The concentrations of 30 elements in aerosol particles collected in western Pacific ocean have been determined by INAA. The crustal element concentrations decrease with increasing distance from land over the remote ar...The concentrations of 30 elements in aerosol particles collected in western Pacific ocean have been determined by INAA. The crustal element concentrations decrease with increasing distance from land over the remote area close to Asia land and fluctuate around its average value over the remote ocean area. The volatile elements exhibite average atmospheric concentrations that are higher than those expected from the flux of seasalt or the continental dust. In order to identify marine aerosol component originating from the continent or ocean, the aerosol particles are examined by scanning electron microscopy combined with energy dispersive X-ray spectroscopy. Particle phase structure shows that the crustal aerosol particles are not present internal mixtures with seasalt aerosol, and it also proves the long-range transport of crustal elements from continent to ocean.展开更多
Aerosol samples were collected in the Shiyi Glacier, Qilian Mountains from July 24 to August 19, 2012 and analyzed for major water-soluble ionic species(F-, Cl-, NO2-, NO3-, SO42-, Na+, NH4+, K+, Mg2+and Ca2+) by ion ...Aerosol samples were collected in the Shiyi Glacier, Qilian Mountains from July 24 to August 19, 2012 and analyzed for major water-soluble ionic species(F-, Cl-, NO2-, NO3-, SO42-, Na+, NH4+, K+, Mg2+and Ca2+) by ion chromatography. SO42-and NH4+were the most abundant components of all the anions and cations, with average concentrations of 94.72 and 54.26 neq/m3, respectively, accounting for 34% and 20% of the total water-soluble ions analyzed. These mean ion concentrations were generally comparable with the background conditions in remote sites of the Qilian Mountains, but were much lower than those in certain cities in China. The particles were grouped into two dominant types according to their morphology and EDX signal: Si-rich particles and Fe-rich particles. Backward air mass trajectory analysis suggested that inland cities may contribute some anthropogenic pollution to this glacier, while the arid and semi-arid regions of central Asia were the primary sources of the mineral particles.展开更多
文摘The concentrations of 30 elements in aerosol particles collected in western Pacific ocean have been determined by INAA. The crustal element concentrations decrease with increasing distance from land over the remote area close to Asia land and fluctuate around its average value over the remote ocean area. The volatile elements exhibite average atmospheric concentrations that are higher than those expected from the flux of seasalt or the continental dust. In order to identify marine aerosol component originating from the continent or ocean, the aerosol particles are examined by scanning electron microscopy combined with energy dispersive X-ray spectroscopy. Particle phase structure shows that the crustal aerosol particles are not present internal mixtures with seasalt aerosol, and it also proves the long-range transport of crustal elements from continent to ocean.
基金supported by the National Natural Science Foundation of China (Nos. 41201065, 41121001, 41261017, 41171057, 41161012)Funds for Creative Research Groups of China (No. 41121001)+3 种基金the Foundation for Excellent Youth Scholars of CAREERI, CAS (No. 51Y251B51)the SKLCS Foundation (No. SKLCSZZ-2012-01-01)the National Basic Research Program of China (Nos. 2010CB951003, 2010CB951404)the Knowledge Innovation Project of the Chinese Academy of Sciences (No. KZCX2-EW-311)
文摘Aerosol samples were collected in the Shiyi Glacier, Qilian Mountains from July 24 to August 19, 2012 and analyzed for major water-soluble ionic species(F-, Cl-, NO2-, NO3-, SO42-, Na+, NH4+, K+, Mg2+and Ca2+) by ion chromatography. SO42-and NH4+were the most abundant components of all the anions and cations, with average concentrations of 94.72 and 54.26 neq/m3, respectively, accounting for 34% and 20% of the total water-soluble ions analyzed. These mean ion concentrations were generally comparable with the background conditions in remote sites of the Qilian Mountains, but were much lower than those in certain cities in China. The particles were grouped into two dominant types according to their morphology and EDX signal: Si-rich particles and Fe-rich particles. Backward air mass trajectory analysis suggested that inland cities may contribute some anthropogenic pollution to this glacier, while the arid and semi-arid regions of central Asia were the primary sources of the mineral particles.
