The ultrafast dissociation dynamics of NO2 molecules was investigated by femtosecond laser pump-probe mass spectra and ion images.The results show that the kinetic energy release of NO+ions has two components,0.05 eV ...The ultrafast dissociation dynamics of NO2 molecules was investigated by femtosecond laser pump-probe mass spectra and ion images.The results show that the kinetic energy release of NO+ions has two components,0.05 eV and 0.25 eV,and the possible dissociation channels have been assigned.The channel resolved transient measurement of NO^+provides a method to disentangle the contribution of ultrafast dissociation pathways,and the transient curves of NO^+ions at different kinetic energy release are fitted by a biexponential function.The fast component with a decay time of 0.25 ps is generated from the evolution of Rydberg states.The slow component is generated from two competitive channels,one of the channel is absorbing one 400nm photon to the excited state A^2B2,which has a decay time of 30.0ps,and the other slow channel is absorbing three 400nm photons to valence type Rydberg states which have a decay time less than 7.2ps.The channel and time resolved experiment present the potential of sorting out the complex ultrafast dissociation dynamics of molecules.展开更多
Electron-positron pair production in an arbitrary polarized ultrastrong laser field is investigated in the first order perturbation approximation in which the Volkov states are used for convenient calculation of scatt...Electron-positron pair production in an arbitrary polarized ultrastrong laser field is investigated in the first order perturbation approximation in which the Volkov states are used for convenient calculation of scattering amplitude and cross section. It is found surprisingly that the optimal pair production depends strongly on the polarization. For some cases of field parameters, the optimal field is e11iptically polarized or evenly circularly polarized one, rather than the usual linear polarization as indicated by previous works interesting unexpected features are a/so discussed briefly. Some insights into pair generation are given and some展开更多
基金supported by the National Natural Science Foundation of China(No.11704148,No.11847039,No.11534004)
文摘The ultrafast dissociation dynamics of NO2 molecules was investigated by femtosecond laser pump-probe mass spectra and ion images.The results show that the kinetic energy release of NO+ions has two components,0.05 eV and 0.25 eV,and the possible dissociation channels have been assigned.The channel resolved transient measurement of NO^+provides a method to disentangle the contribution of ultrafast dissociation pathways,and the transient curves of NO^+ions at different kinetic energy release are fitted by a biexponential function.The fast component with a decay time of 0.25 ps is generated from the evolution of Rydberg states.The slow component is generated from two competitive channels,one of the channel is absorbing one 400nm photon to the excited state A^2B2,which has a decay time of 30.0ps,and the other slow channel is absorbing three 400nm photons to valence type Rydberg states which have a decay time less than 7.2ps.The channel and time resolved experiment present the potential of sorting out the complex ultrafast dissociation dynamics of molecules.
基金Supported by the National Natural Science Foundation of China (NNSFC) under Grant Nos. 11175023, 11175020the Fundamental Research Funds for the Central Universities (FRFCU)
文摘Electron-positron pair production in an arbitrary polarized ultrastrong laser field is investigated in the first order perturbation approximation in which the Volkov states are used for convenient calculation of scattering amplitude and cross section. It is found surprisingly that the optimal pair production depends strongly on the polarization. For some cases of field parameters, the optimal field is e11iptically polarized or evenly circularly polarized one, rather than the usual linear polarization as indicated by previous works interesting unexpected features are a/so discussed briefly. Some insights into pair generation are given and some
