We show that by scanning the frequency of a single mode infrared （IR） optical parametric oscillator （IR- OPO） laser to excite the molecular species of interest and fixing the frequency of a vacuum ultraviolet （VU...We show that by scanning the frequency of a single mode infrared （IR） optical parametric oscillator （IR- OPO） laser to excite the molecular species of interest and fixing the frequency of a vacuum ultraviolet （VUV） laser to photoionize the IR excited species, high-resolution IR spectra of polyatomic neutrals can be obtained with high sensitivity. The fact that this IR-VUV-photoion （IR-VUV-PI） method is based on VUV photoionization probe, and thus, allows the identification of the neutral IR absorber, makes it applicable for IR spectroscopy measurements of isotopemers, radicals, and clusters, which usually exist as impure samples. The highly resolved IR-VUV-PI measurements achieved using the single mode IR-OPO laser have made possible the selection of single rovibrational states of CH3X （X=Br and I）, C2H4, and C3H4 for VUV-pulsed field ionization-photoelectron （VUV-PFI-PE） measurements, resulting in rovibrationally resolved photoelectron spectra for these polyatomic molecules. These experiments show that the signal- to-noise ratios of the IR-VUV-PI and IR-VUV-PFI-PE spectra obtained by employing the high-resolution IR-OPO laser are significantly higher than those observed in previous IR-VUV-PI and IR-VUV-PFI-PE studies using a low-resolution IR-OPO laser. Further improvement in sensitivity of IR-VUV-PI and IR- VUV-PFI-PE measurements by using the collinear arrangement of IR-VUV lasers and molecular beam is discussed.展开更多
We study the absorption probability and Hawking radiation of the scalar field in a d-dimensional black hole with quantum correction arising from the polymer quantization. We find that the quantum length scale k （i.e....We study the absorption probability and Hawking radiation of the scalar field in a d-dimensional black hole with quantum correction arising from the polymer quantization. We find that the quantum length scale k （i.e., the bounce radius） modifies the standard results in greybody factors and Hawking radiation on the brahe and into the bulk. For the black hole with the larger mass M the effects of the parameter k in the four-dimensional black hole spacetime are entirely different from those in the high dimensional cases. When the mass of black hole M becomes very small, we also find that only the sign of the change rate of the greybody factors on the brahe with respect to the dimensional number depends sharply on the bounce radius k. These information can help us know more about the extra dimension and the black holes with quantum correction.展开更多
文摘We show that by scanning the frequency of a single mode infrared （IR） optical parametric oscillator （IR- OPO） laser to excite the molecular species of interest and fixing the frequency of a vacuum ultraviolet （VUV） laser to photoionize the IR excited species, high-resolution IR spectra of polyatomic neutrals can be obtained with high sensitivity. The fact that this IR-VUV-photoion （IR-VUV-PI） method is based on VUV photoionization probe, and thus, allows the identification of the neutral IR absorber, makes it applicable for IR spectroscopy measurements of isotopemers, radicals, and clusters, which usually exist as impure samples. The highly resolved IR-VUV-PI measurements achieved using the single mode IR-OPO laser have made possible the selection of single rovibrational states of CH3X （X=Br and I）, C2H4, and C3H4 for VUV-pulsed field ionization-photoelectron （VUV-PFI-PE） measurements, resulting in rovibrationally resolved photoelectron spectra for these polyatomic molecules. These experiments show that the signal- to-noise ratios of the IR-VUV-PI and IR-VUV-PFI-PE spectra obtained by employing the high-resolution IR-OPO laser are significantly higher than those observed in previous IR-VUV-PI and IR-VUV-PFI-PE studies using a low-resolution IR-OPO laser. Further improvement in sensitivity of IR-VUV-PI and IR- VUV-PFI-PE measurements by using the collinear arrangement of IR-VUV lasers and molecular beam is discussed.
基金Supported by the National Natural Science Foundation of China under Grant No. 11275065the NCET under Grant No. 10-0165+1 种基金the PCSIRT under Grant No. IRT0964the construct program of key disciplines in Hunan Province
文摘We study the absorption probability and Hawking radiation of the scalar field in a d-dimensional black hole with quantum correction arising from the polymer quantization. We find that the quantum length scale k （i.e., the bounce radius） modifies the standard results in greybody factors and Hawking radiation on the brahe and into the bulk. For the black hole with the larger mass M the effects of the parameter k in the four-dimensional black hole spacetime are entirely different from those in the high dimensional cases. When the mass of black hole M becomes very small, we also find that only the sign of the change rate of the greybody factors on the brahe with respect to the dimensional number depends sharply on the bounce radius k. These information can help us know more about the extra dimension and the black holes with quantum correction.
