained self-consistent relativistic mean-field calculations for triaxial shapes.The microscopic potential energy surfaces,together with the characteristic collective observables,illustrate a rapid transition from near spherical shape at the N = 40 subshell,to γ-soft deformed shapes for lighter isotopes.The calculated spectra display fingerprints of a second-order shape phase transition that can be approximately described by the E(5) analytic solution.
基金the National Natural Science Foundation of China (21290190)
文摘We present here a brief summary of a National Natural Science Foundation Major Project entitled "Theoretical study of the low-lying electronic excited state for molecular aggregates". The project focuses on theoretical investigation of the electronic structures and dynamic processes upon photo-and electric-excitation for molecules and aggregates. We aim to develop reliable methodology to predict the optoelectronic properties of molecular materials related to the electronic excitations and to apply in the experiments. We identify two essential scientific challenges: (i) nature of intramolecular and intermolecular electronic excited states; (ii) theoretical description of the dynamic processes of the coupled motion of electronic excitations and nucleus. We propose the following four subjects of research: (i) linear scaling time-dependent density-functional theory and its application to open shell system; (ii) computational method development of electronic excited state for molecular aggregates; (iii) theoretical investigation of the time evolution of the excited state dynamics; (iv) methods to predict the optoelectronic properties starting from electronic excited state investigation for organic materials and experimental verifications.
文摘In the past three decades, molecular magnetism has been a rapidly growing interdisciplinary field in chemistry, phys- ics and materials sciences. It covers diverse range of topics including inorganic/organic/hybrid magnetic molecular ma- terials, multifunctional and/or switchable magnetic molecu- lar materials, molecular nanomagnets, nanostructural mo- lecular magnets, molecular spintronics and biomagnetism. Much research on molecular magnetism has been carried out in China both before and after we organized the Interna- tional Conference on Molecule-Based Magnets 2010 （ICMM 2010） in Beijing.
