China has experienced severe haze and visibility degradation problems in recent years because of rapid urbanization and industrialization.In this study,daily atmospheric fine-aerosol samples were concurrently collecte...China has experienced severe haze and visibility degradation problems in recent years because of rapid urbanization and industrialization.In this study,daily atmospheric fine-aerosol samples were concurrently collected at three sites over the Pearl River Delta(PRD)region during 1–29 October 2014.PM2.5 samples were analyzed for organic carbon and elemental carbon using a thermal/optical carbon analyzer.Major water-soluble inorganic ions including F−,Cl−,NO3−,SO42−,Na+,NH4+,K+,Mg2+,and Ca2+were analyzed by ion chromatography.The results show that the temporal variations of PM2.5 concentration at the three sites were highly parallel,with particle pollution events simultaneously observed during 13–19 October(EP1)and 23–27 October(EP2),suggesting that pollution events in the PRD region are usually regional.This can most likely be attributed to the significant influences of synoptic conditions,which regionally facilitate or block diffusion of air pollutants.The chemical compositions of PM2.5 at the three sites were also found to be similar,dominated by organics and sulfates.The results indicate that accumulation of traffic emissions seems to play important roles in particle pollution for the PRD region,leading in this case to elevated nitrate contributions during both EP1 and EP2 at the three sites.Moreover,the authors found that locally emitted aerosols from biomass burning only markedly influenced the air condition at one site,Nanhai,during EP1,while regionally transported biomass burning aerosols from eastern and northern Guangdong Province influenced all three sampling sites when the PRD was dominated by polluted air from these directions during EP2.展开更多
In recent years, with the acceleration of urbanization, medium-sized cities face increasingly severe, fog and haze increase, the heavy air pollution concentration, which caused acute health problems such as irritation...In recent years, with the acceleration of urbanization, medium-sized cities face increasingly severe, fog and haze increase, the heavy air pollution concentration, which caused acute health problems such as irritation and cardiovascular diseases caused widespread concern in the community. Most scholars believe that the haze is toxic and harmful gases; particulate matter and other pollutants together lead to reduced visibility as the main manifestation of the phenomenon of air pollution. Population health effects caused by the haze have been proven in many studies. The system summarizes the polluting haze weather physicochemical characteristics, introduced widely accepted definition of haze, haze hazard to residents and the proposed requirements.展开更多
基金This work was supported by the National Key Research and Development Program of China[grant numbers 2017YFC0210104 and 2016YFC0203305]the National Natural Science Foundation of China[grant numbers 41875152,41530641,and 41630422]+1 种基金the Special Fund Project for Science and Technology Innovation Strategy of Guangdong Province[Grant No.2019B121205004]the Fundamental Research Funds for the Central Universities[grant number 19lgpy26].
文摘China has experienced severe haze and visibility degradation problems in recent years because of rapid urbanization and industrialization.In this study,daily atmospheric fine-aerosol samples were concurrently collected at three sites over the Pearl River Delta(PRD)region during 1–29 October 2014.PM2.5 samples were analyzed for organic carbon and elemental carbon using a thermal/optical carbon analyzer.Major water-soluble inorganic ions including F−,Cl−,NO3−,SO42−,Na+,NH4+,K+,Mg2+,and Ca2+were analyzed by ion chromatography.The results show that the temporal variations of PM2.5 concentration at the three sites were highly parallel,with particle pollution events simultaneously observed during 13–19 October(EP1)and 23–27 October(EP2),suggesting that pollution events in the PRD region are usually regional.This can most likely be attributed to the significant influences of synoptic conditions,which regionally facilitate or block diffusion of air pollutants.The chemical compositions of PM2.5 at the three sites were also found to be similar,dominated by organics and sulfates.The results indicate that accumulation of traffic emissions seems to play important roles in particle pollution for the PRD region,leading in this case to elevated nitrate contributions during both EP1 and EP2 at the three sites.Moreover,the authors found that locally emitted aerosols from biomass burning only markedly influenced the air condition at one site,Nanhai,during EP1,while regionally transported biomass burning aerosols from eastern and northern Guangdong Province influenced all three sampling sites when the PRD was dominated by polluted air from these directions during EP2.
文摘In recent years, with the acceleration of urbanization, medium-sized cities face increasingly severe, fog and haze increase, the heavy air pollution concentration, which caused acute health problems such as irritation and cardiovascular diseases caused widespread concern in the community. Most scholars believe that the haze is toxic and harmful gases; particulate matter and other pollutants together lead to reduced visibility as the main manifestation of the phenomenon of air pollution. Population health effects caused by the haze have been proven in many studies. The system summarizes the polluting haze weather physicochemical characteristics, introduced widely accepted definition of haze, haze hazard to residents and the proposed requirements.