This minireview summarizes our recent findings on the photoactivity of S-doped nanoporous carbons. The materials were either synthesized from the sulfur-containing polymers or obtained by heat treatment of commercial ...This minireview summarizes our recent findings on the photoactivity of S-doped nanoporous carbons. The materials were either synthesized from the sulfur-containing polymers or obtained by heat treatment of commercial carbon with hydrogen sulfide. Their surface was extensively charac terized from the points of view of its surface chemistry, porosity, morphology, and electronic properties. The carbons showed enhanced activity towards oxidation of arsine and removal of diben-zothiophenes from model diesel fuel. The latter were oxidized to various oxygen containing intermediates and the cleavage of C–C bonds in aromatic ring was detected when carbon with adsorbed species was exposed to UV or visible light. Irradiation resulted in generation of photocurrent in a broad range of wavelength. The presence of sulfur led to the reduction of oxygen and contributed to an increased capacitive performance. We link these effects to the presence of reduced sulfur in the small pores which enhances the dispersive interactions via inducing a positive charge to carbon atoms, to sulfur in oxygenated forms which contribute to Faradaic reactions and increase the polar interactions, and to the hydrophobicity of a surface in small pores where oxygen can be reduced by excited electrons from chromophoric-like sulfur containing groups.展开更多
We discuss the generation of certain kinds of multi-component entangled states for three-level atomic system with hyperfine structure. The method proposed here is based on the interactions of dispersive cavity with on...We discuss the generation of certain kinds of multi-component entangled states for three-level atomic system with hyperfine structure. The method proposed here is based on the interactions of dispersive cavity with only one atom driven by a strong classical field. It is shown that, with a judicious choice of the cavity detuning and applied coherent field detuning, the atom can interact dispersively with the quantized field but the classical driving field gives rise to the creation or destruction of photons conditional on the state of the system. In comparison with previous schemes,our method is likely to be extremely easy to realize in展开更多
Using the mapping method based on q-deformed hyperbolic functions,the exact solutions of generalizedBreor-Kaup equations are obtained.Based on the solutions,two coherent structures,periodic-branch kink and non-propaga...Using the mapping method based on q-deformed hyperbolic functions,the exact solutions of generalizedBreor-Kaup equations are obtained.Based on the solutions,two coherent structures,periodic-branch kink and non-propagating kink,have been obtained.Moreover,one solitonal interaction form,two line solitons interaction on the kinkbackground,has been found.展开更多
We propose a new scheme for realizing deterministic quantum state transfer （QST） between two spatially separated single molecule magnets （SMMs） with the framework of cavity quantum eleetrodynamics （QED）. In the ...We propose a new scheme for realizing deterministic quantum state transfer （QST） between two spatially separated single molecule magnets （SMMs） with the framework of cavity quantum eleetrodynamics （QED）. In the present scheme, two SMMs are trapped in two spatially separated optical cavities coupled by an optical fiber. Through strictly numerically simulating, we demonstrate that our scheme is robust with respect to the SMMs＇ spontaneous decay and fiber loss under the conditions of dispersive SMMs-field interaction and strong coupling of cavity fiber. In addition, we also discuss the influence of photon leakage out of cavities and show that our proposal is good enough to demonstrate the generation of QST with high fidelity utilizing the current experimental technology. The present investigation provides research opportunities for realizing QST between solid-state qubits and may result in a substantial impact on the progress of solid-state-based quantum communications network.展开更多
Within the framework of the macroscopic dielectric continuum model and Loudon＇s uniaxial crystal model, the phonon modes of a wurtzite/zinc-blende one-dimensional （1D） cylindrical nanowire （NW） are derived and st...Within the framework of the macroscopic dielectric continuum model and Loudon＇s uniaxial crystal model, the phonon modes of a wurtzite/zinc-blende one-dimensional （1D） cylindrical nanowire （NW） are derived and studied. The analytical phonon states of phonon modes are given. It is found that there exist two types of polar phonon modes, i.e. interface optical （IO） phonon modes and the quasi-confined （QC） phonon modes existing in 1D wurtzite/zinc-blende NWs. Via the standard procedure of field quantization, the Fr6hlich electron-phonon interaction Hamiltonians are obtained. Numerical calculations of dispersive behavior of these phonon modes on a wurtzite/zinc-blende ZnO/MgO NW are performed. The frequency ranges of the IO and QC phonon modes of the ZnO/MgO NWs are analyzed and discussed. It is found that the IO modes only exist in one frequency range, while QC modes may appear in three frequency ranges. The dispersive properties of the IO and QC modes on the free wave-number kz and the azimuthal quantum number m are discussed. The analytical Hamiltonians of electron-phonon interaction obtained here are quite useful for further investigating phonon influence on optoelectronics properties of wurtzite/zinc-blende 1D NW structures.展开更多
We propose an approach to detect an unknown quantum state of the atom(s) by measuring the phase shifts of the transmitted photons through a dispersively-coupled cavity. In the framework of the input-output theory, we ...We propose an approach to detect an unknown quantum state of the atom(s) by measuring the phase shifts of the transmitted photons through a dispersively-coupled cavity. In the framework of the input-output theory, we derive the relations between the phase shifts of the transmitted photons and the states of the atom(s) in the cavity. It is shown that due to the dispersive interaction between the cavity and the atom(s), information about the atomic state can then be extracted by measuring the phase shifts of the transmitted photons through the cavity. The feasibility of the proposal is also discussed with the experimental parameters by numerical method.展开更多
Transport and diffusion caused by coastal waves have different characteristics from those induced by flows. Through solving the vertical diffusion equation by an analytic method, this paper infers a theoretical formul...Transport and diffusion caused by coastal waves have different characteristics from those induced by flows. Through solving the vertical diffusion equation by an analytic method, this paper infers a theoretical formula of dispersion coefficient under the combined action of current and waves. It divides the general dispersion coefficient into six parts, including coefficients due to tidal current, Stokes drift, wave oscillation and interaction among them. It draws a conclusion that the contribution of dispersive effect induced by coastal waves is mainly produced by Stokes drift, while the contributions to time-averaged dispersion coefficient due to wave orbital motion and interaction between current and waves are very small. The results without tidal current are in agreement with the numerical and experimental results, which proves the correctness of the theoretical derivation. This paper introduces the variation characteristics of both the time-averaged and oscillating dispersion coefficients versus relative water depth, and demonstrates the physical implications of the oscillating mixing coefficient due to waves. We also apply the results to the costal vertical circulation and give its characteristics compared to Stokes drift.展开更多
In the present paper the problem of nonlinear interaction of two mildly-relativistic circularly polarized lasers in a cold plasma is studied in order to investigate electromagneticaily induced transparency （EIT）. Ba...In the present paper the problem of nonlinear interaction of two mildly-relativistic circularly polarized lasers in a cold plasma is studied in order to investigate electromagneticaily induced transparency （EIT）. Based on a relativistic kinetic model, by expansion of relativistic Lorentz factor in terms of lasers amplitude, we obtain the coupled nonlinear dispersion relations. It is observed that due to resonance in the second harmonic of plasma beat-wave, the new EIT pass-band is created in the high intensities of lasers. The effect of amplitude and frequency variation on the dispersion is numerically investigated.展开更多
文摘This minireview summarizes our recent findings on the photoactivity of S-doped nanoporous carbons. The materials were either synthesized from the sulfur-containing polymers or obtained by heat treatment of commercial carbon with hydrogen sulfide. Their surface was extensively charac terized from the points of view of its surface chemistry, porosity, morphology, and electronic properties. The carbons showed enhanced activity towards oxidation of arsine and removal of diben-zothiophenes from model diesel fuel. The latter were oxidized to various oxygen containing intermediates and the cleavage of C–C bonds in aromatic ring was detected when carbon with adsorbed species was exposed to UV or visible light. Irradiation resulted in generation of photocurrent in a broad range of wavelength. The presence of sulfur led to the reduction of oxygen and contributed to an increased capacitive performance. We link these effects to the presence of reduced sulfur in the small pores which enhances the dispersive interactions via inducing a positive charge to carbon atoms, to sulfur in oxygenated forms which contribute to Faradaic reactions and increase the polar interactions, and to the hydrophobicity of a surface in small pores where oxygen can be reduced by excited electrons from chromophoric-like sulfur containing groups.
文摘We discuss the generation of certain kinds of multi-component entangled states for three-level atomic system with hyperfine structure. The method proposed here is based on the interactions of dispersive cavity with only one atom driven by a strong classical field. It is shown that, with a judicious choice of the cavity detuning and applied coherent field detuning, the atom can interact dispersively with the quantized field but the classical driving field gives rise to the creation or destruction of photons conditional on the state of the system. In comparison with previous schemes,our method is likely to be extremely easy to realize in
基金National Natural Science Foundation of China under Grant Nos.10535010 and 10775123the Research Fund of Ministry of Education under Grant No.20070284016
文摘Using the mapping method based on q-deformed hyperbolic functions,the exact solutions of generalizedBreor-Kaup equations are obtained.Based on the solutions,two coherent structures,periodic-branch kink and non-propagating kink,have been obtained.Moreover,one solitonal interaction form,two line solitons interaction on the kinkbackground,has been found.
基金Supported by the Natural Science Foundation of China under Grant Nos.10575040,90503010,10634060,and 10874050 National Basic Research Program of China under Grant No.2005CB724508+1 种基金the Foundation from the Ministry of the National Education of China under Grant No.200804870051 the Science Innovation Foundation of Huazhong University of Science and Technology under Grant No.HF-06-010-08-012
文摘We propose a new scheme for realizing deterministic quantum state transfer （QST） between two spatially separated single molecule magnets （SMMs） with the framework of cavity quantum eleetrodynamics （QED）. In the present scheme, two SMMs are trapped in two spatially separated optical cavities coupled by an optical fiber. Through strictly numerically simulating, we demonstrate that our scheme is robust with respect to the SMMs＇ spontaneous decay and fiber loss under the conditions of dispersive SMMs-field interaction and strong coupling of cavity fiber. In addition, we also discuss the influence of photon leakage out of cavities and show that our proposal is good enough to demonstrate the generation of QST with high fidelity utilizing the current experimental technology. The present investigation provides research opportunities for realizing QST between solid-state qubits and may result in a substantial impact on the progress of solid-state-based quantum communications network.
基金Supported by National Natural Science Foundation of China under Grant No.60906042by the National Basic Research Program of China under Grant No.2006CB921607
文摘Within the framework of the macroscopic dielectric continuum model and Loudon＇s uniaxial crystal model, the phonon modes of a wurtzite/zinc-blende one-dimensional （1D） cylindrical nanowire （NW） are derived and studied. The analytical phonon states of phonon modes are given. It is found that there exist two types of polar phonon modes, i.e. interface optical （IO） phonon modes and the quasi-confined （QC） phonon modes existing in 1D wurtzite/zinc-blende NWs. Via the standard procedure of field quantization, the Fr6hlich electron-phonon interaction Hamiltonians are obtained. Numerical calculations of dispersive behavior of these phonon modes on a wurtzite/zinc-blende ZnO/MgO NW are performed. The frequency ranges of the IO and QC phonon modes of the ZnO/MgO NWs are analyzed and discussed. It is found that the IO modes only exist in one frequency range, while QC modes may appear in three frequency ranges. The dispersive properties of the IO and QC modes on the free wave-number kz and the azimuthal quantum number m are discussed. The analytical Hamiltonians of electron-phonon interaction obtained here are quite useful for further investigating phonon influence on optoelectronics properties of wurtzite/zinc-blende 1D NW structures.
基金Supported by the Special Funds of the National Natural Science Foundation of China under Grant Nos.11247032 and 11247207the National Fundamental Research Program of China under Grant No.2010CB923104
文摘We propose an approach to detect an unknown quantum state of the atom(s) by measuring the phase shifts of the transmitted photons through a dispersively-coupled cavity. In the framework of the input-output theory, we derive the relations between the phase shifts of the transmitted photons and the states of the atom(s) in the cavity. It is shown that due to the dispersive interaction between the cavity and the atom(s), information about the atomic state can then be extracted by measuring the phase shifts of the transmitted photons through the cavity. The feasibility of the proposal is also discussed with the experimental parameters by numerical method.
基金supported by the National Natural Science Foundation of China (Grant Nos. 10672034, 51079024)the Funds for Creative Re-search Groups of China (Grant No. 50921001)
文摘Transport and diffusion caused by coastal waves have different characteristics from those induced by flows. Through solving the vertical diffusion equation by an analytic method, this paper infers a theoretical formula of dispersion coefficient under the combined action of current and waves. It divides the general dispersion coefficient into six parts, including coefficients due to tidal current, Stokes drift, wave oscillation and interaction among them. It draws a conclusion that the contribution of dispersive effect induced by coastal waves is mainly produced by Stokes drift, while the contributions to time-averaged dispersion coefficient due to wave orbital motion and interaction between current and waves are very small. The results without tidal current are in agreement with the numerical and experimental results, which proves the correctness of the theoretical derivation. This paper introduces the variation characteristics of both the time-averaged and oscillating dispersion coefficients versus relative water depth, and demonstrates the physical implications of the oscillating mixing coefficient due to waves. We also apply the results to the costal vertical circulation and give its characteristics compared to Stokes drift.
文摘In the present paper the problem of nonlinear interaction of two mildly-relativistic circularly polarized lasers in a cold plasma is studied in order to investigate electromagneticaily induced transparency （EIT）. Based on a relativistic kinetic model, by expansion of relativistic Lorentz factor in terms of lasers amplitude, we obtain the coupled nonlinear dispersion relations. It is observed that due to resonance in the second harmonic of plasma beat-wave, the new EIT pass-band is created in the high intensities of lasers. The effect of amplitude and frequency variation on the dispersion is numerically investigated.
