Contingent Valuation Method(CVM) was used to investigate the Chinese public's willingness to pay(WTP) for a policy to reduce CO2 emissions. Face to face interviews were conducted to collect 1,653 valid questionnai...Contingent Valuation Method(CVM) was used to investigate the Chinese public's willingness to pay(WTP) for a policy to reduce CO2 emissions. Face to face interviews were conducted to collect 1,653 valid questionnaires from Beijing, Shanghai, Shandong province, and Fujian province. A model was constructed to understand the factors that influence WTP. The results indicate that the Chinese public is willing to pay CN 201.86 annually to support the policy of reducing greenhouse gas emissions. Participants from Beijing show the highest WTP, followed by participants from Fujian and Shandong, while those from Shanghai report the lowest WTP. The findings reveal that participants with higher income, higher satisfaction with their current life, and awareness of climate issues are willing to pay more for CO2 emissions reductions. In addition, those who are young, male and members of the Communist Party also indicate a higher WTP. The results imply that translating the public's willingness to protect climate into actions should be taken into account in China's low carbon policy. There is a need to consider the difference in degree of willingness, among different social groups, to pay for emissions reductions if the market-based mechanisms such as carbon tax were designed to facilitate emissions reductions.展开更多
Using the improved Energy-Environmental Version of the GTAP Model (GTAP-E) and the sixth version of emission database of non-CO2 greenhouse gases, we simulate the emission reduction potential of non-CO2 greenhouse gas...Using the improved Energy-Environmental Version of the GTAP Model (GTAP-E) and the sixth version of emission database of non-CO2 greenhouse gases, we simulate the emission reduction potential of non-CO2 greenhouse gases in China and its policy implications. The results show that at present, China is a country with the greatest emission of non-CO2 greenhouse gases in the world, and the emission will account for about 20% of the world's total emission in 2020. The proportion of emission of non-CO2 greenhouse gases from the agricultural sector reaches 73%. In the next 10 years, the emission of non-CO2 gases from cattle and sheep, industry and service industry will experience the highest growth rate; the growth rate of emission from service industry will be higher than that of emission from industry, and the emission from service industry will exceed that from industry after 2010. China can implement emission reduction policy of non-CO2 greenhouse gases to ease the international pressure of CO2 emission reduction. Although the high carbon tax collected can reduce considerable non-CO2 emission, there is little difference in policy efficiency between high carbon tax and low carbon tax. So, in the implementation of emission reduction carbon tax policy of non-CO2 gases, it is necessary to control the carbon tax at a low level.展开更多
Fossil-fuel burning greenhouse gas induced global warming has been recognized as global environmental problems,reduce and ultimately control the energy production in the use of CO_2 emissions, global energy production...Fossil-fuel burning greenhouse gas induced global warming has been recognized as global environmental problems,reduce and ultimately control the energy production in the use of CO_2 emissions, global energy production will be a major challenge.As a highly intensive materials and energy,iron and steel enterprises,need to be invested to produce one ton of steel about two tons of material and 0.7 t of standard coal energy,and while producing two tons of CO_2.Therefore,reducing CO_2 emissions from iron and steel industry has become the focus of the global steel industry.This paper describes an integrated domestic and international measures to control carbon dioxide emissions research progress and future technology trends, with emphasis on the domestic steel industry emissions of carbon dioxide status of technology development and industrialization of implementation of the proposed on this basis,including dry quenching technology, gas,power generation,coal moisture control technology,blast furnace injection plastics technology,the use of coking process for treating municipal waste plastics technology,sintering heat generation,low pressure saturated steam for power generation,metallurgical slag heat recovery technology,coke oven gas hydrogen technology and the other key technologies energy saving technologies,including the development,promotion and popularization of the steel industry in China will be the CO_2 emission reduction technology direction and focus.At this stage,the Chinese steel industry can be improved the energy efficiency and recycling of waste heat and energy,reduce unit GDP,CO_2 emissions;but in the long run,should increase CO_2 capture and storage on the input of technology can possible effective control of the adverse effects of CO_2 emissions.展开更多
In this investigation, Pt–Ba–Ce/c-Al2O3 catalysts were prepared by incipient wetness impregnation and experiments were performed to evaluate the influence of H2 on the evolution mechanism of nitrogen oxides (NOx) st...In this investigation, Pt–Ba–Ce/c-Al2O3 catalysts were prepared by incipient wetness impregnation and experiments were performed to evaluate the influence of H2 on the evolution mechanism of nitrogen oxides (NOx) storage and reduction (NSR). The physical and chemical properties of the Pt–Ba–Ce/c- Al2O3 catalysts were studied using a combination of characterization techniques, which showed that PtOx, CeO2, and BaCO3, whose peaks were observed in X-ray diffraction (XRD) spectra, dispersed well on the c-Al2O3, as shown by transmission electron microscope (TEM), and that the difference between Ce3+ and Ce4+, as detected by X-ray photoelectron spectroscopy (XPS), facilitated the migration of active oxygen over the catalyst. In the process of a complete NSR experiment, the NOx storage capability was greatly enhanced in the temperature range of 250–350℃, and reached a maximum value of 315.3μmol·gcat^-1 at 350℃, which was ascribed to the increase in NO2 yield. In a lean and rich cycling experiment, the results showed that NOx storage efficiency and conversion were increased when the time of H2 exposure (i.e., 30, 45, and 60 s) was extended. The maximum NOx conversion of the catalyst reached 83.5% when the duration of the lean and rich phases was 240 and 60 s, respectively. The results revealed that increasing the content of H2 by an appropriate amount was favorable to the NSR mechanism due to increased decomposition of nitrate or nitrite, and the refreshing of trapping sites for the next cycle of NSR.展开更多
The conversion of carbon dioxide to chemicals by the electrochemical reactions(ERC)is an efficient solution to the current energy crisis and excess CO_(2) emissions.It is still a great challenge and of significance to...The conversion of carbon dioxide to chemicals by the electrochemical reactions(ERC)is an efficient solution to the current energy crisis and excess CO_(2) emissions.It is still a great challenge and of significance to synthesize a highly selective,efficient,and non-noble metal electrocatalyst that facilitates the ERC reaction.A novel triton X-100(C_(14)H_(22)O(C_(2)H_(4)O)n)assisted electrodeposition method was developed to synthesize the ordered cone-structured tin(OCSn)electrocatalysts with controllable morphology and structure.The results suggest that Triton X-100 plays an important role in directing the structure of the Sn electrocatalysts during the electrodeposition process.The OCSn synthesized at 60 m A cm^(-2) achieves the best performances.It selectively catalyzes the ERC on the onset potential about 110 m V lower than Sn synthesized without Triton X-100.In 0.5 M Na HCO_(3),high faradaic efficiency(92%)for formate product on OCSn has been achieved.More prominently,the catalyst presents excellent stability,showing no performance deterioration during 30 h electrolysis.This work provides an efficient,green,and scalable synthesis method of the electrocatalyst for CO_(2) reduction to formate.展开更多
A rare-earth free upconversion luminescent material, 10BaF2：NaF, Na3AIF6, is synthesized by a hydrothermal method. The study of fluorescent spectrum indicates that it can convert visible light （550 nm-610 nm） into ...A rare-earth free upconversion luminescent material, 10BaF2：NaF, Na3AIF6, is synthesized by a hydrothermal method. The study of fluorescent spectrum indicates that it can convert visible light （550 nm-610 nm） into ultraviolet light （290 nm 350 nm）, and two emission peaks at 304 nm and 324 nm are observed under the excitation of 583 nm at room temperature. Subsequently, 10BaF2：NaF, Na3AIF6/TiO2 composite photocatalyst is prepared and its catalytic activity is evaluated by the photocatalytic reduction of CO2 under visible light irradiation （λ〉 515 nm）. The results show that 10BaF2：NaF, Na3AIF6/TiO2 is a more effective photocatalyst for CO2 reduction than pure TiO2, their corresponding methanol yields are 179 and 0 μmol/g-cat under the same conditions. Additionally, the mechanism of photocatalytic reduction of CO2 on 10BaF2：NaF, Na3AIF6/TiO2 is proposed.展开更多
As an important transportation infrastructure and transportation backbone in China,high-speed rail(HSR)plays a critical role in promoting the development of green and low-carbon transportation.Calculating the CO_(2) e...As an important transportation infrastructure and transportation backbone in China,high-speed rail(HSR)plays a critical role in promoting the development of green and low-carbon transportation.Calculating the CO_(2) emissions reduction performance of HSR will be conduci v e to pr omote the CO_(2) emissions r eduction w ork of the r ail w ay.Based on the Dalkic HSR CO_(2) emissions r eduction performance model,by adjusting the HSR CO_(2) emission factor(CEF HSR),the annual times of departures(T)and other parameters,this study develops a Chinese HSR CO_(2) emissions reduction performance model.Taking the Beijing-Shanghai HSR as the resear c h object,this study conducts a questionnaire survey to explore the substitution effect and demand effect of HSR on different transportation modes;collects data such as passenger v olume,av era ge electricity use and annual times of departures of the Beijing-Shanghai HSR in 2019;and calculates the CO_(2) emissions reduction performance of the Beijing-Shanghai HSR.This study has two main results:(1)It builds a Chinese HSR CO_(2) emissions reduction performance model based on substitution effect and demand effect.(2)In 2019,the CO_(2) emissions of the Beijing-Shanghai HSR are 2898233.62 t,the CO_(2) emissions reduction performance of the Beijing-Shanghai HSR is 17999482.8 t,the annual CO_(2) emissions of the Beijing-Shanghai line in‘No HSR’case are 7.2 times as in the’HSR’case and the PKT of the HSR is 10.2 g/pkm.Based on the research results,this study proposes three CO_(2) emissions reduction policy suggestions.This study would be helpful for further HSR CO_(2) emissions reduction resear c h and departments related to railway transportation management to make CO_(2) emissions reduction policies.展开更多
As part of efforts to reduce anthropogenic CO_(2) emissions by the steelmaking industry,this study investigated the direct reduction of industrially produced hematite pellets with H_(2) using the Doehlert experimental...As part of efforts to reduce anthropogenic CO_(2) emissions by the steelmaking industry,this study investigated the direct reduction of industrially produced hematite pellets with H_(2) using the Doehlert experimental design to evaluate the effect of pellet diameter(10.5-16.5 mm),porosity(0.36-0.44),and temperature(600-1200℃).A strong interactive effect between temperature and pellet size was observed,indicating that these variables cannot be considered independently.The increase in temperature and decrease in pellet size considerably favor the reduction rate,while porosity did not show a relevant effect.The change in pellet size during the reduction was negligible,except at elevated temperatures due to crack formation.A considerable decrease in mechanical strength at high temperatures suggests a maximum process operating temperature of 900℃.Good predictive capacity was achieved using the modified grain model to simulate the three consecutive non-catalytic gas-solid reactions,considering different pellet sizes and porosities,changes during the reaction from 800 to 900℃.However,for other temperatures,different mechanisms of structural modifications must be considered in the modeling.These results represent significant contributions to the development of ore pellets for CO_(2)-free steelmaking technology.展开更多
基金supported by the Foundation of the Humanities and Social Science, Ministry of Education of the People’s Republic of China (No. 09YJA790119)
文摘Contingent Valuation Method(CVM) was used to investigate the Chinese public's willingness to pay(WTP) for a policy to reduce CO2 emissions. Face to face interviews were conducted to collect 1,653 valid questionnaires from Beijing, Shanghai, Shandong province, and Fujian province. A model was constructed to understand the factors that influence WTP. The results indicate that the Chinese public is willing to pay CN 201.86 annually to support the policy of reducing greenhouse gas emissions. Participants from Beijing show the highest WTP, followed by participants from Fujian and Shandong, while those from Shanghai report the lowest WTP. The findings reveal that participants with higher income, higher satisfaction with their current life, and awareness of climate issues are willing to pay more for CO2 emissions reductions. In addition, those who are young, male and members of the Communist Party also indicate a higher WTP. The results imply that translating the public's willingness to protect climate into actions should be taken into account in China's low carbon policy. There is a need to consider the difference in degree of willingness, among different social groups, to pay for emissions reductions if the market-based mechanisms such as carbon tax were designed to facilitate emissions reductions.
文摘Using the improved Energy-Environmental Version of the GTAP Model (GTAP-E) and the sixth version of emission database of non-CO2 greenhouse gases, we simulate the emission reduction potential of non-CO2 greenhouse gases in China and its policy implications. The results show that at present, China is a country with the greatest emission of non-CO2 greenhouse gases in the world, and the emission will account for about 20% of the world's total emission in 2020. The proportion of emission of non-CO2 greenhouse gases from the agricultural sector reaches 73%. In the next 10 years, the emission of non-CO2 gases from cattle and sheep, industry and service industry will experience the highest growth rate; the growth rate of emission from service industry will be higher than that of emission from industry, and the emission from service industry will exceed that from industry after 2010. China can implement emission reduction policy of non-CO2 greenhouse gases to ease the international pressure of CO2 emission reduction. Although the high carbon tax collected can reduce considerable non-CO2 emission, there is little difference in policy efficiency between high carbon tax and low carbon tax. So, in the implementation of emission reduction carbon tax policy of non-CO2 gases, it is necessary to control the carbon tax at a low level.
文摘Fossil-fuel burning greenhouse gas induced global warming has been recognized as global environmental problems,reduce and ultimately control the energy production in the use of CO_2 emissions, global energy production will be a major challenge.As a highly intensive materials and energy,iron and steel enterprises,need to be invested to produce one ton of steel about two tons of material and 0.7 t of standard coal energy,and while producing two tons of CO_2.Therefore,reducing CO_2 emissions from iron and steel industry has become the focus of the global steel industry.This paper describes an integrated domestic and international measures to control carbon dioxide emissions research progress and future technology trends, with emphasis on the domestic steel industry emissions of carbon dioxide status of technology development and industrialization of implementation of the proposed on this basis,including dry quenching technology, gas,power generation,coal moisture control technology,blast furnace injection plastics technology,the use of coking process for treating municipal waste plastics technology,sintering heat generation,low pressure saturated steam for power generation,metallurgical slag heat recovery technology,coke oven gas hydrogen technology and the other key technologies energy saving technologies,including the development,promotion and popularization of the steel industry in China will be the CO_2 emission reduction technology direction and focus.At this stage,the Chinese steel industry can be improved the energy efficiency and recycling of waste heat and energy,reduce unit GDP,CO_2 emissions;but in the long run,should increase CO_2 capture and storage on the input of technology can possible effective control of the adverse effects of CO_2 emissions.
基金the National Natural Science Foundation of China (51676090)the Natural Science Foundation of Jiangsu Province (BK20150513), and the Six Talent Peaks Project in Jiangsu Province.
文摘In this investigation, Pt–Ba–Ce/c-Al2O3 catalysts were prepared by incipient wetness impregnation and experiments were performed to evaluate the influence of H2 on the evolution mechanism of nitrogen oxides (NOx) storage and reduction (NSR). The physical and chemical properties of the Pt–Ba–Ce/c- Al2O3 catalysts were studied using a combination of characterization techniques, which showed that PtOx, CeO2, and BaCO3, whose peaks were observed in X-ray diffraction (XRD) spectra, dispersed well on the c-Al2O3, as shown by transmission electron microscope (TEM), and that the difference between Ce3+ and Ce4+, as detected by X-ray photoelectron spectroscopy (XPS), facilitated the migration of active oxygen over the catalyst. In the process of a complete NSR experiment, the NOx storage capability was greatly enhanced in the temperature range of 250–350℃, and reached a maximum value of 315.3μmol·gcat^-1 at 350℃, which was ascribed to the increase in NO2 yield. In a lean and rich cycling experiment, the results showed that NOx storage efficiency and conversion were increased when the time of H2 exposure (i.e., 30, 45, and 60 s) was extended. The maximum NOx conversion of the catalyst reached 83.5% when the duration of the lean and rich phases was 240 and 60 s, respectively. The results revealed that increasing the content of H2 by an appropriate amount was favorable to the NSR mechanism due to increased decomposition of nitrate or nitrite, and the refreshing of trapping sites for the next cycle of NSR.
基金the financially support of the National Natural Science Foundation of China(No.21576255 and No.21577141)Dalian Science Fund for Distinguished Young Scholars(2018RJ09)。
文摘The conversion of carbon dioxide to chemicals by the electrochemical reactions(ERC)is an efficient solution to the current energy crisis and excess CO_(2) emissions.It is still a great challenge and of significance to synthesize a highly selective,efficient,and non-noble metal electrocatalyst that facilitates the ERC reaction.A novel triton X-100(C_(14)H_(22)O(C_(2)H_(4)O)n)assisted electrodeposition method was developed to synthesize the ordered cone-structured tin(OCSn)electrocatalysts with controllable morphology and structure.The results suggest that Triton X-100 plays an important role in directing the structure of the Sn electrocatalysts during the electrodeposition process.The OCSn synthesized at 60 m A cm^(-2) achieves the best performances.It selectively catalyzes the ERC on the onset potential about 110 m V lower than Sn synthesized without Triton X-100.In 0.5 M Na HCO_(3),high faradaic efficiency(92%)for formate product on OCSn has been achieved.More prominently,the catalyst presents excellent stability,showing no performance deterioration during 30 h electrolysis.This work provides an efficient,green,and scalable synthesis method of the electrocatalyst for CO_(2) reduction to formate.
基金supported by the National Natural Science Foundation of China (Grant No. 20876125)the Research Fund for the Doctoral Program of Higher Education, China (Grant No. 20096101110013)the Northwest University Graduate Interdisciplinary Funds, China (Grant Nos. 09YJC24 and 09YJC27)
文摘A rare-earth free upconversion luminescent material, 10BaF2：NaF, Na3AIF6, is synthesized by a hydrothermal method. The study of fluorescent spectrum indicates that it can convert visible light （550 nm-610 nm） into ultraviolet light （290 nm 350 nm）, and two emission peaks at 304 nm and 324 nm are observed under the excitation of 583 nm at room temperature. Subsequently, 10BaF2：NaF, Na3AIF6/TiO2 composite photocatalyst is prepared and its catalytic activity is evaluated by the photocatalytic reduction of CO2 under visible light irradiation （λ〉 515 nm）. The results show that 10BaF2：NaF, Na3AIF6/TiO2 is a more effective photocatalyst for CO2 reduction than pure TiO2, their corresponding methanol yields are 179 and 0 μmol/g-cat under the same conditions. Additionally, the mechanism of photocatalytic reduction of CO2 on 10BaF2：NaF, Na3AIF6/TiO2 is proposed.
基金This study was supported by the Fundamental Research Funds for the Central Universities(Grant No.2022YJS053).
文摘As an important transportation infrastructure and transportation backbone in China,high-speed rail(HSR)plays a critical role in promoting the development of green and low-carbon transportation.Calculating the CO_(2) emissions reduction performance of HSR will be conduci v e to pr omote the CO_(2) emissions r eduction w ork of the r ail w ay.Based on the Dalkic HSR CO_(2) emissions r eduction performance model,by adjusting the HSR CO_(2) emission factor(CEF HSR),the annual times of departures(T)and other parameters,this study develops a Chinese HSR CO_(2) emissions reduction performance model.Taking the Beijing-Shanghai HSR as the resear c h object,this study conducts a questionnaire survey to explore the substitution effect and demand effect of HSR on different transportation modes;collects data such as passenger v olume,av era ge electricity use and annual times of departures of the Beijing-Shanghai HSR in 2019;and calculates the CO_(2) emissions reduction performance of the Beijing-Shanghai HSR.This study has two main results:(1)It builds a Chinese HSR CO_(2) emissions reduction performance model based on substitution effect and demand effect.(2)In 2019,the CO_(2) emissions of the Beijing-Shanghai HSR are 2898233.62 t,the CO_(2) emissions reduction performance of the Beijing-Shanghai HSR is 17999482.8 t,the annual CO_(2) emissions of the Beijing-Shanghai line in‘No HSR’case are 7.2 times as in the’HSR’case and the PKT of the HSR is 10.2 g/pkm.Based on the research results,this study proposes three CO_(2) emissions reduction policy suggestions.This study would be helpful for further HSR CO_(2) emissions reduction resear c h and departments related to railway transportation management to make CO_(2) emissions reduction policies.
基金Institute of Technological Research–IPT,Fundcao de AmparoàPesquisa do Estado de Sao PauloBrazil[Process 2019/05840-3]+1 种基金Conselho Nacional de Desenvolvimento Científico e TecnológicoBrazil[Process 167470/2018-3]。
文摘As part of efforts to reduce anthropogenic CO_(2) emissions by the steelmaking industry,this study investigated the direct reduction of industrially produced hematite pellets with H_(2) using the Doehlert experimental design to evaluate the effect of pellet diameter(10.5-16.5 mm),porosity(0.36-0.44),and temperature(600-1200℃).A strong interactive effect between temperature and pellet size was observed,indicating that these variables cannot be considered independently.The increase in temperature and decrease in pellet size considerably favor the reduction rate,while porosity did not show a relevant effect.The change in pellet size during the reduction was negligible,except at elevated temperatures due to crack formation.A considerable decrease in mechanical strength at high temperatures suggests a maximum process operating temperature of 900℃.Good predictive capacity was achieved using the modified grain model to simulate the three consecutive non-catalytic gas-solid reactions,considering different pellet sizes and porosities,changes during the reaction from 800 to 900℃.However,for other temperatures,different mechanisms of structural modifications must be considered in the modeling.These results represent significant contributions to the development of ore pellets for CO_(2)-free steelmaking technology.
