Quantum light sources are the core resources for photonics-based quantum information processing.We investigate the spectral engineering of photon triplets generated by third-order spontaneous parametric down-conversio...Quantum light sources are the core resources for photonics-based quantum information processing.We investigate the spectral engineering of photon triplets generated by third-order spontaneous parametric down-conversion in micro/nanofiber.The phase mismatching at one-third pump frequency gives rise to non-degenerate photon triplets,the joint spectral intensity of which has an elliptical locus with a fixed eccentricity of√6/3.Therefore,we propose a frequency-division scheme to separate non-degenerate photon triplets into three channels with high heralding efficiency for the first time.Choosing an appropriate pump wavelength can compensate for the fabrication errors of micro/nanofiber and also generate narrowband,non-degenerate photon triplet sources with a high signal-to-noise ratio.Furthermore,the long-period micro/nanofiber grating introduces a new controllable degree of freedom to tailor phase matching,resulting from the periodic oscillation of dispersion.In this scheme,the wavelength of photon triplets can be flexibly tuned using quasi-phase matching.We study the generation of photon triplets from this novel perspective of spectrum engineering,and we believe that this work will accelerate the practical implementation of photon triplets in quantum information processing.展开更多
Multidimensional integration and multifunctional com-ponent assembly have been greatly explored in recent years to extend Moore’s Law of modern microelectronics.However,this inevitably exac-erbates the inhomogeneity ...Multidimensional integration and multifunctional com-ponent assembly have been greatly explored in recent years to extend Moore’s Law of modern microelectronics.However,this inevitably exac-erbates the inhomogeneity of temperature distribution in microsystems,making precise temperature control for electronic components extremely challenging.Herein,we report an on-chip micro temperature controller including a pair of thermoelectric legs with a total area of 50×50μm^(2),which are fabricated from dense and flat freestanding Bi2Te3-based ther-moelectric nano films deposited on a newly developed nano graphene oxide membrane substrate.Its tunable equivalent thermal resistance is controlled by electrical currents to achieve energy-efficient temperature control for low-power electronics.A large cooling temperature difference of 44.5 K at 380 K is achieved with a power consumption of only 445μW,resulting in an ultrahigh temperature control capability over 100 K mW^(-1).Moreover,an ultra-fast cooling rate exceeding 2000 K s^(-1) and excellent reliability of up to 1 million cycles are observed.Our proposed on-chip temperature controller is expected to enable further miniaturization and multifunctional integration on a single chip for microelectronics.展开更多
Gas hydrate technology has considerable potential in many fields.However,due to the lack of understanding of the micro mechanism of hydrate formation,it has not been commercially applied so far.Gas hydrate formation i...Gas hydrate technology has considerable potential in many fields.However,due to the lack of understanding of the micro mechanism of hydrate formation,it has not been commercially applied so far.Gas hydrate formation is essentially a gas-liquid-solid phase transition of water and gas molecules at a certain temperature and pressure.The key to the hydrate formation is the transformation of water molecule from disordered arrangement to ordered arrangement.In this process,weakly hydrogen bonded water will be correspondingly converted to strongly hydrogen bonded water.Through in situ Raman analysis and experiments,the position change of the corresponding peaks of the strongly hydrogen bonded water and the weakly hydrogen bonded water was compared in this work,and the key microscopic process and influence of gas hydrate formation in different systems were comprehensively studied and summarized.It is found that,with the decrease of temperature,the OAH of the weakly hydrogen bonded water remains unchanged when the temperature drops to a certain value,which is the key to the transformation of water into cage hydrate rather than ice.The conversion from the weakly hydrogen bonded water to the strongly hydrogen bonded water is closely related to the gas-liquid interface force,the hydrophilicity/hydrophobicity of the promoter,the ionization degree of liquid,and the electrostatic field of the system.Among the four most common promoters,tetrahydrofuran(THF)has the highest efficiency in promoting methane(CH4)hydrate formation.Therefore,this study provides a scientific direction and basis for the development of high efficient hydrate formation promoters,which can effectively weaken the hydrogen bond of weakly hydrogen bonded water and promote the conversion of weakly hydrogen bonded water to strongly hydrogen bonded water.展开更多
A novel micro fused-casting(MFC)process is developed for semisolid aluminum alloy slurry.The microstructure evolution and properties of semisolid ZL101 aluminum alloy slurry with difierent pouring temperature by MFC a...A novel micro fused-casting(MFC)process is developed for semisolid aluminum alloy slurry.The microstructure evolution and properties of semisolid ZL101 aluminum alloy slurry with difierent pouring temperature by MFC are investigated in this paper.During the cooling process,the effects of the pouring temperature on microstructure and properties is primarily analyzed.The microstructure of the semisolid ZL101 aluminum alloy is more homogeneous and the grain is smaller under proper pouring temperature.Temperature of liquids and solids of ZL101 aluminum alloy is measured by difierential scanning calorimetry(DSC).Distribution and characteristics of the microstructure of samples are examined by optical microscope(OM),scanning electron microscopy(SEM)equipped with energy dispersive spectrometer(EDS).The results show that the ZL101 semisolid slurry fabricated by MFC presents uniform shape and good grain size under the pouring temperature of 594°C and the stirring velocity of 600 r/min,and the fine grains of the primary a-Al phase with average grain size of 55μm and shape factor up to 0.67 were obtained.Besides,the ultimate tensile strength and the average Vickers hardness for semisolid ZL101 aluminum slurry are 178.19±1.37 MPa and 86.15±1.16 HV,respectively.展开更多
利用全国40个地面台站的观测资料对ERA5及ERA5-Land两种不同空间分辨率的再分析资料开展了地面风速误差评估研究,结果表明:ERA5和ERA5-Land资料多年平均风速偏差的平均值分别为0.08 m s^(−1)、-0.06 m s^(−1),偏差的最大值分别为0.46 m ...利用全国40个地面台站的观测资料对ERA5及ERA5-Land两种不同空间分辨率的再分析资料开展了地面风速误差评估研究,结果表明:ERA5和ERA5-Land资料多年平均风速偏差的平均值分别为0.08 m s^(−1)、-0.06 m s^(−1),偏差的最大值分别为0.46 m s^(−1)、-0.19 m s^(−1),相对偏差的平均值为4.4%、-2.0%,相对偏差的最大值分别为33.0%、-10.1%;月平均风速线性拟合方程的斜率分别为0.93、0.97,截距分别为0.29 m s^(−1)、0.02 m s^(−1),相关系数分别为0.98、0.99;月平均风速均方根误差的平均值分别为0.17 m s^(−1)、0.14 m s^(−1),均方根误差的最大值分别为0.49 m s^(−1)、0.22 m s^(−1),相对均方根误差的平均值为7.4%、5.7%,相对均方根误差的最大值分别为35.2%、13.3%。ERA5-Land高分辨率资料地面风速误差相对较低,有利于提高风能资源评估的准确性。展开更多
提出一种高精度的ZWD模型(tianjin_zwd,TZ)。TZ基于2016-2018年逐小时气压分层的ERA5,欧洲中尺度气象预报中心第五代再分析产品数据,采用BP神经网络建立。然后,根据2019年的ERA5产品导出的ZWD对TZ模型进行了验证。结果表明:相比GPT3模型...提出一种高精度的ZWD模型(tianjin_zwd,TZ)。TZ基于2016-2018年逐小时气压分层的ERA5,欧洲中尺度气象预报中心第五代再分析产品数据,采用BP神经网络建立。然后,根据2019年的ERA5产品导出的ZWD对TZ模型进行了验证。结果表明:相比GPT3模型,TZ模型可提供更贴近真值的ZWD估值;并且,其RMSE由5.0 cm (GPT3)降至4.5 cm,表明10%的精度提升。上述结果表明TZ模型实现了更优的预测性能,该模型的构建策略可为全国其他地区的ZWD建模提供借鉴。展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.61605249)the Science and Technology Key Project of Henan Province of China(Grant Nos.182102210577 and 232102211086).
文摘Quantum light sources are the core resources for photonics-based quantum information processing.We investigate the spectral engineering of photon triplets generated by third-order spontaneous parametric down-conversion in micro/nanofiber.The phase mismatching at one-third pump frequency gives rise to non-degenerate photon triplets,the joint spectral intensity of which has an elliptical locus with a fixed eccentricity of√6/3.Therefore,we propose a frequency-division scheme to separate non-degenerate photon triplets into three channels with high heralding efficiency for the first time.Choosing an appropriate pump wavelength can compensate for the fabrication errors of micro/nanofiber and also generate narrowband,non-degenerate photon triplet sources with a high signal-to-noise ratio.Furthermore,the long-period micro/nanofiber grating introduces a new controllable degree of freedom to tailor phase matching,resulting from the periodic oscillation of dispersion.In this scheme,the wavelength of photon triplets can be flexibly tuned using quasi-phase matching.We study the generation of photon triplets from this novel perspective of spectrum engineering,and we believe that this work will accelerate the practical implementation of photon triplets in quantum information processing.
基金The authors thank D.Berger,D.Hofmann and C.Kupka in IFW Dresden for helpful technical support.H.R.acknowledges funding from the DFG(Deutsche Forschungsgemeinschaft)within grant number RE3973/1-1.Q.J.,H.R.and K.N.conceived the work.With the support from N.Y.and X.J.,Q.J.and T.G.fabricated the thermoelectric films and conducted the structural and compositional characterizations.Q.J.prepared microchips and fabricated the on-chip micro temperature controllers.Q.J.and N.P.carried out the temperature-dependent material and device performance measurements.Q.J.and H.R.performed the simulation and analytical calculations.Q.J.,H.R.and K.N.wrote the manuscript with input from the other coauthors.All the authors discussed the results and commented on the manuscript.
文摘Multidimensional integration and multifunctional com-ponent assembly have been greatly explored in recent years to extend Moore’s Law of modern microelectronics.However,this inevitably exac-erbates the inhomogeneity of temperature distribution in microsystems,making precise temperature control for electronic components extremely challenging.Herein,we report an on-chip micro temperature controller including a pair of thermoelectric legs with a total area of 50×50μm^(2),which are fabricated from dense and flat freestanding Bi2Te3-based ther-moelectric nano films deposited on a newly developed nano graphene oxide membrane substrate.Its tunable equivalent thermal resistance is controlled by electrical currents to achieve energy-efficient temperature control for low-power electronics.A large cooling temperature difference of 44.5 K at 380 K is achieved with a power consumption of only 445μW,resulting in an ultrahigh temperature control capability over 100 K mW^(-1).Moreover,an ultra-fast cooling rate exceeding 2000 K s^(-1) and excellent reliability of up to 1 million cycles are observed.Our proposed on-chip temperature controller is expected to enable further miniaturization and multifunctional integration on a single chip for microelectronics.
基金financial support from the Key Program of National Natural Science Foundation of China(51736009)the Natural Science Foundation of Guangdong Province,China(2023A1515012061)+3 种基金the Guangdong Special Support Program-Local innovation and entrepreneurship team project(2019BT02L278)the Special Project for Marine Economy Development of Guangdong Province(GDME-2022D043)the Fundamental Research&Applied Fundamental Research Major Project of Guangdong Province(2019B030302004,2020B030103003)the Science and Technology Apparatus Development Program of the Chinese Academy of Sciences(YZ201619),the Frontier Sciences Key Research Program of the Chinese Academy of Sciences(QYZDJSSW-JSC033)。
文摘Gas hydrate technology has considerable potential in many fields.However,due to the lack of understanding of the micro mechanism of hydrate formation,it has not been commercially applied so far.Gas hydrate formation is essentially a gas-liquid-solid phase transition of water and gas molecules at a certain temperature and pressure.The key to the hydrate formation is the transformation of water molecule from disordered arrangement to ordered arrangement.In this process,weakly hydrogen bonded water will be correspondingly converted to strongly hydrogen bonded water.Through in situ Raman analysis and experiments,the position change of the corresponding peaks of the strongly hydrogen bonded water and the weakly hydrogen bonded water was compared in this work,and the key microscopic process and influence of gas hydrate formation in different systems were comprehensively studied and summarized.It is found that,with the decrease of temperature,the OAH of the weakly hydrogen bonded water remains unchanged when the temperature drops to a certain value,which is the key to the transformation of water into cage hydrate rather than ice.The conversion from the weakly hydrogen bonded water to the strongly hydrogen bonded water is closely related to the gas-liquid interface force,the hydrophilicity/hydrophobicity of the promoter,the ionization degree of liquid,and the electrostatic field of the system.Among the four most common promoters,tetrahydrofuran(THF)has the highest efficiency in promoting methane(CH4)hydrate formation.Therefore,this study provides a scientific direction and basis for the development of high efficient hydrate formation promoters,which can effectively weaken the hydrogen bond of weakly hydrogen bonded water and promote the conversion of weakly hydrogen bonded water to strongly hydrogen bonded water.
基金Funded by the National Natural Science Foundation of China(No.51341009)。
文摘A novel micro fused-casting(MFC)process is developed for semisolid aluminum alloy slurry.The microstructure evolution and properties of semisolid ZL101 aluminum alloy slurry with difierent pouring temperature by MFC are investigated in this paper.During the cooling process,the effects of the pouring temperature on microstructure and properties is primarily analyzed.The microstructure of the semisolid ZL101 aluminum alloy is more homogeneous and the grain is smaller under proper pouring temperature.Temperature of liquids and solids of ZL101 aluminum alloy is measured by difierential scanning calorimetry(DSC).Distribution and characteristics of the microstructure of samples are examined by optical microscope(OM),scanning electron microscopy(SEM)equipped with energy dispersive spectrometer(EDS).The results show that the ZL101 semisolid slurry fabricated by MFC presents uniform shape and good grain size under the pouring temperature of 594°C and the stirring velocity of 600 r/min,and the fine grains of the primary a-Al phase with average grain size of 55μm and shape factor up to 0.67 were obtained.Besides,the ultimate tensile strength and the average Vickers hardness for semisolid ZL101 aluminum slurry are 178.19±1.37 MPa and 86.15±1.16 HV,respectively.
文摘利用全国40个地面台站的观测资料对ERA5及ERA5-Land两种不同空间分辨率的再分析资料开展了地面风速误差评估研究,结果表明:ERA5和ERA5-Land资料多年平均风速偏差的平均值分别为0.08 m s^(−1)、-0.06 m s^(−1),偏差的最大值分别为0.46 m s^(−1)、-0.19 m s^(−1),相对偏差的平均值为4.4%、-2.0%,相对偏差的最大值分别为33.0%、-10.1%;月平均风速线性拟合方程的斜率分别为0.93、0.97,截距分别为0.29 m s^(−1)、0.02 m s^(−1),相关系数分别为0.98、0.99;月平均风速均方根误差的平均值分别为0.17 m s^(−1)、0.14 m s^(−1),均方根误差的最大值分别为0.49 m s^(−1)、0.22 m s^(−1),相对均方根误差的平均值为7.4%、5.7%,相对均方根误差的最大值分别为35.2%、13.3%。ERA5-Land高分辨率资料地面风速误差相对较低,有利于提高风能资源评估的准确性。
文摘提出一种高精度的ZWD模型(tianjin_zwd,TZ)。TZ基于2016-2018年逐小时气压分层的ERA5,欧洲中尺度气象预报中心第五代再分析产品数据,采用BP神经网络建立。然后,根据2019年的ERA5产品导出的ZWD对TZ模型进行了验证。结果表明:相比GPT3模型,TZ模型可提供更贴近真值的ZWD估值;并且,其RMSE由5.0 cm (GPT3)降至4.5 cm,表明10%的精度提升。上述结果表明TZ模型实现了更优的预测性能,该模型的构建策略可为全国其他地区的ZWD建模提供借鉴。
