3 D roll-forming for high strength steel sheets is a new technology at present.Double racks gear 3D roll forming machine developed by our research group can be used to perform variable cross section roll forming for h...3 D roll-forming for high strength steel sheets is a new technology at present.Double racks gear 3D roll forming machine developed by our research group can be used to perform variable cross section roll forming for high strength steel.In the paper,a dynamic model of 8-DOF double rack gear 3D roll-forming machine is established by the method of Lagrange equation.The expression of the angle acceleration of the system response is obtained by solving the dynamic equations.Through an actual engineering example,the dynamical characters of the 3D roll forming machine are revealed.The results can support the design of 3D roll forming machine.Meanwhile,the research will play an active role in the development of control system.展开更多
Several algorithms were proposed relating to the development of a framework of the perturbation-based stochastic finite element method (PSFEM) for large variation nonlinear dynamic problems. For this purpose, algorith...Several algorithms were proposed relating to the development of a framework of the perturbation-based stochastic finite element method (PSFEM) for large variation nonlinear dynamic problems. For this purpose, algorithms and a framework related to SFEM based on the stochastic virtual work principle were studied. To prove the validity and practicality of the algorithms and framework, numerical examples for nonlinear dynamic problems with large variations were calculated and compared with the Monte-Carlo Simulation method. This comparison shows that the proposed approaches are accurate and effective for the nonlinear dynamic analysis of structures with random parameters.展开更多
The flexible transparent supercapacitors have been considered as one of the key energy-storage components to power the smart portable electronic devices.However,it is still a challenge to explore flexible transparent ...The flexible transparent supercapacitors have been considered as one of the key energy-storage components to power the smart portable electronic devices.However,it is still a challenge to explore flexible transparent capacitive electrodes with high rate capability.Herein,conductive Ni3(HITP)2(HITP=2,3,6,7,10,11-hexaiminotriphenylene)thin films are adopted as capacitive electrodes in flexible transparent supercapacitors.The Ni3(HITP)2 electrode possesses the excellent optoelectronic property with optical transmittance(T)of 78.4%and sheet resistance(Rs)of 51.3Ωsq-1,remarkable areal capacitance(CA)of 1.63 mF cm^-2and highest scan rate up to 5000 mV s-1.The asymmetric Ni3(HITP)2//PEDOT:PSS supercapacitor(T=61%)yields a high CA of 1.06 mF cm^-2at 3μA cm-2,which maintains 77.4%as the current density increases by 50 folds.The remarkable rate capability is ascribed to the collaborative advantages of low diffusion resistance and high ion accessibility,resulting from the intrinsic conductivity,short oriented pores and large specific areas of Ni3(HITP)2 films.展开更多
Binding of fluorescent molecules to the porous matrix through noncovalent interactions will synergistically expand their application spectrum. In this regard, we report an integrative self-assembly of molecule 1 with ...Binding of fluorescent molecules to the porous matrix through noncovalent interactions will synergistically expand their application spectrum. In this regard, we report an integrative self-assembly of molecule 1 with benzothiadizole and 9,9-dihexyl fluorene units, and covalent organic frameworks(COFs) via an emulsion-modulated polymerization process, within which molecules of 1 are able to interact with the scaffolds of COFs through CH-π interactions. Thus the π-πinteractions between the fluorescent molecules are largely suppressed, giving rise to their remarkable monomer-like optical properties. Of particular interest is that, given by the specific interaction between COFs and a nerve agent simulant diethyl chlorophosphite(DCP), these assembled composites show the ability of ultrasensitive detection of DCP with a detection limit of ~40 ppb. Moreover, the present integrative assembly strategy can be extended to encapsulate multiple fluorescent molecules, enabling the assemblies with white light emission. Our results highlight opportunities for the development of highly emissive porous materials by molecular selfassembly of fluorophores and molecular units of COFs.展开更多
基金Supported by the National Science and Technology Supporting Plan Projects of China （No.2011BAG03B03）.
文摘3 D roll-forming for high strength steel sheets is a new technology at present.Double racks gear 3D roll forming machine developed by our research group can be used to perform variable cross section roll forming for high strength steel.In the paper,a dynamic model of 8-DOF double rack gear 3D roll-forming machine is established by the method of Lagrange equation.The expression of the angle acceleration of the system response is obtained by solving the dynamic equations.Through an actual engineering example,the dynamical characters of the 3D roll forming machine are revealed.The results can support the design of 3D roll forming machine.Meanwhile,the research will play an active role in the development of control system.
文摘Several algorithms were proposed relating to the development of a framework of the perturbation-based stochastic finite element method (PSFEM) for large variation nonlinear dynamic problems. For this purpose, algorithms and a framework related to SFEM based on the stochastic virtual work principle were studied. To prove the validity and practicality of the algorithms and framework, numerical examples for nonlinear dynamic problems with large variations were calculated and compared with the Monte-Carlo Simulation method. This comparison shows that the proposed approaches are accurate and effective for the nonlinear dynamic analysis of structures with random parameters.
基金supported by the National Natural Science Foundation of China(NSFC)(61804082,21671108,51473078,and 61935017)Synergetic Innovation Center for Organic Electronics and Information Displays and Projects of International Cooperation and Exchanges NSFC(51811530018)+4 种基金the China Postdoctoral Science Foundation funded project(2018M642286)National Program for Support of Top-Notch Young Professionals,Scientific and Technological Innovation Teams of Colleges and Universities in Jiangsu Province(TJ215006)Priority Academic Program Development of Jiangsu Higher Education Institutions(YX03001)Jiangsu Planned Projects for Postdoctoral Research Funds(2019K047A)Science Foundation of Nanjing University of Posts and Telecommunications(NY217142)。
文摘The flexible transparent supercapacitors have been considered as one of the key energy-storage components to power the smart portable electronic devices.However,it is still a challenge to explore flexible transparent capacitive electrodes with high rate capability.Herein,conductive Ni3(HITP)2(HITP=2,3,6,7,10,11-hexaiminotriphenylene)thin films are adopted as capacitive electrodes in flexible transparent supercapacitors.The Ni3(HITP)2 electrode possesses the excellent optoelectronic property with optical transmittance(T)of 78.4%and sheet resistance(Rs)of 51.3Ωsq-1,remarkable areal capacitance(CA)of 1.63 mF cm^-2and highest scan rate up to 5000 mV s-1.The asymmetric Ni3(HITP)2//PEDOT:PSS supercapacitor(T=61%)yields a high CA of 1.06 mF cm^-2at 3μA cm-2,which maintains 77.4%as the current density increases by 50 folds.The remarkable rate capability is ascribed to the collaborative advantages of low diffusion resistance and high ion accessibility,resulting from the intrinsic conductivity,short oriented pores and large specific areas of Ni3(HITP)2 films.
基金supported by the National Natural Science Foundation of China (21703120,21972076,51903140 and 21925604)China Postdoctoral Science Foundation (2019M662324)Taishan Scholars Program of Shandong Province (tsqn201812011)。
文摘Binding of fluorescent molecules to the porous matrix through noncovalent interactions will synergistically expand their application spectrum. In this regard, we report an integrative self-assembly of molecule 1 with benzothiadizole and 9,9-dihexyl fluorene units, and covalent organic frameworks(COFs) via an emulsion-modulated polymerization process, within which molecules of 1 are able to interact with the scaffolds of COFs through CH-π interactions. Thus the π-πinteractions between the fluorescent molecules are largely suppressed, giving rise to their remarkable monomer-like optical properties. Of particular interest is that, given by the specific interaction between COFs and a nerve agent simulant diethyl chlorophosphite(DCP), these assembled composites show the ability of ultrasensitive detection of DCP with a detection limit of ~40 ppb. Moreover, the present integrative assembly strategy can be extended to encapsulate multiple fluorescent molecules, enabling the assemblies with white light emission. Our results highlight opportunities for the development of highly emissive porous materials by molecular selfassembly of fluorophores and molecular units of COFs.
