The high harmonic generation (HHG) from the CS<sub>2</sub> molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital...The high harmonic generation (HHG) from the CS<sub>2</sub> molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS<sub>2</sub> molecule, which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the z-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover, an isolated 110 as pulse can be obtained by superposing the harmonics from 130th to 180th order.展开更多
The Edlén empirical equations and the two-color method are the commonly used approaches to converting a length measured in air to the corresponding length in vacuum to eliminate the influence of the refractive in...The Edlén empirical equations and the two-color method are the commonly used approaches to converting a length measured in air to the corresponding length in vacuum to eliminate the influence of the refractive index of air. However, it is not well known whether the two-color method is superior to empirical equations in refractive index compensation. We investigated the uncertainties of these approaches via numerical calculations of their sensitivity coefficients of environmental parameters. On the basis of a comparison of their uncertainties, we found that in a 0% humidity environment, the two-color method had potential to provide greater measurement accuracy than the empirical equations.展开更多
基金Supported by the National Natural Science Foundation of China under Grant Nos 11574117,11271158,61575077 and 11575071
文摘The high harmonic generation (HHG) from the CS<sub>2</sub> molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS<sub>2</sub> molecule, which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the z-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover, an isolated 110 as pulse can be obtained by superposing the harmonics from 130th to 180th order.
文摘The Edlén empirical equations and the two-color method are the commonly used approaches to converting a length measured in air to the corresponding length in vacuum to eliminate the influence of the refractive index of air. However, it is not well known whether the two-color method is superior to empirical equations in refractive index compensation. We investigated the uncertainties of these approaches via numerical calculations of their sensitivity coefficients of environmental parameters. On the basis of a comparison of their uncertainties, we found that in a 0% humidity environment, the two-color method had potential to provide greater measurement accuracy than the empirical equations.
