Retrieval of the Single Scattering Albedo of Asian Dust Mixed with Pollutants Using Lidar Observations

The vertical distribution of single scattering albedos （SSAs） of Asian dust mixed with pollutants was derived using the multi-wavelength Raman lidar observation system at Gwangju （35.10°N,126.53°E）.Vertical profiles of both backscatter and extinction coefficients for dust and non-dust aerosols were extracted from a mixed Asian dust plume using the depolarization ratio from lidar observations.Vertical profiles of backscatter and extinction coefficients of non-dust particles were input into an inversion algorithm to retrieve the SSAs of non-dust aerosols.Atmospheric aerosol layers at different heights had different light-absorbing characteristics.The SSAs of non-dust particles at each height varied with aerosol type,which was either urban/industrial pollutants from China transported over long distances at high altitude,or regional/local pollutants from the Korean peninsula.Taking advantage of independent profiles of SSAs of non-dust particles,vertical profiles of SSAs of Asian dust mixed with pollutants were estimated for the first time,with a new approach suggested in this study using an empirical determination of the SSA of pure dust.The SSAs of the Asian dust-pollutants mixture within the planetary boundary layer （PBL） were in the range 0.88-0.91,while the values above the PBL were in the range 0.76-0.87,with a very low mean value of 0.76 ± 0.05.The total mixed dust plume SSAs in each aerosol layer were integrated over height for comparison with results from the Aerosol Robotics Network （AERONET） measurements.Values of SSA retrieved from lidar observations of 0.92 ± 0.01 were in good agreement with the results from AERONET measurements.

Response of Heterotrophic Bacteria Abundance and Community Structure to Asian Dust Addition in the Oligotrophic Northwest Pacific Ocean

The dust storms from the continent usually affect the abundance and diversity of planktons by supplying trace elements. As such, the response of heterotrophic planktonic bacteria to dusts, nutrients(i.e., nitrogen and phosphorus) or ferrous dosages was investigated in the Kuroshio Extension region of the Northwest Pacific Ocean(NWPO) through on-board incubation experiments during an oceanographic survey in spring 2014. The flow cytometry and 16S rRNA high-throughput sequencing methods were applied to explore the abundance and community structure of bacteria, and the percentage of high nucleic acid bacteria(HNA%). The results showed that the heterotrophic bacteria abundance was low(average 2.55×10^5 cells mL^-1) and subjected to both nitrogen(N) and ferrous(Fe) limitation. Sand-dust deposition observably promoted the activity of heterotrophic planktonic bacteria. The maximum abundance of heterotrophic bacteria was 6.98×10^5 cells mL^-1 in the dust-dosage group, which was 44% higher than the control(P < 0.05). The HNA% in the dust-dosage group was 1.37 times higher than the control(P < 0.05). The activation mechanism was mainly related to the dissolution of N and Fe in the dusts. The relative abundance of genus Winogradskyella was significantly increased by dust deposition while the relative abundance of the genera Tenacibaculum and Hyphomonas was decreased. These variations of bacterial community structure were ascribed to the dissolution of nutrients N and P. Comparing the results of different experimental groups, this study concluded that dust storm improved the abundance of heterotrophic bacteria by dissolution of N and Fe.

On Eastern Asian Dust Storm

In this paper, the characteristics of eastern Asian dust storm are examined with emphasis on the satellite measurements of aerosol optical thickness. The reflectivity of solar radiation from the earth's atmosphere depends on the optical thickness. The satellite measurement of radiance of sunlight, scattered by the earth and its atmosphere, is used to derive the properties of aerosol on oceanic surfaces. This paper involves the following: (1) investigation of the measurement of dust storm over the oceanic surface by GMS satellite; (2) investigation of the measurement of dust storm over the land surface by ground-based instruments such as actinometer, lidar, etc.; (3) for comparison, deriving an atmospheric aerosol size distribution over the oceanic surface of calm weather through measurements of NOAA satellite; and (4) the weather process and its mass load of eastern Asian dust storm.

Simulating Dry Deposition Fluxes of PM_(10) and Particulate Inorganic Nitrogen over the Eastern China Seas During a Severe Asian Dust Event Using WRF-Chem Model

A WRF-Chem model including a comprehensive gas-phase nitrogen chemistry module was used to simulate a severe dust event appearing in the eastern China on 19-25 March, 2002. The modeling result well reproduced PM10 concentrations in various distances from the dust sources and the transport pathway of the dust strom. The results showed that both the concentrations and the dry deposition fluxes of PM10 increased over the China seas during the dust event following the passage of a cold front system. The maximum fluxes of PM10 in the Yellow Sea and the East China Sea during the dust event were 5.5 and 8.4 times of those before the event, respectively. However, the temporal variations of the dry deposition fluxes of particulate inorganic nitrogen differed over the Yellow Sea from those over the East China Sea. Nitrate and ammonium in the whole northern China rapidly decreased because of the intrusion of dust-loaded air on 19 March. The dust plume arrived in the Yellow Sea on 20 March, decreasing the particulate inorganic nitrogen in mass concentration accordingly. The minimum dry deposition fluxes of nitrate and ammonium in the Yellow Sea were about 3/5 and 1/6 of those before the dust arrival, respectively. In contrast, when the dust plume crossed over the Yangtze Delta area, it became abundant in nitrate and ammonium and increased the concentrations and dry deposition fluxes of particulate inorganic nitrogen over the East China Sea, where the maximum dry deposition fluxes of nitrate and ammonium increased approximately by 4.1 and 2.6 times of those prior to the dust arrival.

Mineralogy and Possible Sources of Dust Particles During One Asian Dust Episode

A severe Asian Dust Storm(ADS)event occurred on April 16-17th,2006 in northem China.Mineral components of dust samples were analyzed using X-ray diffraction(XRD).The result indicates that dust particles were dominated by quartz(37.4%)and clay (32.9%),followed by plagioclase(13.7%),with small amounts of calcite,K-feldspar,dolomite,homblende, and gypsum(all【10%).The clay fractions with diameter less than 2μm were separated from the

Effect of Asian Dust Storms on the Ambient SO₂Concentration over North-East India: A Case Study

Ambient SO2 concentration at a high rain fall site, Shillong (25.67oN, 91.91oE, 1064 m ASL), located in North-East India, was measured during March 2009 and January 2010 with the aim to understand the effect of long range transport of pollutants from North-East Asia on the ambient SO2 levels at this relatively clean site. The concentrations recorded during the former sampling period were very high (Max: 262.3 ppb)—which decayed down gradually towards the end the sampling period—whereas those during the latter sampling period were well within the acceptable limits (Max: 29.7 ppb). This elevated SO2 concentrations during March 2009 is proposed to have association with a major cold air outbreak and an associated cyclone preceding one of the dust storm events reported in China, and a resultant sudden change in wind trajectory leading to the long range transport of pollutants to the sampling site. The argument is formulated on the basis of the back trajectory analysis performed using HYSPLIT for the month of March 2009—the plots clearly showed a drastic change in wind trajectories between 8th and 15th of March 2009 wherein the winds traveled over some of the highly polluted regions such as the Perm region of Russia—and on the results from model runs performed using the global 3-D model of tropospheric chemistry, GEOS-Chem (v8-03-01)—it clearly showed the tropospheric SO2 over Perm region in Russia peaking during Nov, Dec, Jan, Feb and Mar every year, possibly due to central heating. The observation of long range transport of SO2 from the highly industrialized areas of Perm in Russia to North-East India during dust storm events has important implications to the present understanding on its relative contribution to the Asian pollutant outflow to the Pacific during spring as the GEOS-Chem model runs also showed regions in and around Russia with relatively high concentrations of atmospheric NOx, Peroxyacetyl Nitrate, Lumped Peroxypropionyl Nitrate, HNO3, HNO4,C3H8, C2H6, SO4, NH4, Inorganic Sulphur Nitrates and Lumped Alkyl Nitrate.

INFLUENCE OF ASIAN DUSTS ON THE PHYSICOCHEMICAL PROPERTIES OF ATMOSPHERIC AEROSOLS IN TAIWAN DISTRICT——USING THE PENGHU ISLANDS AS AN EXAMPLE

Using the Penghu Islands as an example, this study investigates the influence of Asian dusts on the physicochemical properties of atmospheric aerosols in Taiwan District in the year of 2002. An aerosol-sampling site was established at Xiaumen, the Penghu Islands, to collect sea level atmospheric aerosols for further analysis of their phys-icochemical properties. This study revealed that, during the sampling campaign, three Asian dust storms were trans-ported from North China and Mongolia to the Penghu Islands. The mass concentrations of atmospheric aerosols, par-ticularly PM2.5~10, were generally 2~3 times higher than the regular level. An increase of coarse particle mode in the size distribution of atmospheric aerosols further validated the invasion of Asian dusts. Moreover, the comparison of wa-ter-soluble ionic species, carbonaceous content, and metallic content of atmospheric aerosols indicated that Asian dusts could significantly influence the chemical properties of atmospheric aerosols in Taiwan District. A significant increase of Cl-, Br-, Na+, K+, SO42-, Mg2+ and Ca2+ concentration on coarse particle mode was observed. It suggested that not just natural soil dusts and oceanic spray, but also anthropogenic pollutants could accompany Asian dusts. Source appor-tionment of atmospheric aerosols indicated that the concentration (percentage) of aerosol particles contributed from soil dusts increased significantly from 20.98 mg.m-3 (29.2%) to 60.37 mg.m-3 (47.7%), and then decreased to the regular level of 22.44 mg.m-3 (28.2%).

Effects of Asian dust events on atmospheric bacterial communities at different distances downwind of the source region

Aeolian dust particles arising from arid and semiarid zones are known to carry microbes by air currents. The effect of wind-borne bacteria on atmospheric bacterial population at various downwind distances from the dust source regions must be clarified, but has not yet been reported. This study monitored the bacterial abundance and community composition in outdoor aerosol samples in Beijing, China, which is close to the Asian dust source regions, and compared them with the results obtained in a distant region（Osaka, Japan）.The Asian dust collected in Beijing contained（4 ± 3） × 10^4 bacterial cells/m^3, approximately 4 times higher than in Osaka. On 15 April 2015, Beijing experienced severe Asian dust events with a 1000-fold increase in bacterial abundance, relative to non-Asian dust days. Dominant bacterial phyla and classes in Asian dust collected in Beijing were Actinobacteria, Bacilli and Acidobacteria, and the bacterial community composition varied more widely than in Osaka.The bacterial community compositions differed between the Beijing and Osaka dusts, even for the same Asian dust events. These results indicated that aerosol bacterial communities nearer the dust source are more affected by eolian dust than their distant counterparts.

Dry deposition of PM_(10) over the Yellow Sea during Asian dust events from 2001 to 2007

Dry deposition velocities and fluxes of PM10 during Asian dust events over the Yellow Sea from 2001 to 2007 were investigated using observation data in Qingdao, China and Jeju, Korea. The dry deposition velocities of PM 10 during dust events over the Yellow Sea ranged from 0.19 to 8.17 cm/sec, with an average of 3.38 cm/sec. Dry deposition fluxes of PM10 during dust events over the Yellow Sea were in the range of 68.5-2647.1 mg/（m2.day）, with an average of 545.4 mg/（m2.day）, which is 2-10 times higher than those reported by other studies for both dust and non-dust periods. It was estimated that 2.6× 10^11-48.7 × 10^11 g dust particles deposit to the Yellow Sea during dust events through dry deposition every year. Compared with the results in previous studies, it was found that the dry deposition of PM10 over the Yellow Sea during dust events in the years with high frequency of dust could account for a large or overwhelming fraction of the annual total dry deposition. Backward air mass trajectory analysis showed that dust events influenced Jeju mainly originated from the desert regions located in Mongolia and Inner Mongolia, China. There were 119 backward trajectories influenced both Qingdao and Jeju during 15 dust events from 2001 to 2007, accounting for 61.3% of the total trajectories of 194, indicating that Qingdao and Jeju were usually on the same pathway of dust transport downwind from source areas.

Forecasting of Asian dust storm that occurred on May 10-13, 2011, using an ensemble-based data assimilation system

An ensemble-based assimilation system that used the MASINGAR ink-2 （Model of Aerosol Species IN the Global AtmospheRe Mark 2） dust forecasting model and satellite-derived aerosol optical thickness （AOT） data. processed in the JAXA （Japan Aerospace Exploration Agency） Satellite Monitoring for Environmental Studies （JASMES） system with MODIS （Moderate Resolution Imaging Spectroradiometer） observations. was used to quantify the impact of assimilation on forecasts of a severe Asian dust storm during May 10-13. 2011. The modeled bidirectional reflectance function and observed vegetation index employed in JASMES enable AOT retrievals in areas of high surface reflectance, making JASMES effective for dust forecasting and early warning by enabling assimilations in dust storm source regions. Forecasts both with and without assimilation were validated using PM^0 observations from China, Korea, and Japan in the TEMM WG1 dataset. Only the forecast with assimilation successfully captured the contrast between the core and tail of the dust storm by increasing the AOT around the core by 70-150% and decreasing it around the tail by 20-30% in the 18-h forecast. The forecast with assimilation improved the agreement with observed PMlo concentrations, but the effect was limited at downwind sites in Korea and Japan because of the lack of observational constraints for a mis-forecasted dust storm due to cloud.

Asian Dust Workshop Held in USA

An Asian Dust Storm International Workshop was held on 25—26 June 1992 at the Grad-uate School of Oceanography,University of Rhode Island,U.S.A.Dr.Richard Arimoto of theCenter for Atmospheric Chemistry Studies,University of Rhode Island was the organizer forthis workshop.More than 30 scientists from China,Japan and the United States attended themeeting.

Geochemical studies on the source region of Asian dust

The North China and the neighbouring Mongolia in Asian Interior is characterized by extremely dry climate, resulted in one of the world's major dust emission centres. Deciphering the source region of Asian dust is critical for revealing the mechanism of the dust production, interpreting the paleo-environmental records of eolian deposits, predicting the overall environmental effects of dust, and setting the strategies for the control of contemporary dust storms. This paper summarizes the geochemical methods applied to the source tracing of Asian dust. Nd-Sr isotopes were the most extensively studied source tracer of Asian dust and have been successfully applied in many cases. Geochemistry of detrital monomineral shows great theoretical advantages in source tracing and deserves further studies. The short-range transportation of Chinese loess with direction similar to that of the prevailing near surface wind is revealed. Source tracing also shows that the Asian dust has two ultimate material sources from the northern margin of the Tibetan Plateau and the Central Asian Orogen, which confirms the importance of mountain processes in the production of silt eolian particles. Based on the recent progresses on the source tracing of Asian dust, discussions are expanded on the natural background of Asian dust storms and potential anthropogenic influence, the materials evolution of the source regions of Asian dust and its relationships with climate changes and Tibetan uplift, and the role of Tibetan uplift in the Asian dust system.

Mineralogical characteristics of airborne particles collected in Beijing during a severe Asian dust storm period in spring 2002

Asian dust storm (ADS) samples were collected on March 20,2002 in Beijing,China. High-resolution field emission scanning electron microscopy with energy dispersive X-ray detector (FESEM-EDX) and X-ray diffraction (XRD) were used to study the morphology,chemical compositions,number-size dis-tributions and mineralogical compositions of ADS particles. The mineral particles were major compo-nents in the ADS samples,accounting for 94% by number. The XRD analysis indicated that the dust particles were dominated by clay (40.3%),and quartz (19.5%),followed by plagioclase (8.4%),calcite (7.5%),K-feldspar (1.5%),hematite (0.9%),pyrite (0.9%),hornblende (0.4%) and gypsum (0.3%),with a certain amount of noncrystalline materials (20.3%). Clay minerals were mainly illite/smectite mixed lay-ers (78%),followed by illite (9%),kaolinite (6%),and chlorite (7%). In addition to these main minerals,FESEM-EDX also detected some trace minerals,such as dolomite,pyrite,thenardite,as well as heavy minerals represented by rutile,ilmenite and apatite. The mineralogical compositions of the 2002-03-20 Asian dust storm and the Saharan dust plumes were similar but the clay mineralogy showed a great distinction,with the illite/smectite mixed layers being common in the Asian dust storm but illite being common in the Saharan dust plumes.

Compound-specific carbon isotope compositions of individual long-chain n-alkanes in severe Asian dust episodes in the North China coast in 2002

The molecular compositions and com- pound-specific carbon isotope compositions of indi- vidual long-chain n-alkanes of atmospheric aerosols collected during two severe Asian dust episodes in Qingdao in spring of 2002 were analyzed using gas chromatography/mass spectrometry (GC/MS) and gas chromatography/isotope ratio mass spectrometry (GC/IRMS). Typical plant wax n-alkanes (C29 and C31) had lower δ 13C values than those from anthropo- genic (engine exhaust) sources (C21―C23). The av- erage δ 13C value of plant wax n-alkane C29 in non-dust episode periods was -30.5‰ (?30.3‰― ?31.9‰), while -31.3‰ (?31.1‰―?31.5‰) in dust episode periods; for C31, it was ?31.4‰ (?31.1‰― ?33.0‰) in non-dust episode periods, and ?31.7‰ (?31.3‰―?32.6‰) in dust episode periods. Plant wax in the dust episode samples was mainly from herbaceous plants via long-range transport, while local plant wax was mainly from deciduous plants and woody plants. In North China coast, 83.3% of the plant wax in the severe dust episode samples was from C3 plants while 80.0% for the non-dust samples, indicating that plant wax transported to the north- western Pacific Ocean by airborne dust from East Asia was mainly from C3 plants. The results suggestthat the molecular and molecular-isotopic composi- tions of individual long-chain n-alkanes can, as an effective indicator, identify the terrestrial organic components in the dust from East Asia and sedi- ments in the northwest Pacific Ocean.

Climatology of yellow sand (Asian sand, Asian dust or Kosa) in East Asia

In order to study climatology of yellow sand (Asian sand, Asian dust or Kosa) in EastAsia, secular fluctuation in China, Korea and Japan in the recent 30 years was presented. Thenumber of days with sand-dust storm at five stations in China-Hotan, Zhangye, Minqin, Jurhand Beijing, decreases a lot at the former three stations, but changed little at the latter two stations.Suggesting that the recent global warming is more evident in Xinjiang and Gansu, where the fre-quency of cold air invasions from the higher latitudes is decreasing. But, the eastern parts ofMongolia, inner Mongolia, and North China encounter stronger cyclones in early spring as a resultof global warming. These cyclones bring cold air from higher latitudes, causing severe duststorms. Secular variation in the annual days with sand-dust storms in China and Kosa days in Ko-rea and Japan show a parallel change with higher frequency from 1975 to 1985. This may be re-lated to the higher frequency of La Nina years. However, different tendency was shown in theperiod from 1986 to 1996. Since 1996 or 1997, a sharp increase is clear, which may be caused bythe developed cyclones in East Asia as well as human activities, and stronger land degradationunder La Nina conditions. Anomalies of the total number of stations with Kosa days were dis-cussed in accordance with some synoptic meteorological conditions such as the differences be-tween Siberian anticyclone and Aleutian cyclone center at 500 hPa level during the previous winter.

Relationship between East Asian Monsoon and Dust Weather Frequency over Beijing

The relationship between dust weather frequency （DWF）, which denotes the number of days of dust weather events, over Beijing and the East Asian Monsoon （EAM） was studied using DWF data for Beijing during the period 1951-2006. Results show that, during this period, the blowing-dust weather frequency （BDWF）, as well as the indices of East Asian winter monsoon （EAWM） and East Asian summer monsoon （EASM）, all decreased considerably, with a t-test confidence level of 99%. The correlation coeffcients between the chosen EAWM index and BDWF over Beijing in winter and the following spring were 0.34 and 0.33, respectively, with significance levels of 0.01 and 0.02, respectively. For the chosen EASM index and BDWF, these correlation coeffcients were 0.51 and 0.45, respectively, with both at a confidence level exceeding 99.9%. With the linear trends removed, the values （in the same order as above） were 0.14, 0.14, -0.12, and -0.09, all not significant at the 95% confidence level. Clearly, the EAM relates mainly to DWF over long timescales. To a certain extent, the EAM might have some impact on DWF by affecting the associated surface air temperature and precipitation during the corresponding time period in sand-dust source regions at the interannual scale. A stronger （weaker） EAWM might advance （suppress） the occurrence of DWF, and the opposite for the EASM.

IMPACT OF DESERT DUST ON THE EAST ASIAN SUMMER MONSOON

The radiative forcing(RF) of Asian desert dust and its regional feedbacks to the East Asian summer monsoon(EASM) system are investigated with a coupled regional climate-desert dust model.The statistical significance of desert dust effects are analyzed through 20 summer seasons(1990-2009).In order to estimate the dust effects reasonably,some improvement has been achieved for the coupled model,including the updates of optical properties and desert source area distribution.We find that the desert dust can result in a roughly weakened monsoon in eastern China,Korean Peninsula,Japan and Indian Peninsula and a strengthened monsoon in Indochina Peninsula in the lower troposphere.Moreover,the precipitation comparisons between observational data and simulated patterns are also suggestive of the desert dust effect on the EASM.In the upper troposphere,the southward shift of the westerly jet(WJ) by the dust effect can be seen as an indicator of the weakened monsoon in great part of the monsoon areas.The change of the moist static energy(MSE) contrast between land and ocean is the main reason for the EASM variations.

Seasonal Variations in Dustfall and Its Iron Content over North China

Extensive dustfall collections were carried out from April 2001 to May 2002 in North China. The highest level of dustfall occurred in the Gobi deserts and at the margins of sandy deserts in the region. The iron content in dustfall in North China varied from 0.6% to 6.0% and there was significant seasonal variation, which indicates the dust sources differed during the year. Although the iron content in dustfall in North China is higher in the Loess Plateau and arable lands and lower in the Gobi and sandy deserts, the total iron deposition was higher in the Gobi desert regions. If the fine particles （PM10） in dustfall in North China are the major contributors of dust transport to eastern China and western parts of the North Pacific, then the annual deposition rates of iron may have been underestimated in previous studies. Our analysis indicates that iron deposition may reach 1.38 × 10^3 to 2.43 × 10^3 kg km^-2 and that most iron deposition occurs in spring and summer. If the more-coarse fractions （PM50） are considered, deposition rates may reach 2.75 × 10^3 and 6.80 × 10^3 kg km^-2, which would represent a large source of iron deposition in eastern China and the western North Pacific.

The Mineralogy and Possible Sources of Spring Dust Particles over Beijing

A severe Asian Dust Storm （ADS） event occurred on 16-17 April 2006 in northern China. The mineral compositions of dust samples were analyzed using X-ray diffraction （XRD）. The results indicated that dust particles of the ＂17 April 2006＂ dust storm were dominated by quartz （37.4%） and clay （32.9%）, followed by plagioclase （13.7%）, with small amounts of calcite, K-feldspar, dolomite, hornblende and gypsum （all less than 10%）. The clay fractions with diameter less than 2 μm were separated from the dust storm particles by centrifuging and were further analyzed by XRD. The results revealed that the clay species were mainly illite/smectite mixed layers （I/S） （49%） and illite （34%）, with small amount of kaolinite （8%） and chlorite （9%）. In order to evaluate the feasibility of using the mineralogy to trace the sources of dust particles, the XRD results of the ＂17 April 2006＂ dustfall particles were compared with the dust particles over past years. The results confirmed that the finer dust particles represented by the ADS PM10 displayed a smaller quartz/clay ratio than the dustfall particles. The dust storm particles, either from the ADS PM10 or from the ＂17 April 2006＂ dustfall, showed a lower level of dolomite contents and lower dolomite/clay ratios compared with the non-dust storm dustfall particles. This implies that dolomite could be used to distinguish between the dust contributions from local and non-local sources. Similar trends were found for the gypsum and the gypsum/clay ratio. Moreover, the two dustfall samples had a lower level of illite/smectite mixed layers and a higher level of illite than airborne PM10, implying that the dustfall particles tend to be enriched with illite in its clay fraction.

Element and mineral characterization of dust emission from the saline land at Songnen Plain, Northeastern China

Recent observations of Asian dust storms show an eastern expansion of the source area to degraded lands, where dust emissions have been little studied. The dust concentrations over the saline land of the western Songnen Plain （SSL）, Northeastern China, are circumstantially higher than those from the northwestern Chinese deserts. These concentrations are sensitive to the surface soil conditions and wind velocity on the ground. The dust samples collected during dust storm events on the SSL contain abundant Na, Mg, A1, K, Ca, Fe and Ti, as well as toxic elements such as Cu, V, Zn and Ba. Individual particle analysis reveals that fine saline particles （〈 10 μm in diameter） on the saline land, consisting largely of carbonate, halite and sulfate together with lithogenic minerals such as SiO2 and aluminosilicate, are eventually uplifted during the interval from spring to autuum. The predominantly fine saline particles uplifted from the SSL are likely transported eastward by the winter monsoon circulation and westerlies. Recent degradation of saline lands in Northeastern China would not only increase the frequency of dust storm events in the downwind area, but also might change the chemical composition of the Asian dust emissions.