Raman lasers based on potassium gadolinium tungstate and lead tungstate crystals pumped by a≈120 ps Nd: YAG laser at 1.064/μm were developed. High reflection mirrors for the Stokes wavelength have been used to gener...Raman lasers based on potassium gadolinium tungstate and lead tungstate crystals pumped by a≈120 ps Nd: YAG laser at 1.064/μm were developed. High reflection mirrors for the Stokes wavelength have been used to generate near-infrared and eye safe spectral region of 1.15 - 1.32/μm. Second harmonic generation of the generated Raman lasers was observed. Eifficient multiple Stokes and anti-Stokes picosecond generation in 64 crystals have been shown to exhibit stimulated Raman scattering on about 700 lines covering the whole visible and near-infrared spectrum. All stimulated Raman scattering (SRS) wavelengths in the visible and near-infrared spectrum are identified and attributed to the SRS-active vibration modes of these crystals.展开更多
We present a comparative study on the C-H stretching vibrations at air/DMSO （dimethyl sulfoxide） interface with both the free-induction decay （FID） coherent vibrational dynamics and the sub-wavenumber high resolut...We present a comparative study on the C-H stretching vibrations at air/DMSO （dimethyl sulfoxide） interface with both the free-induction decay （FID） coherent vibrational dynamics and the sub-wavenumber high resolution sum-frequency generation vibrational spectroscopy measurements. In principle the frequency-domain and time-domain spectroscopic measurements should generate identical information for a given molecular system. However, when the molecular systems are with several coupled or overlapping vibrational modes, obtain- ing detailed spectroscopic and coherent dynamics information is not as straightforward and rather difficult from either the time-domain or the frequency domain measurements. For the case of air/DMSO interface that is with moderately complex vibrational spectra, we show that the frequency-domain measurement with sub-wavenumber high-resolution sum-frequency generation vibrational spectroscopy is probably more advantageous than the time- domain measurement in obtaining quantitative understanding of the structure and coherent dynamics of the molecular interface.展开更多
Shaping either the spatial or the spectral output of a nonlinear interaction is accomplished by introducing basic concepts of computer-generated holography into the nonlinear optics regime. The possibilities of arbitr...Shaping either the spatial or the spectral output of a nonlinear interaction is accomplished by introducing basic concepts of computer-generated holography into the nonlinear optics regime. The possibilities of arbitrarily spatially shaping the result of a nonlinear interaction are presented for different phase-matching schemes allowing for both one- and two-dimensional shaping. Shaping the spectrum of a beam in nonlinear interaction is also possible by utilizing similar holographic techniques. The novel and complete control of the output of a nonlinear interaction opens exciting options in the fields of particle manipulation, optical communications, spectroscopy and quantum information.展开更多
The absorption spectra and the refractive index changes are calculated theoretically for an exeiton in a core/shell quantum dot. The advantage of our methodology is that one can investigate the influence of the repuls...The absorption spectra and the refractive index changes are calculated theoretically for an exeiton in a core/shell quantum dot. The advantage of our methodology is that one can investigate the influence of the repulsive core by varying two parameters in the confinement potential. The dimensionality effect of exciton quantum dots on the optical absorptions has been studied. It has been found that in the same regime, the optical absorption intensities of excitons axe much smaller for the core/shell quantum dots than for the two-dimensional quantum rings. The linear and the nonlinear optical absorption coefficients and refractive index changes have been examined with the change of the confinement potential. The results show that the optical absorptions and the refractive index changes are strongly affected by the repulsive core of core/shell quantum dots. Moreover, the calculated results also reveal that as the inner radius increases, the peak values of the absorption coefficients and the refractive index changes of an exciton will show the optical Aharonov-Bohm oscillation in core/shell quantum dots.展开更多
In the present paper, the author studies the existence of sign-changing solutions for nonlinear elliptic equations, which have jumping nonlinearities, and may or may not be resonant with respect to Fucik spectrum, via...In the present paper, the author studies the existence of sign-changing solutions for nonlinear elliptic equations, which have jumping nonlinearities, and may or may not be resonant with respect to Fucik spectrum, via linking methods under Cerami condition.展开更多
文摘Raman lasers based on potassium gadolinium tungstate and lead tungstate crystals pumped by a≈120 ps Nd: YAG laser at 1.064/μm were developed. High reflection mirrors for the Stokes wavelength have been used to generate near-infrared and eye safe spectral region of 1.15 - 1.32/μm. Second harmonic generation of the generated Raman lasers was observed. Eifficient multiple Stokes and anti-Stokes picosecond generation in 64 crystals have been shown to exhibit stimulated Raman scattering on about 700 lines covering the whole visible and near-infrared spectrum. All stimulated Raman scattering (SRS) wavelengths in the visible and near-infrared spectrum are identified and attributed to the SRS-active vibration modes of these crystals.
文摘We present a comparative study on the C-H stretching vibrations at air/DMSO （dimethyl sulfoxide） interface with both the free-induction decay （FID） coherent vibrational dynamics and the sub-wavenumber high resolution sum-frequency generation vibrational spectroscopy measurements. In principle the frequency-domain and time-domain spectroscopic measurements should generate identical information for a given molecular system. However, when the molecular systems are with several coupled or overlapping vibrational modes, obtain- ing detailed spectroscopic and coherent dynamics information is not as straightforward and rather difficult from either the time-domain or the frequency domain measurements. For the case of air/DMSO interface that is with moderately complex vibrational spectra, we show that the frequency-domain measurement with sub-wavenumber high-resolution sum-frequency generation vibrational spectroscopy is probably more advantageous than the time- domain measurement in obtaining quantitative understanding of the structure and coherent dynamics of the molecular interface.
基金supported by the Israel Science Foundation(1310/13)the Israeli Ministry of Science,Technology and Space in the framework of the Israel–Italy bi-national collaboration program
文摘Shaping either the spatial or the spectral output of a nonlinear interaction is accomplished by introducing basic concepts of computer-generated holography into the nonlinear optics regime. The possibilities of arbitrarily spatially shaping the result of a nonlinear interaction are presented for different phase-matching schemes allowing for both one- and two-dimensional shaping. Shaping the spectrum of a beam in nonlinear interaction is also possible by utilizing similar holographic techniques. The novel and complete control of the output of a nonlinear interaction opens exciting options in the fields of particle manipulation, optical communications, spectroscopy and quantum information.
文摘The absorption spectra and the refractive index changes are calculated theoretically for an exeiton in a core/shell quantum dot. The advantage of our methodology is that one can investigate the influence of the repulsive core by varying two parameters in the confinement potential. The dimensionality effect of exciton quantum dots on the optical absorptions has been studied. It has been found that in the same regime, the optical absorption intensities of excitons axe much smaller for the core/shell quantum dots than for the two-dimensional quantum rings. The linear and the nonlinear optical absorption coefficients and refractive index changes have been examined with the change of the confinement potential. The results show that the optical absorptions and the refractive index changes are strongly affected by the repulsive core of core/shell quantum dots. Moreover, the calculated results also reveal that as the inner radius increases, the peak values of the absorption coefficients and the refractive index changes of an exciton will show the optical Aharonov-Bohm oscillation in core/shell quantum dots.
基金Project supported by the National Natural Science Foundation of China(No.10571123)the Shandong Provincial Natural Science Foundation of China(No.Y2006A04).
文摘In the present paper, the author studies the existence of sign-changing solutions for nonlinear elliptic equations, which have jumping nonlinearities, and may or may not be resonant with respect to Fucik spectrum, via linking methods under Cerami condition.
