Perovskite quantum-dot-based light-emitting diodes(QLEDs)are highly promising for future solid-state lightings and high-definition displays due to their excellent color purity.However,their device performance is easil...Perovskite quantum-dot-based light-emitting diodes(QLEDs)are highly promising for future solid-state lightings and high-definition displays due to their excellent color purity.However,their device performance is easily affected by charge accumulation induced luminescence quenching due to imbalanced charge injection in the devices.Here we report green perovskite QLEDs with simultaneously improved efficiency and operational lifetime through balancing the charge injection with the employment of a bilayered electron transport structure.The charge-balanced QLEDs exhibit a color-saturated green emission with a full-width at half-maximum(FWHM)of 18 nm and a peak at 520 nm,a low turn-on voltage of2.0 V and a champion external quantum efficiency(EQE)of 21.63%,representing one of the most efficient perovskite QLEDs so far.In addition,the devices with modulated charge balance demonstrate a nearly 20-fold improvement in the operational lifetime compared to the control device.Our results demonstrate the great potential of further improving the device performance of perovskite QLEDs toward practical applications in lightings and displays via rational device engineering.展开更多
This paper is devoted to the analysis of the Cauchy problem for a system of PDEs arising in radiative hydrodynamics. This system, which comes from the so-called equilibrium diffusion regime, is a variant of the usual ...This paper is devoted to the analysis of the Cauchy problem for a system of PDEs arising in radiative hydrodynamics. This system, which comes from the so-called equilibrium diffusion regime, is a variant of the usual Euler equations, where the energy and pressure functionals are modified to take into account the effect of radiation and the energy balance containing a nonlinear diffusion term acting on the temperature. The problem is studied in the multi-dimensional framework. The authors identify the existence of a strictly convex entropy and a stability property of the system, and check that the Kawashima-Shizuta condition holds. Then, based on these structure properties, the wellposedness close to a constant state can be proved by using fine energy estimates. The asymptotic decay of the solutions are also investigated.展开更多
基金supported by the National Natural Science Foundation of China (51922049, 61604074)the National Key Research and Development Program of China (2016YFB0401701)+2 种基金the Natural Science Foundation of Jiangsu Province (BK20180020)the Fundamental Research Funds for the Central Universities (30920032102)PAPD of Jiangsu Higher Education Institutions
文摘Perovskite quantum-dot-based light-emitting diodes(QLEDs)are highly promising for future solid-state lightings and high-definition displays due to their excellent color purity.However,their device performance is easily affected by charge accumulation induced luminescence quenching due to imbalanced charge injection in the devices.Here we report green perovskite QLEDs with simultaneously improved efficiency and operational lifetime through balancing the charge injection with the employment of a bilayered electron transport structure.The charge-balanced QLEDs exhibit a color-saturated green emission with a full-width at half-maximum(FWHM)of 18 nm and a peak at 520 nm,a low turn-on voltage of2.0 V and a champion external quantum efficiency(EQE)of 21.63%,representing one of the most efficient perovskite QLEDs so far.In addition,the devices with modulated charge balance demonstrate a nearly 20-fold improvement in the operational lifetime compared to the control device.Our results demonstrate the great potential of further improving the device performance of perovskite QLEDs toward practical applications in lightings and displays via rational device engineering.
基金Project supported by the Fundamental Research Funds for the Central Universities (No. 2009B27514)the National Natural Science Foundation of China (No. 10871059)
文摘This paper is devoted to the analysis of the Cauchy problem for a system of PDEs arising in radiative hydrodynamics. This system, which comes from the so-called equilibrium diffusion regime, is a variant of the usual Euler equations, where the energy and pressure functionals are modified to take into account the effect of radiation and the energy balance containing a nonlinear diffusion term acting on the temperature. The problem is studied in the multi-dimensional framework. The authors identify the existence of a strictly convex entropy and a stability property of the system, and check that the Kawashima-Shizuta condition holds. Then, based on these structure properties, the wellposedness close to a constant state can be proved by using fine energy estimates. The asymptotic decay of the solutions are also investigated.