The exchanges of NOx between snow and air have significant impact on the atmospheric components and photochemical processes in the overlying boundary layer. Such exchanges increase the oxidizing capacity of the atmosp...The exchanges of NOx between snow and air have significant impact on the atmospheric components and photochemical processes in the overlying boundary layer. Such exchanges increase the oxidizing capacity of the atmosphere and may have a crucial impact on the air signals that are retrieved from ice cores. In the recent years, sunlit snow and ice have been demonstrated to be important NOx sources in the polar atmospheric boundary layer. This paper makes a thorough review on the release of NOx from snow and ice, including field observations and experimental evidences, release mechanisms and influential parameters that affect such a release process, polar NOx concentrations and fluxes, and environmental impacts of the chemical processes of NOx in the polar atmospheric boundary layer. In the Tibetan Plateau, the released NOx observed recently in the sunlit snow/ice-cover is 1-order magnitude more than that in polar regions, but further scientific research is still needed to reveal its impact on the atmospheric oxidizing capacity.展开更多
A dipole pattern of summer precipitation over the mid-high latitudes of Asia, which is characterized by opposing summer precipitation variations between the Mongolian and Northeast China(MNC) region and the West Siber...A dipole pattern of summer precipitation over the mid-high latitudes of Asia, which is characterized by opposing summer precipitation variations between the Mongolian and Northeast China(MNC) region and the West Siberian Plain(WSP), is found to be clear and stable on both interdecadal and interannual scales during 1981–2011. Spring snow cover anomalies over a small region within the WSP and the Heilongjiang River(HR) region are closely related to the variation of this dipole mode during the subsequent summer, and they can therefore be considered as forecasting factors. Our statistical results imply a potential process explaining the relationship between the spring snow anomalies and the summer rainfall dipole. Corresponding to the snow anomalies, Rossby waves propagate along a path from the WSP region, via the Mongolian Plateau, to the Stanovoy Range during summer. At the same time, Rossby-wave energy divergences and convergences along this path maintain and reinforce an anomalous cyclone and anticyclone pairing over the Asian continent, which is significantly linked to opposite summer precipitation anomalies between the MNC and WSP regions. Numerical experiments are needed to further confirm the above conjecture and demonstrate the detailed physical mechanisms linking the spring snow cover anomalies and summer precipitation dipole.展开更多
基金supported by the Fund of Polar Scientific Research(No.20080216) of State Ocean Administration, Chinaby Chinese Natural Science Foundation(No. 20407001,No.40701170)
文摘The exchanges of NOx between snow and air have significant impact on the atmospheric components and photochemical processes in the overlying boundary layer. Such exchanges increase the oxidizing capacity of the atmosphere and may have a crucial impact on the air signals that are retrieved from ice cores. In the recent years, sunlit snow and ice have been demonstrated to be important NOx sources in the polar atmospheric boundary layer. This paper makes a thorough review on the release of NOx from snow and ice, including field observations and experimental evidences, release mechanisms and influential parameters that affect such a release process, polar NOx concentrations and fluxes, and environmental impacts of the chemical processes of NOx in the polar atmospheric boundary layer. In the Tibetan Plateau, the released NOx observed recently in the sunlit snow/ice-cover is 1-order magnitude more than that in polar regions, but further scientific research is still needed to reveal its impact on the atmospheric oxidizing capacity.
基金the joint support of the National Natural Science Foundation of China (Grant No. 41375090)the Basic Research Fund of the Chinese Academy of Meteorological Sciences (Grant No. 2013Z002)the International Cooperation and Exchange of the Ministry of Science and Technology of China (Grant No. 2009DFA21430)
文摘A dipole pattern of summer precipitation over the mid-high latitudes of Asia, which is characterized by opposing summer precipitation variations between the Mongolian and Northeast China(MNC) region and the West Siberian Plain(WSP), is found to be clear and stable on both interdecadal and interannual scales during 1981–2011. Spring snow cover anomalies over a small region within the WSP and the Heilongjiang River(HR) region are closely related to the variation of this dipole mode during the subsequent summer, and they can therefore be considered as forecasting factors. Our statistical results imply a potential process explaining the relationship between the spring snow anomalies and the summer rainfall dipole. Corresponding to the snow anomalies, Rossby waves propagate along a path from the WSP region, via the Mongolian Plateau, to the Stanovoy Range during summer. At the same time, Rossby-wave energy divergences and convergences along this path maintain and reinforce an anomalous cyclone and anticyclone pairing over the Asian continent, which is significantly linked to opposite summer precipitation anomalies between the MNC and WSP regions. Numerical experiments are needed to further confirm the above conjecture and demonstrate the detailed physical mechanisms linking the spring snow cover anomalies and summer precipitation dipole.
