Coal-based Magnetic Activated Carbons （CMAC＇s） were prepared from three representative coal samples of various ranks： Baorigele lignite from Inner Mongolia; Datong bitumite from Shanxi province; and Taixi anthraci...Coal-based Magnetic Activated Carbons （CMAC＇s） were prepared from three representative coal samples of various ranks： Baorigele lignite from Inner Mongolia; Datong bitumite from Shanxi province; and Taixi anthracite from Ningxia Hui Auto- nomous Region. Fe3O4 was used as a magnetic additive. A nitrogen-adsorption analyzer was used to determine the specific surface area and pore structure of the resulting activated carbons. The adsorption capacity was assessed by the adsorption of iodine and methylene blue. X-ray diffraction was used to measure the evolution behavior of Fe304 during the preparation process. Magnetic properties were characterized with a vibrating-sample magnetometer. The effect of the activation temperature on the performance of CMAC＇s was also studied. The results show that, compared to Baorigele lignite and Taixi anthracite, the Datong bitumite is more appropriate for the preparation of CMAC＇s with a high specific surface area, an advanced pore structure and suitable magnetic properties. Fe304 can effectively enhance the magnetic properties and control the pore structure by increasing the ratio of meso- pores. An addition of 6.0% Fe304 and an activation temperature of 880 ℃ produced a CMAC having a specific surface area, an iodine adsorption, a methylene blue adsorption and a specific saturation magnetization of 1152.0 m2/g, 1216.7 mg/g, 229.5 mg/g and 4.623 emu/g, respectively. The coal used to prepare this specimen was Datong bitumite.展开更多
Maritime-type glaciers in the eastern Nyainqêntanglha Range, located in the southeastern part of the Tibetan Plateau, are an important water source for downstream residents and ecological systems. To better under...Maritime-type glaciers in the eastern Nyainqêntanglha Range, located in the southeastern part of the Tibetan Plateau, are an important water source for downstream residents and ecological systems. To better understand the variability of glaciers in this region, we used the band ratio threshold（TM3/TM5 for the Landsat TM /ETM＋ and TM4/TM6 for Landsat OLI） to extract glacier outlines in ~1999 and ~2013. After that, we also generated a series of glacier boundaries and monitored glacier variations in the past 40 years with the help of the Chinese Glacier Inventory data（1975） and Landsat TM, ETM＋ and OLI data. The total glacier area decreased by 37.69 ± 2.84% from 1975 to 2013. The annual percentage area change（APAC） was ~1.32% a-1 and ~1.29% a-1 in the periods 1975-1999 and 1999-2013, respectively. According to the lag theory, the reaction time is probably about 10 years and we discuss the variations of temperature and precipitation between 1965 and 2011. Temperature and precipitation increased between 1965 and 2011 at a rate of 0.34°C /10 a and 15.4 mm/10 a, respectively. Extensive meteorological data show that the glacier shrinkage rate over the period may be mainly due to increasing air temperature, while the increasing precipitation partly made up for the mass loss of glacier ice resulting from increasing temperature may also lead to the low APAC between 1999 and 2013. The lag theory suggests that glacier shrinkage may accelerate in the next 10 years. Small glaciers were more sensitive to climate change, and there was a normal distribution between glacier area and elevation. Glaciers shrank in all aspects, and south aspects diminished faster than others.展开更多
Wetlands are sensitive to climate change, in the same time, wetlands can influence climate. This study analyzed the spa- rio-temporal characteristics of wetland change in the semi-arid zone of Northeast China from 198...Wetlands are sensitive to climate change, in the same time, wetlands can influence climate. This study analyzed the spa- rio-temporal characteristics of wetland change in the semi-arid zone of Northeast China from 1985 to 2010, and investigated the impact of large area of wetland change on local climate. Results showed that the total area of wetlands was on a rise in the study area. Although natural wetlands （marshes, riparians and lakes） decreased, constructed wetlands （rice fields） increased significantly, and the highest in- crease rate in many places exceeded 30%. Anthropogenic activities are major driving factors for wetland change. Wetland change pro- duced an impact on local climate, mainly on maximum temperature and precipitation during the period of May-September. The increase （or decrease） of wetland area could reduce （or increase） the increment of maximum temperature and the decrement of precipitation. The changes in both maximum temperature and precipitation corresponded with wetland change in spatial distribution. Wetland change played a more important role in moderating local climate compared to the contribution of woodland and grassland changes in the study area. Cold-humid effect of wetlands was main way to moderating local climate as well as alleviating climatic wanning and drying in the study area, and heterogeneity of underlying surface broadened the cold-humid effect of wetlands.展开更多
基金supported by the National Natural Science Foundation of China (No20776150)the National High Technology Research and Development Program of China (No2008AA05Z308)
文摘Coal-based Magnetic Activated Carbons （CMAC＇s） were prepared from three representative coal samples of various ranks： Baorigele lignite from Inner Mongolia; Datong bitumite from Shanxi province; and Taixi anthracite from Ningxia Hui Auto- nomous Region. Fe3O4 was used as a magnetic additive. A nitrogen-adsorption analyzer was used to determine the specific surface area and pore structure of the resulting activated carbons. The adsorption capacity was assessed by the adsorption of iodine and methylene blue. X-ray diffraction was used to measure the evolution behavior of Fe304 during the preparation process. Magnetic properties were characterized with a vibrating-sample magnetometer. The effect of the activation temperature on the performance of CMAC＇s was also studied. The results show that, compared to Baorigele lignite and Taixi anthracite, the Datong bitumite is more appropriate for the preparation of CMAC＇s with a high specific surface area, an advanced pore structure and suitable magnetic properties. Fe304 can effectively enhance the magnetic properties and control the pore structure by increasing the ratio of meso- pores. An addition of 6.0% Fe304 and an activation temperature of 880 ℃ produced a CMAC having a specific surface area, an iodine adsorption, a methylene blue adsorption and a specific saturation magnetization of 1152.0 m2/g, 1216.7 mg/g, 229.5 mg/g and 4.623 emu/g, respectively. The coal used to prepare this specimen was Datong bitumite.
基金supported by the National Science Foundation of China (Grant Nos. 41271024, 41411130204)
文摘Maritime-type glaciers in the eastern Nyainqêntanglha Range, located in the southeastern part of the Tibetan Plateau, are an important water source for downstream residents and ecological systems. To better understand the variability of glaciers in this region, we used the band ratio threshold（TM3/TM5 for the Landsat TM /ETM＋ and TM4/TM6 for Landsat OLI） to extract glacier outlines in ~1999 and ~2013. After that, we also generated a series of glacier boundaries and monitored glacier variations in the past 40 years with the help of the Chinese Glacier Inventory data（1975） and Landsat TM, ETM＋ and OLI data. The total glacier area decreased by 37.69 ± 2.84% from 1975 to 2013. The annual percentage area change（APAC） was ~1.32% a-1 and ~1.29% a-1 in the periods 1975-1999 and 1999-2013, respectively. According to the lag theory, the reaction time is probably about 10 years and we discuss the variations of temperature and precipitation between 1965 and 2011. Temperature and precipitation increased between 1965 and 2011 at a rate of 0.34°C /10 a and 15.4 mm/10 a, respectively. Extensive meteorological data show that the glacier shrinkage rate over the period may be mainly due to increasing air temperature, while the increasing precipitation partly made up for the mass loss of glacier ice resulting from increasing temperature may also lead to the low APAC between 1999 and 2013. The lag theory suggests that glacier shrinkage may accelerate in the next 10 years. Small glaciers were more sensitive to climate change, and there was a normal distribution between glacier area and elevation. Glaciers shrank in all aspects, and south aspects diminished faster than others.
基金Under the auspices of National Environmental Protection Public Welfare Industry Research Fund(No.2011467032)
文摘Wetlands are sensitive to climate change, in the same time, wetlands can influence climate. This study analyzed the spa- rio-temporal characteristics of wetland change in the semi-arid zone of Northeast China from 1985 to 2010, and investigated the impact of large area of wetland change on local climate. Results showed that the total area of wetlands was on a rise in the study area. Although natural wetlands （marshes, riparians and lakes） decreased, constructed wetlands （rice fields） increased significantly, and the highest in- crease rate in many places exceeded 30%. Anthropogenic activities are major driving factors for wetland change. Wetland change pro- duced an impact on local climate, mainly on maximum temperature and precipitation during the period of May-September. The increase （or decrease） of wetland area could reduce （or increase） the increment of maximum temperature and the decrement of precipitation. The changes in both maximum temperature and precipitation corresponded with wetland change in spatial distribution. Wetland change played a more important role in moderating local climate compared to the contribution of woodland and grassland changes in the study area. Cold-humid effect of wetlands was main way to moderating local climate as well as alleviating climatic wanning and drying in the study area, and heterogeneity of underlying surface broadened the cold-humid effect of wetlands.
