A series of materials Ce0.3+xZr0.6-xY0.1O1.95 were prepared by co-precipitation routine and the property of these materials was studied by means of oxygen storage capacity, temperature programming reduction, X-ray dif...A series of materials Ce0.3+xZr0.6-xY0.1O1.95 were prepared by co-precipitation routine and the property of these materials was studied by means of oxygen storage capacity, temperature programming reduction, X-ray diffraction, transmission electronic microscope, and X-ray photoelectron spectroscopy. The results indicate that the materials with a low Ce/Zr molar ratio possess higher cerium atom utilization ratio, reducibility and thermal stability than the materials with a high Ce/Zr ratio, and Ce0.35Zr0.55Y0.1O1.95 possesses the best properties.展开更多
The dynamic coupling effects on fusion cross sections for reactions^(32)S + ^(94,96)Zr and ^(40)Ca + ^(94,96)Zr are studied with the universal fusion function formalism and an empirical coupled channel(ECC) model. An ...The dynamic coupling effects on fusion cross sections for reactions^(32)S + ^(94,96)Zr and ^(40)Ca + ^(94,96)Zr are studied with the universal fusion function formalism and an empirical coupled channel(ECC) model. An examination of the reduced fusion functions shows that the total effect of couplings to inelastic excitations and neutron transfer channels on fusion in ^(32)S +^(94)Zr(^(40)Ca +^(94)Zr) is almost the same as that in ^(32)S +^(96)Zr(^(40)Ca +^(96)Zr). The enhancements of the fusion cross section at sub-barrier energies due to inelastic channel coupling and neutron transfer channel coupling are evaluated separately by using the ECC model. The results show that effect of couplings to inelastic excitations channels in the reactions with94 Zr as target should be similar as that in the reactions with ^(96) Zr as target. This implies that the quadrupole deformation parameters β_2of ^(94)Zr and^(96) Zr should be similar to each other.However, β_2 's predicted from the finite-range droplet model, which are used in the ECC model, are quite different. Experiments on^(48) Ca +^(94)Zr or^(36) S +^(94)Zr are suggested to solve the puzzling issue concerning β_2for^(94)Zr.展开更多
文摘A series of materials Ce0.3+xZr0.6-xY0.1O1.95 were prepared by co-precipitation routine and the property of these materials was studied by means of oxygen storage capacity, temperature programming reduction, X-ray diffraction, transmission electronic microscope, and X-ray photoelectron spectroscopy. The results indicate that the materials with a low Ce/Zr molar ratio possess higher cerium atom utilization ratio, reducibility and thermal stability than the materials with a high Ce/Zr ratio, and Ce0.35Zr0.55Y0.1O1.95 possesses the best properties.
基金supported by the National Key Basic Research Program of China(Grant No.2013CB834400)the National Natural Science Foundation of China(Grant Nos.11175252+4 种基金111201010051127524811475115and 11525524)the Knowledge Innovation Project of the Chinese Academy of Sciences(Grant No.KJCX2-EW-N01)
文摘The dynamic coupling effects on fusion cross sections for reactions^(32)S + ^(94,96)Zr and ^(40)Ca + ^(94,96)Zr are studied with the universal fusion function formalism and an empirical coupled channel(ECC) model. An examination of the reduced fusion functions shows that the total effect of couplings to inelastic excitations and neutron transfer channels on fusion in ^(32)S +^(94)Zr(^(40)Ca +^(94)Zr) is almost the same as that in ^(32)S +^(96)Zr(^(40)Ca +^(96)Zr). The enhancements of the fusion cross section at sub-barrier energies due to inelastic channel coupling and neutron transfer channel coupling are evaluated separately by using the ECC model. The results show that effect of couplings to inelastic excitations channels in the reactions with94 Zr as target should be similar as that in the reactions with ^(96) Zr as target. This implies that the quadrupole deformation parameters β_2of ^(94)Zr and^(96) Zr should be similar to each other.However, β_2 's predicted from the finite-range droplet model, which are used in the ECC model, are quite different. Experiments on^(48) Ca +^(94)Zr or^(36) S +^(94)Zr are suggested to solve the puzzling issue concerning β_2for^(94)Zr.
