A burnup calculation has been performed to evaluate heavy rare earth (terbium--Tb, dysprosium--Dy) production in spent gadolinium oxide (Gd203) installed as a BP (burnable poison). Each amount of Tb and Dy produ...A burnup calculation has been performed to evaluate heavy rare earth (terbium--Tb, dysprosium--Dy) production in spent gadolinium oxide (Gd203) installed as a BP (burnable poison). Each amount of Tb and Dy production derived from the BP has been about 30-40 times larger than those created in FP (fission products). Required cooling time to achieve exemption level on radioactivity concentration produced Tb and Dy derived from the BP are much shorter (BP-Tb: 7.9y, BP-Dy: 〈 0.1y) than those created in FP (FP-Tb: 3,616y, FP-Dy: 6.9y). However, the BP is mixed homogeneously with UO2 pellet in current nuclear fuel system of LWRs (light water reactors), and hence mixing of FP cannot be not avoided. In such a mixture case, the required cooling time of recovered Tb will become 2,653y and that of recovered Dy be 4.8y. For this reason, recovered Tb is unlikely to be resource for utilization, while recovered Dy must be the resource provided the precise separation from the other FP.展开更多
文摘A burnup calculation has been performed to evaluate heavy rare earth (terbium--Tb, dysprosium--Dy) production in spent gadolinium oxide (Gd203) installed as a BP (burnable poison). Each amount of Tb and Dy production derived from the BP has been about 30-40 times larger than those created in FP (fission products). Required cooling time to achieve exemption level on radioactivity concentration produced Tb and Dy derived from the BP are much shorter (BP-Tb: 7.9y, BP-Dy: 〈 0.1y) than those created in FP (FP-Tb: 3,616y, FP-Dy: 6.9y). However, the BP is mixed homogeneously with UO2 pellet in current nuclear fuel system of LWRs (light water reactors), and hence mixing of FP cannot be not avoided. In such a mixture case, the required cooling time of recovered Tb will become 2,653y and that of recovered Dy be 4.8y. For this reason, recovered Tb is unlikely to be resource for utilization, while recovered Dy must be the resource provided the precise separation from the other FP.