In the light of the needs to develop high-performance heat transfer component for nation-level large-scale scientific projects of China,a hypervapotron experimental platform with supply of heat flux 1 10 MW m-2 was es...In the light of the needs to develop high-performance heat transfer component for nation-level large-scale scientific projects of China,a hypervapotron experimental platform with supply of heat flux 1 10 MW m-2 was established.With this platform,the multiphase flow and heat transfer phenomena on the surface of triangular fin when the subcooled water flowed through were observed and measured with the planar laser induced fluorescence(PLIF) and high-speed photography techniques.The temperature contour on the slice plane of fin symmetry was measured and the heat flux contour was processed based on gradient computation.It is confirmed that:1) PLIF with high-speed photography is very powerful technique to investigate the multiphase flow of hypervapotron quantitatively;2) evaporation is the primary way in heat transfer mechanism of hypervapotron flow under the condition of high heat flux.The techniques and results obtained will provide useful reference in the R&D of hypervapotron technology in China.展开更多
Based on the coherence theory of diffracted optical field and the model for partially coherent beams,analytical expressions for the cross-spectral density and the irradiance spectral density in the far zone are derive...Based on the coherence theory of diffracted optical field and the model for partially coherent beams,analytical expressions for the cross-spectral density and the irradiance spectral density in the far zone are derived,respectively.Utilizing the theoretical model of radiation from secondary planar sources,the physical conditions for sources generating a cosh-Gaussian(CHG) beam are investigated.Analytical results demonstrate that the parametric conditions strongly depend on the coherence property of sources.When almost coherence property is satisfied in the source plane,the conditions are the same as those for fundamental Gaussian beams;when partial coherence or almost incoherence property is satisfied in the spatial source plane,the conditions are the same as those for Gaussian-Schell model beams.The results also indicate that the variance of cosine parameters has no influence on the conditions.Our results may provide potential applications for some investigations such as the modulations of cosh-Gaussian beams and the designs of source beam parameters.展开更多
We demonstrated an efficient solar photovoltaic-powered electrochemical CO_(2) reduction device with a high-pressure CO_(2)-captured liquid feed.In an“air-to-barrel”picture,this device holds promise to avoid both hi...We demonstrated an efficient solar photovoltaic-powered electrochemical CO_(2) reduction device with a high-pressure CO_(2)-captured liquid feed.In an“air-to-barrel”picture,this device holds promise to avoid both high-temperature gaseous CO_(2) regeneration and high energy-cost gas product separation steps,while these steps are necessary for devices with a gaseous CO_(2) feed.To date,solar fuel production with a CO_(2)-saturated liquid feed suffers from high over-potential to suppress the hydrogen evolution reaction and consequently,low solar-to-chemical(STC)energy conversion efficiency.Here,we presented a distinct high-pressure operando strategy,i.e.,we took extra advantage of the high pressure in catalyst synthesis besides in the period of the CO_(2) reduction reaction(CO_(2)RR).The power of this strategy was demonstrated by a proof-of-concept device in which a representative copper catalyst was first synthesized in operando in a high-pressure(50 bar)CO_(2)-saturated KHCO3 solution,and then this high-pressure CO_(2)-captured liquid was converted to solar fuel using the operando synthesized Cu catalyst.This Cu catalyst achieved 95%CO_(2)RR selectivity at the recorded low potential of−0.3 V vs.RHE enabled by the combination of operando facet engineering and oxide derivation.Furthermore,this device achieved a record-high STC efficiency of 21.6%under outdoor illumination,superior to other CO_(2)-saturated liquid-fed devices,and compared favorably to gaseous CO_(2)-fed devices.展开更多
基金supported by the Fundamental Research Funds for the Central Universities of Chinathe National Magnetic Confined Fusion Energy Program of China (Grant No. 2009GB104005)
文摘In the light of the needs to develop high-performance heat transfer component for nation-level large-scale scientific projects of China,a hypervapotron experimental platform with supply of heat flux 1 10 MW m-2 was established.With this platform,the multiphase flow and heat transfer phenomena on the surface of triangular fin when the subcooled water flowed through were observed and measured with the planar laser induced fluorescence(PLIF) and high-speed photography techniques.The temperature contour on the slice plane of fin symmetry was measured and the heat flux contour was processed based on gradient computation.It is confirmed that:1) PLIF with high-speed photography is very powerful technique to investigate the multiphase flow of hypervapotron quantitatively;2) evaporation is the primary way in heat transfer mechanism of hypervapotron flow under the condition of high heat flux.The techniques and results obtained will provide useful reference in the R&D of hypervapotron technology in China.
文摘Based on the coherence theory of diffracted optical field and the model for partially coherent beams,analytical expressions for the cross-spectral density and the irradiance spectral density in the far zone are derived,respectively.Utilizing the theoretical model of radiation from secondary planar sources,the physical conditions for sources generating a cosh-Gaussian(CHG) beam are investigated.Analytical results demonstrate that the parametric conditions strongly depend on the coherence property of sources.When almost coherence property is satisfied in the source plane,the conditions are the same as those for fundamental Gaussian beams;when partial coherence or almost incoherence property is satisfied in the spatial source plane,the conditions are the same as those for Gaussian-Schell model beams.The results also indicate that the variance of cosine parameters has no influence on the conditions.Our results may provide potential applications for some investigations such as the modulations of cosh-Gaussian beams and the designs of source beam parameters.
基金supported by the National Natural Science Foundation of China(51888103,52006103,51976090,and 52006101)Scientific and Technological Innovation Project of Carbon Emission Peak and Carbon Neutrality of Jiangsu Province(BE2022024)+1 种基金Natural Science Foundation of Jiangsu Province(BK20200072,BK20200491,and BK20200500)China Postdoctoral Science Foundation(2020M681603)。
文摘We demonstrated an efficient solar photovoltaic-powered electrochemical CO_(2) reduction device with a high-pressure CO_(2)-captured liquid feed.In an“air-to-barrel”picture,this device holds promise to avoid both high-temperature gaseous CO_(2) regeneration and high energy-cost gas product separation steps,while these steps are necessary for devices with a gaseous CO_(2) feed.To date,solar fuel production with a CO_(2)-saturated liquid feed suffers from high over-potential to suppress the hydrogen evolution reaction and consequently,low solar-to-chemical(STC)energy conversion efficiency.Here,we presented a distinct high-pressure operando strategy,i.e.,we took extra advantage of the high pressure in catalyst synthesis besides in the period of the CO_(2) reduction reaction(CO_(2)RR).The power of this strategy was demonstrated by a proof-of-concept device in which a representative copper catalyst was first synthesized in operando in a high-pressure(50 bar)CO_(2)-saturated KHCO3 solution,and then this high-pressure CO_(2)-captured liquid was converted to solar fuel using the operando synthesized Cu catalyst.This Cu catalyst achieved 95%CO_(2)RR selectivity at the recorded low potential of−0.3 V vs.RHE enabled by the combination of operando facet engineering and oxide derivation.Furthermore,this device achieved a record-high STC efficiency of 21.6%under outdoor illumination,superior to other CO_(2)-saturated liquid-fed devices,and compared favorably to gaseous CO_(2)-fed devices.