[Objective]We aimed to study the degradation of 1,1,2,2-tetrachloroethane by mechanochemical method.[Method] Nano-scale NiO particles were prepared by homogeneous precipitation method using nickel sulfate hexahydrate ...[Objective]We aimed to study the degradation of 1,1,2,2-tetrachloroethane by mechanochemical method.[Method] Nano-scale NiO particles were prepared by homogeneous precipitation method using nickel sulfate hexahydrate NiSO 4 ·6H 2 O as a raw material and ammonium carbonate (NH 4) 2 CO 3 as precipitant.The catalytic effect of NiO on the degradation of 1,1,2,2-tetrachloroethane has been investigated.[Result]The concentrations of chloride ion increased as the enhancement of initial concentrations of tetrachloroethane and amounts of catalyst,and the degradation efficiency of tetrachloroethane in water were influenced by the initial concentrations of tetrachloroethane,amounts of catalyst and so on.[Conclusion] This research could provide a novel method for the degradation of 1,1,2,2-tetrachloroethane as an organic pollutant.展开更多
化工、纺织印染与农药化肥等产业的蓬勃发展推动着人类社会的进步,但同时也给环境治理带来了巨大难题。目前,光催化降解局限于在特定波长下针对单一有机污染物进行降解,然而现实中的情况往往更复杂。因此,开发一种多功能光催化材料用于...化工、纺织印染与农药化肥等产业的蓬勃发展推动着人类社会的进步,但同时也给环境治理带来了巨大难题。目前,光催化降解局限于在特定波长下针对单一有机污染物进行降解,然而现实中的情况往往更复杂。因此,开发一种多功能光催化材料用于光催化降解不同有机污染物显得尤为重要。采用一步无模板溶剂热法合成了核壳结构的C-TiO_(2)复合材料前驱体,并在氩气气氛下煅烧得到高结晶度的C-TiO_(2)复合光催化材料。运用SEM、TEM、XRD和TG等表征手段对材料进行表征,结论如下:550℃煅烧时的样品为包含少量碳的高结晶度的锐钛矿相TiO 2,且550℃煅烧时的样品依然保持了完整的核壳结构。此外,C-TiO_(2)复合材料的比表面积高达85.69 m 2·g^(-1),平均孔径为16.4 nm以及孔体积为0.423 m 3·g^(-1)。在UV-Vis光照射下,C-TiO_(2)复合材料分别对罗丹明B(RhB)、亚甲基蓝(MB)和刚果红(CR)3种染料显示出增强的光催化降解活性。展开更多
基金Supported by Guangxi National Natural Science Foundation (No.0640066)Key Laboratory Project of Guangxi Zhuangzu Autonomous Region,China (No. 0702K020 )Guangxi Department of Education Research Project (No. 200911MS60)
文摘[Objective]We aimed to study the degradation of 1,1,2,2-tetrachloroethane by mechanochemical method.[Method] Nano-scale NiO particles were prepared by homogeneous precipitation method using nickel sulfate hexahydrate NiSO 4 ·6H 2 O as a raw material and ammonium carbonate (NH 4) 2 CO 3 as precipitant.The catalytic effect of NiO on the degradation of 1,1,2,2-tetrachloroethane has been investigated.[Result]The concentrations of chloride ion increased as the enhancement of initial concentrations of tetrachloroethane and amounts of catalyst,and the degradation efficiency of tetrachloroethane in water were influenced by the initial concentrations of tetrachloroethane,amounts of catalyst and so on.[Conclusion] This research could provide a novel method for the degradation of 1,1,2,2-tetrachloroethane as an organic pollutant.
文摘化工、纺织印染与农药化肥等产业的蓬勃发展推动着人类社会的进步,但同时也给环境治理带来了巨大难题。目前,光催化降解局限于在特定波长下针对单一有机污染物进行降解,然而现实中的情况往往更复杂。因此,开发一种多功能光催化材料用于光催化降解不同有机污染物显得尤为重要。采用一步无模板溶剂热法合成了核壳结构的C-TiO_(2)复合材料前驱体,并在氩气气氛下煅烧得到高结晶度的C-TiO_(2)复合光催化材料。运用SEM、TEM、XRD和TG等表征手段对材料进行表征,结论如下:550℃煅烧时的样品为包含少量碳的高结晶度的锐钛矿相TiO 2,且550℃煅烧时的样品依然保持了完整的核壳结构。此外,C-TiO_(2)复合材料的比表面积高达85.69 m 2·g^(-1),平均孔径为16.4 nm以及孔体积为0.423 m 3·g^(-1)。在UV-Vis光照射下,C-TiO_(2)复合材料分别对罗丹明B(RhB)、亚甲基蓝(MB)和刚果红(CR)3种染料显示出增强的光催化降解活性。