As a novel one-atom-thick carbon allotrope,graphdiyne(GDY)has attracted wide interest in two-dimensional materials owing to its unique feature with a planar layer comprising sp2-and sp-hybridized carbon atoms and a di...As a novel one-atom-thick carbon allotrope,graphdiyne(GDY)has attracted wide interest in two-dimensional materials owing to its unique feature with a planar layer comprising sp2-and sp-hybridized carbon atoms and a direct natural bandgap.A high-quality saturable absorber(SA)based on GDY was successfully fabricated,and the nonlinear saturable absorption properties were investigated.A compact diode-pumped solid-state passively Q-switched laser based on the as-prepared GDY-SA could be operated at 2µm.The Q-switched laser delivered a maximum average output power of 1.29 W at a central wavelength of 1908.41 nm with up to 54.8%slope efficiency.A repetition rate of 91.58 kHz and single pulse energy of 23.08µJ were obtained.This work is the first application of GDY as an SA to generate all-solid-state pulsed lasers.These results indicate that GDY is a promising SA for solid-state pulsed lasers and has further application potential for ultrafast photonic devices in the 2-µm region.展开更多
基金financially supported by the National Natural Science Foundation of China (11974220, 61635012,61875138, 61961136001, and U1801254)the State Key Research Development Program of China (2019YFB2203503)
文摘As a novel one-atom-thick carbon allotrope,graphdiyne(GDY)has attracted wide interest in two-dimensional materials owing to its unique feature with a planar layer comprising sp2-and sp-hybridized carbon atoms and a direct natural bandgap.A high-quality saturable absorber(SA)based on GDY was successfully fabricated,and the nonlinear saturable absorption properties were investigated.A compact diode-pumped solid-state passively Q-switched laser based on the as-prepared GDY-SA could be operated at 2µm.The Q-switched laser delivered a maximum average output power of 1.29 W at a central wavelength of 1908.41 nm with up to 54.8%slope efficiency.A repetition rate of 91.58 kHz and single pulse energy of 23.08µJ were obtained.This work is the first application of GDY as an SA to generate all-solid-state pulsed lasers.These results indicate that GDY is a promising SA for solid-state pulsed lasers and has further application potential for ultrafast photonic devices in the 2-µm region.
